325 research outputs found

    Deterministic quantum state transfer from an electronic charge qubit to a photonic polarization qubit

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    Building on an earlier proposal for the production of polarization-entangled microwaves by means of intraband transitions in a pair of quantum dots, we show how this device can be used to transfer an unknown single-qubit state from electronic charge to photonic polarization degrees of freedom. No postselection is required, meaning that the quantum state transfer happens deterministically. Decoherence of the charge qubit causes a non-monotonic decay of the fidelity of the transferred state with increasing decoherence rate.Comment: 3 pages, 3 figure

    Determining the Electron-Phonon Coupling Strength in Correlated Electron Systems from Resonant Inelastic X-ray Scattering

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    We show that high resolution Resonant Inelastic X-ray Scattering (RIXS) provides direct, element-specific and momentum-resolved information on the electron-phonon (e-p) coupling strength. Our theoretical analysis demonstrates that the e-p coupling can be extracted from RIXS spectra by determining the differential phonon scattering cross section. An alternative, very direct manner to extract the coupling is to use the one and two-phonon loss ratio, which is governed by the e-p coupling strength and the core-hole life-time. This allows measurement of the e-p coupling on an absolute energy scale.Comment: 4 pages, 3 figure

    Bimagnon studies in cuprates with Resonant Inelastic X-ray Scattering at the O K edge. I - An assessment on La2CuO4 and a comparison with the excitation at Cu L3 and Cu K edges

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    We assess the capabilities of magnetic Resonant Inelastic X-ray Scattering (RIXS) at the O KK edge in undoped cuprates by taking La_{2}CuO_{4} as a benchmark case, based on a series of RIXS measurements that we present here. By combining the experimental results with basic theory we point out the fingerprints of bimagnon in the O KK edge RIXS spectra. These are a dominant peak around 450 meV, the almost complete absence of dispersion both with π\pi and σ\sigma polarization and the almost constant intensity vs. the transferred momentum with σ\sigma polarization. This behavior is quite different from Cu L3L_3 edge RIXS giving a strongly dispersing bimagnon tending to zero at the center of the Brillouin zone. This is clearly shown by RIXS measurements at the Cu L3L_3 edge that we present. The Cu L3L_3 bimagnon spectra and those at Cu KK edge - both from the literature and from our data - however, have the same shape. These similarities and differences are understood in terms of different sampling of the bimagnon continuum. This panorama points out the unique possibilities offered by O KK RIXS in the study of magnetic excitations in cuprates near the center of the BZ

    Momentum dependence of orbital excitations in Mott-insulating titanates

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    High-resolution resonant inelastic x-ray scattering has been used to determine the momentum dependence of orbital excitations in Mott-insulating LaTiO3_3 and YTiO3_3 over a wide range of the Brillouin zone. The data are compared to calculations in the framework of lattice-driven and superexchange-driven orbital ordering models. A superexchange model in which the experimentally observed modes are attributed to two-orbiton excitations yields the best description of the data.Comment: to appear in PR

    Measurement of magnetic excitations in the two-dimensional antiferromagnetic Sr2CuO2Cl2 insulator using resonant x-ray scattering:Evidence for extended interactions

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    Using high-resolution resonant inelastic x-ray scattering (RIXS), we performed a momentum-resolved study of magnetic excitations in the model spin-1/2 2D antiferromagnetic insulator Sr_2CuCl_2O_2. We identify both a single-spin-wave feature and a multi-magnon continuum, and show that the X-ray polarization can be used to distinguish these two contributions in the cross-section. The spin-waves display a large (70 meV) dispersion between the zone-boundary points (π\pi,0) and (π\pi/2,π\pi/2). Employing an extended tt-t′t'-t"t"-UU one-band Hubbard model, we find significant electronic hopping beyond nearest-neighbor Cu ions. We conclude that sizeable extended magnetic interactions are present in \scoc{} and probably important in all undoped cuprates.Comment: 4 pages, 4 figure

    Resonant Inelastic X-ray Scattering Studies of Elementary Excitations

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    In the past decade, Resonant Inelastic X-ray Scattering (RIXS) has made remarkable progress as a spectroscopic technique. This is a direct result of the availability of high-brilliance synchrotron X-ray radiation sources and of advanced photon detection instrumentation. The technique's unique capability to probe elementary excitations in complex materials by measuring their energy-, momentum-, and polarization-dependence has brought RIXS to the forefront of experimental photon science. We review both the experimental and theoretical RIXS investigations of the past decade, focusing on those determining the low-energy charge, spin, orbital and lattice excitations of solids. We present the fundamentals of RIXS as an experimental method and then review the theoretical state of affairs, its recent developments and discuss the different (approximate) methods to compute the dynamical RIXS response. The last decade's body of experimental RIXS data and its interpretation is surveyed, with an emphasis on RIXS studies of correlated electron systems, especially transition metal compounds. Finally, we discuss the promise that RIXS holds for the near future, particularly in view of the advent of x-ray laser photon sources.Comment: Review, 67 pages, 44 figure

    Dispersive charge density wave excitations and temperature dependent commensuration in Bi2Sr2CaCu2O8+{\delta}

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    Experimental evidence on high-Tc cuprates reveals ubiquitous charge density wave (CDW) modulations, which coexist with superconductivity. Although the CDW had been predicted by theory, important questions remain about the extent to which the CDW influences lattice and charge degrees of freedom and its characteristics as functions of doping and temperature. These questions are intimately connected to the origin of the CDW and its relation to the mysterious cuprate pseudogap. Here, we use ultrahigh resolution resonant inelastic x-ray scattering (RIXS) to reveal new CDW character in underdoped Bi2Sr2CaCu2O8+{\delta} (Bi2212). At low temperature, we observe dispersive excitations from an incommensurate CDW that induces anomalously enhanced phonon intensity, unseen using other techniques. Near the pseudogap temperature T*, the CDW persists, but the associated excitations significantly weaken and the CDW wavevector shifts, becoming nearly commensurate with a periodicity of four lattice constants. The dispersive CDW excitations, phonon anomaly, and temperature dependent commensuration provide a comprehensive momentum space picture of complex CDW behavior and point to a closer relationship with the pseudogap state
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