217 research outputs found

    High-order Harmonic Generation and Dynamic Localization in a driven two-level system, a non-perturbative solution using the Floquet-Green formalism

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    We apply the Floquet-Green operator formalism to the case of a harmonically-driven two-level system. We derive exact expressions for the quasi-energies and the components of the Floquet eigenstates with the use of continued fractions. We study the avoided crossings structure of the quasi-energies as a function of the strength of the driving field and give an interpretation in terms of resonant multi-photon processes. From the Floquet eigenstates we obtain the time-evolution operator. Using this operator we study Dynamic Localization and High-order Harmonic Generation in the non-perturbative regime

    Theory of high-order harmonic generation by an elliptically polarized laser field

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    We generalize a recently formulated theory of high-order harmonic generation by low-frequency laser fields [Anne L'Huillier et al., Phys. Rev. A 48, R3433 (1993)] to the case of an elliptically polarized light. Our theoretical description includes both the single-atom response and propagation. Phase matching significantly modifies the results obtained in the single-atom response. The results of our calculations, including propagation for both the intensity and polarization properties of harmonics as a function of laser ellipticity, compare very well with recent experimental observations

    Two-photon double ionization of neon using an intense attosecond pulse train

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    We present the first demonstration of two-photon double ionization of neon using an intense extreme ultraviolet (XUV) attosecond pulse train (APT) in a photon energy regime where both direct and sequential mechanisms are allowed. For an APT generated through high-order harmonic generation (HHG) in argon we achieve a total pulse energy close to 1 μ\muJ, a central energy of 35 eV and a total bandwidth of 30\sim30 eV. The APT is focused by broadband optics in a neon gas target to an intensity of 310123\cdot10^{12} W\cdotcm2^{-2}. By tuning the photon energy across the threshold for the sequential process the double ionization signal can be turned on and off, indicating that the two-photon double ionization predominantly occurs through a sequential process. The demonstrated performance opens up possibilities for future XUV-XUV pump-probe experiments with attosecond temporal resolution in a photon energy range where it is possible to unravel the dynamics behind direct vs. sequential double ionization and the associated electron correlation effects

    Attosecond pulse trains generated using two color laser fields

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    We investigate the spectral and temporal structure of high harmonic emission from argon exposed to an infrared laser field and its second harmonic. For a wide range of generating conditions, trains of attosecond pulses with only one pulse per infrared cycle are generated. The synchronization necessary for producing such trains ensures that they have a stable pulse-to-pulse carrier envelope phase, unlike trains generated from one color fields, which have two pulses per cycle and a pi phase shift between consecutive pulses. Our experiment extends the generation of phase stabilized few cycle pulses to the extreme ultraviolet regime

    Spatio-temporal coupling of attosecond pulses

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    The shortest light pulses produced to date are of the order of a few tens of attoseconds, with central frequencies in the extreme ultraviolet range and bandwidths exceeding tens of eV. They are often produced as a train of pulses separated by half the driving laser period, leading in the frequency domain to a spectrum of high, odd-order harmonics. As light pulses become shorter and more spectrally wide, the widely-used approximation consisting in writing the optical waveform as a product of temporal and spatial amplitudes does not apply anymore. Here, we investigate the interplay of temporal and spatial properties of attosecond pulses. We show that the divergence and focus position of the generated harmonics often strongly depend on their frequency, leading to strong chromatic aberrations of the broadband attosecond pulses. Our argumentation uses a simple analytical model based on Gaussian optics, numerical propagation calculations and experimental harmonic divergence measurements. This effect needs to be considered for future applications requiring high quality focusing while retaining the broadband/ultrashort characteristics of the radiation

    Ionization and fragmentation of C-60 via multiphoton-multiplasmon excitation

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    We study the intensity dependence of ionization and fragmentation of buckminsterfullerene (C-60) in strong laser fields. Our data provide strong evidence that at intensities less than or similar to 10(14) W/cm(2) these processes occur predominantly via multiphoton excitation of the 20 eV plasmon resonance of C-60 At least two plasmons have to be created to initiate fragmentation or multiple ionization
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