Nano-film functionalized exposed core fibers enabling resonance-driven dispersive wave tailoring

Light sources with specific optical properties are the backbone of optical technologies such as spectroscopy or hyperspectral imaging. Yet, the creation of broadband, stable, and spectrally flat light sources, especially at low pump energies, remains a particular challenge. Supercontinuum generation (SCG) is a well-established method for broadband light generation in optical fibers. For tailorable SCG spectra, it is essential to accurately design and precisely control the dispersion of fibers with new methods. This thesis aims to explore nonlinear frequency conversion in resonance-enhanced fibers to create tunable broadband light sources with tailored properties at low pump energies. By depositing high refractive index nano-films with different thicknesses on the surface of the exposed fiber core, the dispersion of the fibers and thus the output spectrum of SCG can be tuned. Different nano-film geometries are investigated, featuring TiO2 nano-films with a uniform thickness, Ta2O5 nano-films with a gradually increasing thickness along the fiber length, and periodically structured Ta2O5 nano-films. Experiments and simulations reveal the advantages of a longitudinally varying dispersion over uniformly coated fibers concerning an enhanced spectral flatness and an enlarged bandwidth. Furthermore, periodically structured nano-films lead to multi-color tailorable higher-order dispersive waves via quasi phase-matching, which are outside of the wavelength range of classical soliton-based SCG. Resonance-based modifications of the fiber dispersion by using nano-films are a powerful new tool to efficiently shape nonlinear frequency conversion in SCG even at low pump energies. It has high technological potential for the realization of novel, ultrafast, broadband, and stable nonlinear light sources for biophotonics, environmental, life sciences, medical diagnostics, and metrology

Electric current-driven spectral tunability of surface plasmon polaritons in gold coated tapered fibers

Here we introduce the concept of electrically tuning surface plasmon polaritons using current-driven heat dissipation, allowing controlling plasmonic properties via a straightforward-to-access quantity. The key idea is based on an electrical current flowing through the plasmonic layer, changing plasmon dispersion and phase-matching condition via a temperature-imposed modification of the refractive index of one of the dielectric media involved. This scheme was experimentally demonstrated on the example of an electrically connected plasmonic fiber taper that has sensitivities >50000 nm/RIU. By applying a current, dissipative heat generated inside metal film heats the surrounding liquid, reducing its refractive index correspondingly and thus modifying the phase-matching condition to the fundamental taper mode. We observed spectral shifts of the plasmonic resonance up to 300 nm towards shorter wavelength by an electrical power of ≤ 80 mW, clearly showing that our concept is important for applications that demand precise real-time and external control on plasmonic dispersion and resonance wavelengths

Understanding Nonlinear Pulse Propagation in Liquid Strand-Based Photonic Bandgap Fibers

Ultrafast supercontinuum generation crucially depends on the dispersive properties of the underlying waveguide. This strong dependency allows for tailoring nonlinear frequency conversion and is particularly relevant in the context of waveguides that include geometry-induced resonances. Here, we experimentally uncovered the impact of the relative spectral distance between the pump and the bandgap edge on the supercontinuum generation and in particular on the dispersive wave formation on the example of a liquid strand-based photonic bandgap fiber. In contrast to its air-hole-based counterpart, a bandgap fiber shows a dispersion landscape that varies greatly with wavelength. Particularly due to the strong dispersion variation close to the bandgap edges, nanometer adjustments of the pump wavelength result in a dramatic change of the dispersive wave generation (wavelength and threshold). Phase-matching considerations confirm these observations, additionally revealing the relevance of third order dispersion for interband energy transfer. The present study provides additional insights into the nonlinear frequency conversion of resonance-enhanced waveguide systems which will be relevant for both understanding nonlinear processes as well as for tailoring the spectral output of nonlinear fiber sources

Electric current-driven spectral tunability of surface plasmon polaritons in gold coated tapered fibers

Here we introduce the concept of electrically tuning surface plasmon polaritons using current-driven heat dissipation, allowing controlling plasmonic properties via a straightforward-to-access quantity. The key idea is based on an electrical current flowing through the plasmonic layer, changing plasmon dispersion and phase-matching condition via a temperature-imposed modification of the refractive index of one of the dielectric media involved. This scheme was experimentally demonstrated on the example of an electrically connected plasmonic fiber taper that has sensitivities >50000 nm/RIU. By applying a current, dissipative heat generated inside metal film heats the surrounding liquid, reducing its refractive index correspondingly and thus modifying the phase-matching condition to the fundamental taper mode. We observed spectral shifts of the plasmonic resonance up to 300 nm towards shorter wavelength by an electrical power of ≤ 80 mW, clearly showing that our concept is important for applications that demand precise real-time and external control on plasmonic dispersion and resonance wavelengths

Understanding Nonlinear Pulse Propagation in Liquid Strand-Based Photonic Bandgap Fibers

Ultrafast supercontinuum generation crucially depends on the dispersive properties of the underlying waveguide. This strong dependency allows for tailoring nonlinear frequency conversion and is particularly relevant in the context of waveguides that include geometry-induced resonances. Here, we experimentally uncovered the impact of the relative spectral distance between the pump and the bandgap edge on the supercontinuum generation and in particular on the dispersive wave formation on the example of a liquid strand-based photonic bandgap fiber. In contrast to its air-hole-based counterpart, a bandgap fiber shows a dispersion landscape that varies greatly with wavelength. Particularly due to the strong dispersion variation close to the bandgap edges, nanometer adjustments of the pump wavelength result in a dramatic change of the dispersive wave generation (wavelength and threshold). Phase-matching considerations confirm these observations, additionally revealing the relevance of third order dispersion for interband energy transfer. The present study provides additional insights into the nonlinear frequency conversion of resonance-enhanced waveguide systems which will be relevant for both understanding nonlinear processes as well as for tailoring the spectral output of nonlinear fiber sources

Resonance-Induced Dispersion Tuning for Tailoring Nonsolitonic Radiation via Nanofilms in Exposed Core Fibers

Efficient supercontinuum generation demands for fine-tuning of the dispersion of the underlying waveguide. Resonances introduced into waveguide systems can substantially improve nonlinear dynamics in ultrafast supercontinuum generation via modal hybridization and formation of avoided crossings. Using the example of exposed core fibers functionalized by nanofilms with sub-nanometer precision both zero-dispersion and dispersive wave emission wavelengths are shifted by 227 and 300 nm, respectively, at tuning slopes higher than 20 nm/nm. The presented concept relies on dispersion management via induced resonances and can be straightforwardly extended to other deposition techniques and film geometries such as multilayers or 2D materials. It allows for the creation of unique dispersion landscapes, thus tailoring nonlinear dynamics and emission wavelengths and for making otherwise unsuitable waveguides relevant for ultrafast nonlinear photonics. © 2020 The Authors. Published by WILEY-VCH Verlag GmbH & Co. KGaA, Weinhei