Temperature dependence of the nitrogen-vacancy magnetic resonance in diamond

The temperature dependence of the magnetic resonance spectra of nitrogen-vacancy (NV-) ensembles in the range of 280-330 K was studied. Four samples prepared under different conditions were studied with NV- concentrations ranging from 10 ppb to 15 ppm. For all of these samples, the axial zero-field splitting (ZFS) parameter, D, was found to vary significantly with temperature, T, as dD/dT = -74.2(7) kHz/K. The transverse ZFS parameter, E, was non-zero (between 4 and 11 MHz) in all samples, and exhibited a temperature dependence of dE/(EdT) = -1.4(3) x 10^(-4) K^(-1). The results might be accounted for by considering local thermal expansion. The observation of the temperature dependence of the ZFS parameters presents a significant challenge for room-temperature diamond magnetometers and may ultimately limit their bandwidth and sensitivity.Comment: 5 pages, 2 figures, 1 tabl

From time series to superstatistics

Complex nonequilibrium systems are often effectively described by a `statistics of a statistics', in short, a `superstatistics'. We describe how to proceed from a given experimental time series to a superstatistical description. We argue that many experimental data fall into three different universality classes: chi^2-superstatistics (Tsallis statistics), inverse chi^2-superstatistics, and log-normal superstatistics. We discuss how to extract the two relevant well separated superstatistical time scales tau and T, the probability density of the superstatistical parameter beta, and the correlation function for beta from the experimental data. We illustrate our approach by applying it to velocity time series measured in turbulent Taylor-Couette flow, which is well described by log-normal superstatistics and exhibits clear time scale separation.Comment: 7 pages, 9 figure

Optical quenching and recovery of photoconductivity in single-crystal diamond

We study the photocurrent induced by pulsed-light illumination (pulse duration is several nanoseconds) of single-crystal diamond containing nitrogen impurities. Application of additional continuous-wave light of the same wavelength quenches pulsed photocurrent. Characterization of the optically quenched photocurrent and its recovery is important for the development of diamond based electronics and sensing

Nuclear-spin relaxation of 207^{207}Pb in ferroelectric powders

Motivated by a recent proposal by O. P. Sushkov and co-workers to search for a P,T-violating Schiff moment of the $^{207}$Pb nucleus in a ferroelectric solid, we have carried out a high-field nuclear magnetic resonance study of the longitudinal and transverse spin relaxation of the lead nuclei from room temperature down to 10 K for powder samples of lead titanate (PT), lead zirconium titanate (PZT), and a PT monocrystal. For all powder samples and independently of temperature, transverse relaxation times were found to be $T_2\approx 1.5$ms, while the longitudinal relaxation times exhibited a temperature dependence, with $T_1$ of over an hour at the lowest temperatures, decreasing to $T_1\approx 7$s at room temperature. At high temperatures, the observed behavior is consistent with a two-phonon Raman process, while in the low temperature limit, the relaxation appears to be dominated by a single-phonon (direct) process involving magnetic impurities. This is the first study of temperature-dependent nuclear-spin relaxation in PT and PZT ferroelectrics at such low temperatures. We discuss the implications of the results for the Schiff-moment search.Comment: 6 pages, 4 figure

Quantified Morphology of HI Disks in the Universe

he upcoming new perspective of the high redshift Universe in the 21 cm line of atomic hydrogen opens possibilities to explore topics of spiral disk evolution, hitherto reserved for the optical regime. The growth of spiral gas disks over Cosmic time can be explored with the new generation of radio telescopes, notably the SKA, and its precursors, as accurately as with the Hubble Space Telescope for stellar disks. Since the atomic hydrogen gas is the building block of these disks, it should trace their formation accurately. Morphology of HI disks can now equally be quantified over Cosmic time. In studies of HST deep fields, the optical or UV morphology of high-redshift galaxy disks have been characterized using a few quantities: concentration (C), asymmetry (A), smoothness (S), second-order-moment (M20), the GINI coefficient (G), and Ellipticity (E). We have applied these parameters across wavelengths and compared them to the HI morphology over the THINGS sample. NGC 3184, an unperturbed disk, and NGC 5194, the canonical 3:1 interaction, serve as examples for quantified morphology. We find that morphology parameters determined in HI are as good or better a tracer of interaction compared to those in any other wavelength, notably in Asymmetry, Gini and M20. This opens the possibility of using them in the parameterization pipeline for SKA precursor catalogues to select interacting or harassed galaxies from their HI morphology. Asymmetry, Gini and M20 may be redefined for use on data-cubes rather than HI column density image.Comment: 6 pages, 3 figures, proceeding of the conference "Panoramic Radio Astronomy: Wide-field 1-2 GHz research on galaxy evolution", June 02 - 05 2009, Groningen, update after small edit

Quantified HI Morphology II : Lopsidedness and Interaction in WHISP Column Density Maps

Lopsidedness of the gaseous disk of spiral galaxies is a common phenomenon in disk morphology, profile and kinematics. Simultaneously, the asymmetry of a galaxy's stellar disk, in combination with other morphological parameters, has seen extensive use as an indication of recent merger or interaction in galaxy samples. Quantified morphology of stellar spiral disks is one avenue to determine the merger rate over much of the age of the Universe. In this paper, we measure the quantitative morphology parameters for the HI column density maps from the Westerbork observations of neutral Hydrogen in Irregular and SPiral galaxies (WHISP). These are Concentration, Asymmetry, Smoothness, Gini, M20, and one addition of our own, the Gini parameter of the second order moment (GM). Our aim is to determine if lopsided or interacting disks can be identified with these parameters. Our sample of 141 HI maps have all previous classifications on their lopsidedness and interaction. We find that the Asymmetry, M20, and our new GM parameter correlate only weakly with the previous morphological lopsidedness quantification. These three parameters may be used to compute a probability that an HI disk is morphologically lopsided but not unequivocally to determine it. However, we do find that that the question whether or not an HI disk is interacting can be settled well using morphological parameters. Parameter cuts from the literature do not translate from ultraviolet to HI directly but new selection criteria using combinations of Asymmetry and M20 or Concentration and M20, work very well. We suggest that future all-sky HI surveys may use these parameters of the column density maps to determine the merger fraction and hence rate in the local Universe with a high degree of accuracy.Comment: 12 pages, 5 figures, 1 table, accepted by MNRAS, appendix not include

A nanoparticle catalyst for heterogeneous phase para-hydrogen-induced polarization in water.

Para-hydrogen-induced polarization (PHIP) is a technique capable of producing spin polarization at a magnitude far greater than state-of-the-art magnets. A significant application of PHIP is to generate contrast agents for biomedical imaging. Clinically viable and effective contrast agents not only require high levels of polarization but heterogeneous catalysts that can be used in water to eliminate the toxicity impact. Herein, we demonstrate the use of Pt nanoparticles capped with glutathione to induce heterogeneous PHIP in water. The ligand-inhibited surface diffusion on the nanoparticles resulted in a (1) H polarization of P=0.25% for hydroxyethyl propionate, a known contrast agent for magnetic resonance angiography. Transferring the (1) H polarization to a (13) C nucleus using a para-hydrogen polarizer yielded a polarization of 0.013%. The nuclear-spin polarizations achieved in these experiments are the first reported to date involving heterogeneous reactions in water