225 research outputs found

    Unbound states of 32Cl and the 31S(p,\gamma)32Cl reaction rate

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    The 31S(p,\gamma)32Cl reaction is expected to provide the dominant break-out path from the SiP cycle in novae and is important for understanding enrichments of sulfur observed in some nova ejecta. We studied the 32S(3He,t)32Cl charge-exchange reaction to determine properties of proton-unbound levels in 32Cl that have previously contributed significant uncertainties to the 31S(p,\gamma)32Cl reaction rate. Measured triton magnetic rigidities were used to determine excitation energies in 32Cl. Proton-branching ratios were obtained by detecting decay protons from unbound 32Cl states in coincidence with tritons. An improved 31S(p,\gamma)32Cl reaction rate was calculated including robust statistical and systematic uncertainties

    Measurement of \u3csup\u3e17\u3c/sup\u3eF + p reactions with ANASEN

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    Reactions involving radioactive nuclei play an important role in stellar explosions, but those reactions involving short-lived nuclei have only limited experimental information available due to currently limited beam intensities. Several facilities are aiming to provide greater access to these unstable isotopes at higher beam intensities, but more efficient and selective techniques and devices are needed to properly study these important reactions. The Array for Nuclear Astrophysics Studies with Exotic Nuclei (ANASEN), a charged particle detector designed by Louisiana State University (LSU) and Florida State University (FSU), was created for this purpose. ANASEN is used to study the reactions important in the αp- and rp- processes with proton-rich exotic nuclei, providing essentially complete solid angle coverage through an array of 40 silicon-strip detectors backed with CsI scintillators, covering an area of roughly 1300 cm2. ANASEN also includes an active gas target/detector in a position-sensitive annular gas proportional counter, which allows direct measurement of (α,p) reactions in inverse kinematics. The first in-beam measurements with a partial implementation of ANASEN were performed at the RESOLUT radioactive beam facility of FSU during the summer of 2011. They included stable beam experiments and measurements of the 17F(p,p) 17F and 17F(p,α)14O reactions which are important to understanding the structure of 18Ne and the 14O(α,p)17F reaction rate. The performance of ANASEN and initial results from the 17F studies will be presented. © Published under licence by IOP Publishing Ltd

    Clustering in non-self-conjugate nuclei \u3csup\u3e10\u3c/sup\u3eBe and \u3csup\u3e18\u3c/sup\u3eO

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    Clustering phenomena in 10Be and 18O were studied by means of resonance elastic scattering of α-particles on 6He and 14C. Excitation functions for α+6He and α+14C were measured and detailed R-matrix analyses of the excitation functions was performed. We compare the experimental results with the predictions of modern theoretical approaches and discuss properties of cluster rotational bands

    Clustering in A=10 nuclei

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    We discuss the identification and properties of the states that belong to the highly clustered rotational band in A=10 nuclei, 10Be, 10B(T=1) and 10C. The band is of interest because it may correspond to an exotic α:nn:α configuration

    Heparan Sulfate Domains Required for Fibroblast Growth Factor 1 and 2 Signaling through Fibroblast Growth Factor Receptor 1c

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    A small library of well defined heparan sulfate (HS) polysaccharides was chemoenzymatically synthesized and used for a detailed structure-activity study of fibroblast growth factor (FGF) 1 and FGF2 signaling through FGF receptor (FGFR) 1c. The HS polysaccharide tested contained both undersulfated (NA) domains and highly sulfated (NS) domains as well as very well defined non-reducing termini. This study examines differences in the HS selectivity of the positive canyons of the FGF12-FGFR1c2 and FGF22-FGFR1c2 HS binding sites of the symmetric FGF2-FGFR2-HS2 signal transduction complex. The results suggest that FGF12-FGFR1c2 binding site prefers a longer NS domain at the non-reducing terminus than FGF22-FGFR1c2. In addition, FGF22-FGFR1c2 can tolerate an HS chain having an N-acetylglucosamine residue at its non-reducing end. These results clearly demonstrate the different specificity of FGF12-FGFR1c2 and FGF22-FGFR1c2 for well defined HS structures and suggest that it is now possible to chemoenzymatically synthesize precise HS polysaccharides that can selectively mediate growth factor signaling. These HS polysaccharides might be useful in both understanding and controlling the growth, proliferation, and differentiation of cells in stem cell therapies, wound healing, and the treatment of cancer

    Experimental Investigation of the Ne 19 (p,γ)20Na Reaction Rate and Implications for Breakout from the Hot CNO Cycle

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    The Ne19(p,γ)Na20 reaction is the second step of a reaction chain which breaks out from the hot CNO cycle, following the O15(α,γ)Ne19 reaction at the onset of x-ray burst events. We investigate the spectrum of the lowest proton-unbound states in Na20 in an effort to resolve contradictions in spin-parity assignments and extract reliable information about the thermal reaction rate. The proton-transfer reaction Ne19(d,n)Na20 is measured with a beam of the radioactive isotope Ne19 at an energy around the Coulomb barrier and in inverse kinematics. We observe three proton resonances with the Ne19 ground state, at 0.44, 0.66, and 0.82 MeV c.m. energies, which are assigned 3+, 1+, and (0+), respectively. In addition, we identify two resonances with the first excited state in Ne19, one at 0.20 MeV and one, tentatively, at 0.54 MeV. These observations allow us for the first time to experimentally quantify the astrophysical reaction rate on an excited nuclear state. Our experiment shows an efficient path for thermal proton capture in Ne19(p,γ)Na20, which proceeds through ground state and excited-state capture in almost equal parts and eliminates the possibility for this reaction to create a bottleneck in the breakout from the hot CNO cycle

    Synthesis of Uridine 5′-diphosphoiduronic Acid: A Potential Substrate for the Chemoenzymatic Synthesis of Heparin

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    An improved understanding of the biological activities of heparin requires structurally defined heparin oligosaccharides. The chemoenzymatic synthesis of heparin oligosaccharides relies on glycosyltransferases that use UDP-sugar nucleotides as donors. Uridine 5′-diphosphoiduronic acid (UDP-IdoA) and uridine 5′-diphosphohexenuronic acid (UDP-HexUA) have been synthesized as potential analogues of uridine 5′-diphosphoglucuronic acid (UDP-GlcA) for enzymatic incorporation into heparin oligosaccharides. Non-natural UDP-IdoA and UDP-HexUA were tested as substrates for various glucuronosyltransferases to better understand enzyme specificity

    γ spectroscopy of states in Cl 32 relevant for the S 31 (p,γ) Cl 32 reaction rate

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    Background: The S31(p,γ)Cl32 reaction becomes important for sulfur production in novae if the P31(p,α)Si28 reaction rate is somewhat greater than currently accepted. The rate of the S31(p,γ)Cl32 reaction is uncertain, primarily due to the properties of resonances at Ec.m.=156 and 549 keV. Purpose: We precisely determined the excitation energies of states in Cl32 through high-resolution γ spectroscopy including the two states most important for the S31(p,γ)Cl32 reaction at nova temperatures. Method: Excited states in Cl32 were populated using the B10(Mg24,2n)Cl32 reaction with a Mg24 beam from the ATLAS facility at Argonne National Laboratory. The reaction channel of interest was selected using recoils in the Fragment Mass Analyzer, and precise level energies were determined by detecting γ rays with Gammasphere. Results: We observed γ rays from the decay of six excited states in Cl32. The excitation energies for two unbound levels at Ex=1738.1 (6) keV and 2130.5 (10) keV were determined and found to be in agreement with a previous high-precision measurement of the S32(He3,t)Cl32 reaction [1]. Conclusions: An updated S31(p,γ)Cl32 reaction rate is presented. With the excitation energies of important levels firmly established, the dominant uncertainty in the reaction rate at nova temperatures is due to the strength of the resonance corresponding to the 2131-keV state in Cl32

    Measurement of F 17 (d,n) Ne 18 and the impact on the F 17 (p,γ) Ne 18 reaction rate for astrophysics

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    Background: The F17(p,γ)Ne18 reaction is part of the astrophysical hot CNO cycles that are important in astrophysical environments like novas. Its thermal reaction rate is low owing to the relatively high energy of the resonances and therefore is dominated by direct, nonresonant capture in stellar environments at temperatures below 0.4 GK. Purpose: An experimental method is established to extract the proton strength to bound and unbound states in experiments with radioactive ion beams and to determine the parameters of direct and resonant capture in the F17(p,γ)Ne18 reaction. Method: The F17(d,n)Ne18 reaction is measured in inverse kinematics using a beam of the short-lived isotope F17 and a compact setup of neutron, proton, γ-ray, and heavy-ion detectors called resoneut. Results: The spectroscopic factors for the lowest l=0 proton resonances at Ec.m.=0.60 and 1.17 MeV are determined, yielding results consistent within 1.4σ of previous proton elastic-scattering measurements. The asymptotic normalization coefficients of the bound 21+ and 22+ states in Ne18 are determined and the resulting direct-capture reaction rates are extracted. Conclusions: The direct-capture component of the F17(p,γ)Ne18 reaction is determined for the first time from experimental data on Ne18
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