Pressure effects in the triangular layered cobaltites NaxCoO2

We have measured transport properties as a function of temperature and pressure up to 30GPa in the NaxCoO2 system. For the x=0.5 sample the transition temperature at 53K increases with pressure, while paradoxically the sample passes from an insulating to a metallic ground state. A similar transition is observed in the x=0.31 sample under pressure. Compression on the x=0.75 sample transforms the sample from a metallic to an insulating state. We discuss our results in terms of interactions between band structure effects and Na+ order.Comment: 18 pages, 5 figure

Mott-Hubbard quantum criticality in paramagnetic CMR pyrochlores

We present a correlated {\it ab initio} description of the paramagnetic phase of Tl$_2$Mn$_2$O$_7$, employing a combined local density approximation (LDA) with multiorbital dynamical mean field theory (DMFT) treatment. We show that the insulating state observed in this colossal magnetoresistance (CMR) pyrochlore is determined by strong Mn intra- and inter-orbital local electron-electron interactions. Hybridization effects are reinforced by the correlation-induced spectral weight transfer. Our result coincides with optical conductivity measurements, whose low energy features are remarkably accounted for by our theory. Based on this agreement, we study the disorder-driven insulator-metal transition of doped compounds, showing the proximity of Tl$_2$Mn$_2$O$_7$ to quantum phase transitions, in agreement with recent measurements.Comment: 4 pages, 4 figure

Pressure control of conducting channels in singlewall nanotube networks

We measure electrical transport on networks of single wall nanotube ropes as a function of temperature T, voltage V and pressure up to 22GPa. We observe Luttinger liquid (LL) behavior, a conductance ~T^alpha and a dynamic conductance ~V^alpha. With pressure conductance increases while alpha decreases, enabling us to test the theoretical prediction for LL on the alpha dependence of the T and V independent coefficient of the tunneling conductance, and to obtain the high frequency cut-off of LL modes. The possible transition to a fermi liquid at alpha -> 0 is unattainable, as nanotubes collapse to an insulating state at high pressures.Comment: 13 pages, 4 figure

Strong enhancement of superconductivity at high pressures within the charge-density-wave states of 2H-TaS 2 and 2H-TaSe 2

We present measurements of the superconducting and charge density wave critical temperatures (Tc and TCDW) as a function of pressure in the transition metal dichalchogenides 2H-TaSe2 and 2H-TaS2. Resistance and susceptibility measurements show that Tc increases from temperatures below 1 K up to 8.5 K at 9.5 GPa in 2H-TaS2 and 8.2 K at 23 GPa in 2H-TaSe2. We observe a kink in the pressure dependence of TCDW at about 4 GPa that we attribute to the lock-in transition from incommensurate CDW to commensurate CDW. Above this pressure, the commensurate TCDW slowly decreases coexisting with superconductivity within our full pressure range.Comment: Published in Phys. Rev B 93, 184512 (2016

Novel Phases of Planar Fermionic Systems

We discuss a {\em family} of planar (two-dimensional) systems with the following phase strucure: a Fermi liquid, which goes by a second order transition (with non classical exponent even in mean-field) to an intermediate, inhomogeneous state (with nonstandard ordering momentum) , which in turn goes by a first order transition to a state with canonical order parameter. We analyze two examples: (i) a superconductor in a parallel magnetic field (which was discussed independently by Bulaevskii)for which the inhomogeneous state is obtained for $1.86 T_c \stackrel{\sim}{<} B \stackrel{\sim}{<} 1.86 \sqrt{2} T_c$ where $T_c$ is the critical temperature (in Kelvin) of the superconductor without a field and $B$ is measured in Tesla, and (ii) spinless (or, as is explained, spin polarized) fermions near half-filling where a similar, sizeable window (which grows in size with anisotropy) exists for the intermediate CDW phase at an ordering momentum different from $(\pi , \pi )$. We discuss the experimental conditions for realizing and observing these phases and the Renormalization Group approach to the transitions.Comment: ([email protected],[email protected]) 29 p Latex 4 figs uuencoded separatel

Estudio experimental de procesos de calentamiento y enfriamiento. Resultados e implicaciones didácticas

A detailed experimental study on different processes of heating and cooling allows to deduce that temperature variation, in these processes, in the course of time is not always the same, but it depends, to a great extent, on how the process is carried out. So to confuse the T-Q relations (always lineal) wirth T-t relations (dependent on the process) is a mistake that is necessary to avoid in our classes

Interlayer Magnetic Frustration in Quasi-stoichiometric Li1-xNi1+xO2

Susceptibility, high-field magnetization and submillimeter wave electron spin resonance measurements of layered quasi-stoichiometric Li1-xNi1+xO2 are reported and compared to isomorphic NaNiO2. A new mechanism of magnetic frustration induced by the excess Ni ions always present in the Li layers is proposed. We finally comment on the possible realization of an orbital liquid state in this controversial compound.Comment: 4 pages, 5 figures, submitted to Phys.Rev.B, Rapid Com

New Superhard Phases for 3D C60-based Fullerites

We have explored new possible phases of 3D C60-based fullerites using semiempirical potentials and ab-initio density functional methods. We have found three closely related structures - two body centered orthorhombic and one body centered cubic - having 52, 56 and 60 tetracoordinated atoms per molecule. These 3D polymers result in semiconductors with bulk moduli near 300 GPa, and shear moduli around 240 GPa, which make them good candidates for new low density superhard materials.Comment: To be published in Physical Review Letter