90 research outputs found

    Magnetization plateaux cascade in the frustrated quantum antiferromagnet Cs2_2CoBr4_4

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    We have found an unusual competition of two frustration mechanisms in the 2D quantum antiferromagnet Cs2_2CoBr4_4. The key actors are the alternation of single-ion planar anisotropy direction of the individual magnetic Co2+^{2+} ions, and their arrangement in a distorted triangular lattice structure. In particular, the uniquely oriented Ising-type anisotropy emerges from the competition of easy-plane ones, and for a magnetic field applied along this axis one finds a cascade of five ordered phases at low temperatures. Two of these phases feature magnetization plateaux. The low-field one is supposed to be a consequence of a collinear ground state stabilized by the anisotropy, while the other plateau bears characteristics of an "up-up-down" state exclusive for lattices with triangular exchange patterns. Such coexistence of the magnetization plateaux is a fingerprint of competition between the anisotropy and the geometric frustration in Cs2_2CoBr4_4.Comment: 10 pages, 8 figure

    Electron Spin Resonance in a Spin-1/2 Heisenberg Strong-rung Ladder

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    Cu(C8_8H6_6N2_2)Cl2_2, a strong-rung spin-1/2 Heisenberg ladder compound, is probed by means of electron spin resonance (ESR) spectroscopy in the field-induced gapless phase above Hc1H_{c1}. The temperature dependence of the ESR linewidth is analyzed in the quantum field theory framework, suggesting that the anisotropy of magnetic interactions plays a crucial role, determining the peculiar low-temperature ESR linewidth behavior. In particular, it is argued that the uniform Dzyaloshinskii-Moriya interaction (which is allowed on the bonds along the ladder legs) can be the source of this behavior in Cu(C8_8H6_6N2_2)Cl2_2

    Modes of magnetic resonance in the spin liquid phase of Cs2CuCl4

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    We report the observation of a frequency shift and splitting of the electron spin resonance (ESR) mode of the low-dimensional S=1/2 frustrated antiferromagnet Cs2CuCl4 in the spin-correlated state below the Curie-Weiss temperature 4 K but above the ordering temperature 0.62 K. The shift and splitting exhibit strong anisotropy with respect to the direction of the applied magnetic field and do not vanish in zero field. The low-temperature evolution of spin resonance response is a result of the specific modification of one-dimensional spinon continuum under the action of the uniform Dzyaloshinskii-Moriya interaction (DM) within the spin chains. Parameters of the uniform DM interaction are derived from the experiment.Comment: 10 pages, 12 figure

    Confinement of fractional excitations in a triangular lattice antiferromagnet

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    High-resolution neutron and THz spectroscopies are used to study the magnetic excitation spectrum of Cs2_2CoBr4_4, a distorted-triangular-lattice antiferromagnet with nearly XY-type anisotropy. What was previously thought of as a broad excitation continuum [Phys. Rev. Lett. 129, 087201 (2022)] is shown to be a series of dispersive bound states reminiscent of "Zeeman ladders" in quasi-one-dimensional Ising systems. At wave vectors where inter-chain interactions cancel at the Mean Field level, they can indeed be interpreted as bound finite-width kinks in individual chains. Elsewhere in the Brillouin zone their true two-dimensional structure and propagation are revealed.Comment: 11 pages, 8 figure

    Synthesis of phenanthridine derivatives

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