Search for ultralight scalar dark matter with atomic spectroscopy

We report new limits on ultralight scalar dark matter (DM) with dilaton-like couplings to photons that can induce oscillations in the fine-structure constant alpha. Atomic dysprosium exhibits an electronic structure with two nearly degenerate levels whose energy splitting is sensitive to changes in alpha. Spectroscopy data for two isotopes of dysprosium over a two-year span is analyzed for coherent oscillations with angular frequencies below 1 rad/s. No signal consistent with a DM coupling is identified, leading to new constraints on dilaton-like photon couplings over a wide mass range. Under the assumption that the scalar field comprises all of the DM, our limits on the coupling exceed those from equivalence-principle tests by up to 4 orders of magnitude for masses below 3 * 10^-18 eV. Excess oscillatory power, inconsistent with fine-structure variation, is detected in a control channel, and is likely due to a systematic effect. Our atomic spectroscopy limits on DM are the first of their kind, and leave substantial room for improvement with state-of-the-art atomic clocks.Comment: 5 pages, 4 figures; v2: references adde

Investigation of two-frequency Paul traps for antihydrogen production

Radio-frequency (rf) Paul traps operated with multifrequency rf trapping potentials provide the ability to independently confine charged particle species with widely different charge-to-mass ratios. In particular, these traps may find use in the field of antihydrogen recombination, allowing antiproton and positron clouds to be trapped and confined in the same volume without the use of large superconducting magnets. We explore the stability regions of two-frequency Paul traps and perform numerical simulations of small, multispecies charged-particle mixtures that indicate the promise of these traps for antihydrogen recombination.Comment: 11 pages, 10 figure

Microwave-free magnetometry with nitrogen-vacancy centers in diamond

We use magnetic-field-dependent features in the photoluminescence of negatively charged nitrogen-vacancy centers to measure magnetic fields without the use of microwaves. In particular, we present a magnetometer based on the level anti-crossing in the triplet ground state at 102.4 mT with a demonstrated noise floor of 6 nT/$\sqrt{\text{Hz}}$, limited by the intensity noise of the laser and the performance of the background-field power supply. The technique presented here can be useful in applications where the sensor is placed closed to conductive materials, e.g. magnetic induction tomography or magnetic field mapping, and in remote-sensing applications since principally no electrical access is needed.Comment: 5 pages, 4 figure

Novel Magnetic-Sensing Modalities with Nitrogen-Vacancy Centers in Diamond

In modern-day quantum metrology, quantum sensors are widely employed to detect weak magnetic fields or nanoscale signals. Quantum devices, exploiting quantum coherence, are inevitably connected to physical constants and can achieve accuracy, repeatability, and precision approaching fundamental limits. As a result, these sensors have shown utility in a wide range of research domains spanning both science and technology. A rapidly emerging quantum sensing platform employs atomic-scale defects in crystals. In particular, magnetometry using nitrogen-vacancy (NV) color centers in diamond has garnered increasing interest. NV systems possess a combination of remarkable properties, optical addressability, long coherence times, and biocompatibility. Sensors based on NV centers excel in spatial resolution and magnetic sensitivity. These diamond-based sensors promise comparable combination of high spatial resolution and magnetic sensitivity without cryogenic operation. The above properties of NV magnetometers promise increasingly integrated quantum measurement technology, as a result, they have been extensively developed with various protocols and find use in numerous applications spanning materials characterization, nuclear magnetic resonance (NMR), condensed matter physics, paleomagnetism, neuroscience and living systems biology, and industrial vector magnetometry. In this chapter, NV centers are explored for magnetic sensing in a number of contexts. In general, we introduce novel regimes for magnetic-field probes with NV ensembles. Specifically, NV centers are developed for sensitive magnetometers for applications where microwaves (MWs) are prohibitively invasive and operations need to be carried out under zero ambient magnetic field. The primary goal of our discussion is to improve the utility of these NV center-based magnetometers

Search for variation of the fine-structure constant and violation of Lorentz symmetry using atomic dysprosium

We report on the spectroscopy of radio-frequency transitions between nearly-degenerate, opposite-parity excited states in atomic dysprosium (Dy). Theoretical calculations predict that these states are very sensitive to variation of the fine-structure constant, $\alpha$, owing to large relativistic corrections of opposite sign for the opposite-parity levels. The near degeneracy reduces the relative precision necessary to place constraints on variation of $\alpha$ competitive with results obtained from the best atomic clocks in the world. Additionally, the existence of several abundant isotopes of Dy allows isotopic comparisons that suppress common-mode systematic errors. The frequencies of the 754-MHz transition in $^{164}$Dy and 235-MHz transition in $^{162}$Dy were measured over the span of two years. Linear variation of $\alpha$ is found to be $\dot{\alpha}/\alpha = (-5.8\pm6.9)\times10^{-17}$~yr$^{-1}$, consistent with zero. The same data are used to constrain the dimensionless parameter $k_\alpha$, characterizing a possible coupling of $\alpha$ to a changing gravitational potential. We find that $k_\alpha = (-5.5\pm5.2)\times10^{-7}$, essentially consistent with zero and the best constraint to date.The same data are used to report a joint test of local Lorentz invariance and the Einstein Equivalence Principle for electrons. We present many-body calculations which demonstrate that the energy splitting of these states is particularly sensitive to violations of both special and general relativity. Lorentz violation for electrons is limited at the level of $10^{-17}$, matching or improving the best laboratory and astrophysical limits by up to a factor of 10, and gravitational redshift anomalies for electrons to the level of $10^{-8}$. With some enhancements, our experiment may be sensitive to Lorentz violation at the level of $9\times 10^{-20}$.We also report measurements of the differential polarizability between the nearly degenerate, opposite parity states. The differential scalar and tensor polarizabilities due to additional states were measured for the $|M| = 7,\dots,10$ sublevels in $^{164}$Dy and $^{162}$Dy and determined to be \overline{\balpha}_{\sss BA}^{(0)} = 180\,(45)_\text{stat}\,(8)_\text{sys} mHz cm$^2$/V$^2$ and \overline{\balpha}_{\sss BA}^{(2)} = -163\,(65)_\text{stat}\,(5)_\text{sys} mHz cm$^2$/V$^2$, respectively. The average blackbody radiation induced Stark shift of the Zeeman spectrum was measured around 300 K and found to be $-34(4)$~mHz/K and $+29(4)$~mHz/K for the $^{164}$Dy and $^{162}$Dy isotopes, respectively. We conclude that ac-Stark related systematics will not limit the precision of a search for variation of the fine-structure constant, using dysprosium, down to the level of $|\dot{\alpha}/\alpha|=2.6\times10^{-17}$~yr$^{-1}$ for a one-year experiment

Eddy current imaging with an atomic radio-frequency magnetometer

We use a radio-frequency $^{85}$Rb alkali-vapor cell magnetometer based on a paraffin-coated cell with long spin-coherence time and a small, low-inductance driving coil to create highly resolved conductivity maps of different objects. We resolve sub-mm features in conductive objects, we characterize the frequency response of our technique, and by operating at frequencies up to 250 kHz we are able to discriminate between differently conductive materials based on the induced response. The method is suited to cover a wide range of driving frequencies and can potentially be used for detecting non-metallic objects with low DC conductivity.Comment: 6 pages, 4 figure

Constraints on exotic spin-dependent interactions between electrons from helium fine-structure spectroscopy

Agreement between theoretical calculations of atomic structure and spectroscopic measurements is used to constrain possible contribution of exotic spin-dependent interactions between electrons to the energy differences between states in helium-4. In particular, constraints on dipole-dipole interactions associated with the exchange of pseudoscalar bosons (such as axions or axion-like particles, ALPs) with masses $10^{-2}~{\rm eV} \lesssim m \lesssim 10^{4}~{\rm eV}$ are improved by a factor of $\sim 100$. The first atomic-scale constraints on several exotic velocity-dependent dipole-dipole interactions are established as well