Concentration- and thickness-dependent magnetic properties of NixMn100−x in epitaxially grown NixMn100−x/Ni/(Co/)Cu3Au(001)

Magnetic proximity effects in single-crystalline NixMn100x/Ni(/Co) bilayers on Cu3Au.001/ are investigated for in-plane (IP) and out-of-plane (OoP) magnetization by means of the longitudinal and polar magneto-optical Kerr effect. Attention is paid to the influence on concentration- and thickness- dependent antiferromagnetic ordering (TAFM) and blocking (Tb) temperatures as well as the exchange bias field (Heb). For all the NixMn100x films under study in contact with IP Ni, increasing TAFM is observed with decreasing Ni concentration from 50 to 20%, whereas only a slight change in TAFM is observed for the OoP case. Between 28% and 35% Ni concentration, a crossover temperature exists below which TAFM for the IP samples is higher than for the OoP samples and vice versa. Tb is higher for the IP case than for OoP, except for an equi-atomic NiMn film, while Heb increases significantly for both magnetization directions with decreasingx. These results are attributed to: (i) a rotation of the non-collinear 3Q-like spin structure of NixMn100-x from the more-OoP to the more-IP direction for decreasing Ni concentrationx, along with an associated increased magnetic anisotropy, and (ii) a smaller domain wall width within the NixMn100-x films at smaller x, leading to a smaller thickness required to establish exchange bias at a fixed temperature

Influence of topography and Co domain walls on the magnetization reversal of the FeNi layer in FeNi/Al_2\_2O_3\_3/Co magnetic tunnel junctions

We have studied the magnetization reversal dynamics of FeNi/Al$\_2$O$\_3$/Co magnetic tunnel junctions deposited on step-bunched Si substrates using magneto-optical Kerr effect and time-resolved x-ray photoelectron emission microscopy combined with x-ray magnetic circular dichroism (XMCD-PEEM). Different reversal mechanisms have been found depending on the substrate miscut angle. Larger terraces (smaller miscut angles) lead to a higher nucleation density and stronger domain wall pinning. The width of domain walls with respect to the size of the terraces seems to play an important role in the reversal. We used the element selectivity of XMCD-PEEM to reveal the strong influence of the stray field of domain walls in the hard magnetic layer on the magnetic switching of the soft magnetic layer.Comment: 8 Pages, 7 Figure

Dynamics of magnetic domain wall motion after nucleation: Dependence on the wall energy

The dynamics of magnetic domain wall motion in the FeNi layer of a FeNi/Al2O3/Co trilayer has been investigated by a combination of x-ray magnetic circular dichroism, photoelectron emission microscopy, and a stroboscopic pump-probe technique. The nucleation of domains and subsequent expansion by domain wall motion in the FeNi layer during nanosecond-long magnetic field pulses was observed in the viscous regime up to the Walker limit field. We attribute an observed delay of domain expansion to the influence of the domain wall energy that acts against the domain expansion and that plays an important role when domains are small.Comment: Accepted for publication in Physical Review Letter

Ferromagnetic coupling of mononuclear Fe centers in a self-assembled metal-organic network on Au(111)

The magnetic state and magnetic coupling of individual atoms in nanoscale structures relies on a delicate balance between different interactions with the atomic-scale surrounding. Using scanning tunneling microscopy, we resolve the self-assembled formation of highly ordered bilayer structures of Fe atoms and organic linker molecules (T4PT) when deposited on a Au(111) surface. The Fe atoms are encaged in a three-dimensional coordination motif by three T4PT molecules in the surface plane and an additional T4PT unit on top. Within this crystal field, the Fe atoms retain a magnetic ground state with easy-axis anisotropy, as evidenced by X-ray absorption spectroscopy and X-ray magnetic circular dichroism. The magnetization curves reveal the existence of ferromagnetic coupling between the Fe centers

Interplay between magnetic anisotropy and interlayer coupling in nanosecond magnetization reversal of spin-valve trilayers

The influence of magnetic anisotropy on nanosecond magnetization reversal in coupled FeNi/Cu/Co trilayers was studied using a photoelectron emission microscope combined with x-ray magnetic circular dicroism. In quasi-isotropic samples the reversal of the soft FeNi layer is determined by domain wall pinning that leads to the formation of small and irregular domains. In samples with uniaxial magnetic anisotropy, the domains are larger and the influence of local interlayer coupling dominates the domain structure and the reversal of the FeNi layer

Magnetic coupling of porphyrin molecules through graphene

Graphene is expected to complement todays Si-based information technology. In particular, magnetic molecules in contact with graphene constitute a tantalizing approach towards organic spin electronics because of the reduced conductivity mismatch at the interface. In such a system a bit is represented by a single molecular magnetic moment, which must be stabilized against thermal fluctuations. Here, we show in a combined experimental and theoretical study that the moments of paramagnetic Co-octaethylporphyrin (CoOEP) molecules on graphene can be aligned by a remarkable antiferromagnetic coupling to a Ni substrate underneath the graphene. This coupling is mediated via the \pi\ electronic system of graphene, while no covalent bonds between the molecule and the substrate are established.Comment: 27 pages, 12 figures, Accepted at Adv. Mate

Spin Motion in Electron Transmission through Ultrathin Ferromagnetic Films Accessed by Photoelectron Spectroscopy

Ab initio and model calculations demonstrate that the spin motion of electrons transmitted through ferromagnetic films can be analyzed in detail by means of angle- and spin-resolved core-level photoelectron spectroscopy. The spin motion appears as precession of the photoelectron spin polarization around and as relaxation towards the magnetization direction. In a systematic study for ultrathin Fe films on Pd(001) we elucidate its dependence on the Fe film thickness and on the Fe electronic structure. In addition to elastic and inelastic scattering, the effect of band gaps on the spin motion is addressed in particular.Comment: 4 pages, 5 figure