38,925 research outputs found

    Spectrum of the gamma-ray diffuse component observed from HEAO-1

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    The spectrum of the diffuse X and gamma ray background was measured between 15 keV and 4 MeV with the scintillation detectors aboard the HEAO 1 satellite. The apertures of the detectors were modulated on time scales of hours and the difference in counting rates measured the diffuse component flux. The observed spectrum is presented and compared with other measurements. At least two components are indicated, one below -100 keV and the other above. Possible origins are discussed

    Strong electron correlations in cobalt valence tautomers

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    We have examined cobalt based valence tautomer molecules such as Co(SQ)2_2(phen) using density functional theory (DFT) and variational configuration interaction (VCI) approaches based upon a model Hamiltonian. Our DFT results extend earlier work by finding a reduced total energy gap (order 0.6 eV) between high temperature and low temperature states when we fully relax the coordinates (relative to experimental ones). Futhermore we demonstrate that the charge transfer picture based upon formal valence arguments succeeds qualitatively while failing quantitatively due to strong covalency between the Co 3dd orbitals and ligand pp orbitals. With the VCI approach, we argue that the high temperature, high spin phase is strongly mixed valent, with about 30 % admixture of Co(III) into the predominantly Co(II) ground state. We confirm this mixed valence through a fit to the XANES spectra. Moreover, the strong electron correlations of the mixed valent phase provide an energy lowering of about 0.2-0.3 eV of the high temperature phase relative to the low temperature one. Finally, we use the domain model to account for the extraordinarily large entropy and enthalpy values associated with the transition.Comment: 10 pages, 4 figures, submitted to J. Chem. Phy

    Spinor Dynamics in an Antiferromagnetic Spin-1 Condensate

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    We observe coherent spin oscillations in an antiferromagnetic spin-1 Bose-Einstein condensate of sodium. The variation of the spin oscillations with magnetic field shows a clear signature of nonlinearity, in agreement with theory, which also predicts anharmonic oscillations near a critical magnetic field. Measurements of the magnetic phase diagram agree with predictions made in the approximation of a single spatial mode. The oscillation period yields the best measurement to date of the sodium spin-dependent interaction coefficient, determining that the difference between the sodium spin-dependent s-wave scattering lengths af=2af=0a_{f=2}-a_{f=0} is 2.47±0.272.47\pm0.27 Bohr radii.Comment: 5 pages, 2 figures. Changes: added reference, minor correction

    Dynamics of a deformable body in a fast flowing soap film

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    We study the behavior of an elastic loop embedded in a flowing soap film. This deformable loop is wetted into the film and is held fixed at a single point against the oncoming flow. We interpret this system as a two-dimensional flexible body interacting in a two-dimensional flow. This coupled fluid-structure system shows bistability, with both stationary and oscillatory states. In its stationary state, the loop remains essentially motionless and its wake is a von K\'arm\'an vortex street. In its oscillatory state, the loop sheds two vortex dipoles, or more complicated vortical structures, within each oscillation period. We find that the oscillation frequency of the loop is linearly proportional to the flow velocity, and that the measured Strouhal numbers can be separated based on wake structure

    Standing wave oscillations in binary mixture convection: from onset via symmetry breaking to period doubling into chaos

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    Oscillatory solution branches of the hydrodynamic field equations describing convection in the form of a standing wave (SW) in binary fluid mixtures heated from below are determined completely for several negative Soret coefficients. Galerkin as well as finite-difference simulations were used. They were augmented by simple control methods to obtain also unstable SW states. For sufficiently negative Soret coefficients unstable SWs bifurcate subcritically out of the quiescent conductive state. They become stable via a saddle-node bifurcation when lateral phase pinning is exerted. Eventually their invariance under time-shift by half a period combined with reflexion at midheight of the fluid layer gets broken. Thereafter they terminate by undergoing a period-doubling cascade into chaos

    Bias Dependent 1/f Conductivity Fluctuations in Low-Doped La1x_{1-x}Cax_{x}MnO3_3 Manganite Single Crystals

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    Low frequency noise in current biased La0.82_{0.82}Ca0.18_{0.18}MnO3_{3} single crystals has been investigated in a wide temperature range from 79 K to 290 K. Despite pronounced changes in magnetic properties and dissipation mechanisms of the sample with changing temperature, the noise spectra were found to be always of the 1/f type and their intensity (except the lowest temperature studied) scaled as a square of the bias. At liquid nitrogen temperatures and under bias exceeding some threshold value, the behavior of the noise deviates from the quasi-equilibrium modulation noise and starts to depend in a non monotonic way on bias. It has been verified that the observed noise obeys Dutta and Horn model of 1/f noise in solids. The appearance of nonequilibrium 1/f noise and its dependence on bias have been associated with changes in the distribution of activation energies in the underlying energy landscape. These changes have been correlated with bias induced changes in the intrinsic tunneling mechanism dominating dissipation in La0.82_{0.82}Ca0.18_{0.18}MnO3_{3} at low temperatures.Comment: Accepted for publication in the Journal of Applied Physic

    Spectroscopic Evidence for Anisotropic S-Wave Pairing Symmetry in MgB2

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    Scanning tunneling spectroscopy of superconducting MgB2_2 (Tc=39T_c = 39 K) were studied on high-density pellets and c-axis oriented films. The sample surfaces were chemically etched to remove surface carbonates and hydroxides, and the data were compared with calculated spectra for all symmetry-allowed pairing channels. The pairing potential (Δk\Delta_k) is best described by an anisotropic s-wave pairing model, with Δk=Δxysin2θk+Δzcos2θk\Delta_k = \Delta_{xy} \sin ^2 \theta_k + \Delta_z \cos ^2 \theta_k, where θk\theta_k is the angle relative to the crystalline c-axis, Δz8.0\Delta_z \sim 8.0 meV, and Δxy5.0\Delta_{xy} \sim 5.0 meV.Comment: 4 pages and 3 figures. Submitted to Physical Review Letters. Corresponding author: Nai-Chang Yeh (e-mail: [email protected]

    Nonequilibrium 1/f Noise in Low-doped Manganite Single Crystals

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    1/f noise in current biased La0.82Ca0.18MnO3 crystals has been investigated. The temperature dependence of the noise follows the resistivity changes with temperature suggesting that resistivity fluctuations constitute a fixed fraction of the total resistivity, independently of the dissipation mechanism and magnetic state of the system. The noise scales as a square of the current as expected for equilibrium resistivity fluctuations. However, at 77 K at bias exceeding some threshold, the noise intensity starts to decrease with increasing bias. The appearance of nonequilibrium noise is interpreted in terms of bias dependent multi-step indirect tunneling.Comment: 4pages, 3figures,APL accepte

    Statistics of transition times, phase diffusion and synchronization in periodically driven bistable systems

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    The statistics of transitions between the metastable states of a periodically driven bistable Brownian oscillator are investigated on the basis of a two-state description by means of a master equation with time-dependent rates. The results are compared with extensive numerical simulations of the Langevin equation for a sinusoidal driving force. Very good agreement is achieved both for the counting statistics of the number of transitions and the residence time distribution of the process in either state. The counting statistics corroborate in a consistent way the interpretation of stochastic resonance as a synchronisation phenomenon for a properly defined generalized Rice phase.Comment: 15 pages, 9 figure
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