1212型銅酸化物のエピタキシャル成長とその超伝導特性

京都大学0048新制・課程博士博士(工学)甲第19720号工博第4175号新制||工||1644(附属図書館)32756京都大学大学院工学研究科電子工学専攻(主査)教授 川上 養一, 教授 田中 勝久, 准教授 掛谷 一弘学位規則第4条第1項該当Doctor of Philosophy (Engineering)Kyoto UniversityDFA

Spin-orbit coupling suppression and singlet-state blocking of spin-triplet Cooper pairs

An inhomogeneous magnetic exchange field at a superconductor/ferromagnet interface converts spin-singlet Cooper pairs to a spin-aligned (i.e. spin-polarized) triplet state. Although the decay envelope of such triplet pairs within ferromagnetic materials is well studied, little is known about their decay in non-magnetic metals and superconductors, and in particular in the presence of spin-orbit coupling (SOC). Here we investigate devices in which triplet supercurrents are injected into the s-wave superconductor Nb. In the normal state of Nb, triplet supercurrents decay over a distance of 5 nm, which is an order of magnitude smaller than the decay of spin singlet pairs due to the SOC interacting with the spin associated with triplet pairs. In the superconducting state of Nb, triplet supercurrents are not able to couple with the singlet wavefunction and thus blocked by the absence of available equilibrium states in the singlet gap. The results offer new insight into the dynamics between s-wave singlet and s-wave triplet states.S.K., J.M.D-S., G.Y., X.M., L.F.C., H.K., M.G.B., and J.W.A.R. acknowledge funding from the EPSRC Programme Grant “Superspin” (no. EP/N017242/1) and EPSRC International Network Grant “Oxide Superspin” (no. EP/P026311/1). K.O. acknowledges the JSPS Programme “Fostering Globally Talented Researchers” (JPMXS05R2900005). S.M. and A.I.B. acknowledge funding from Russian Science Foundation (grant no. 20-12-00053, in part related to the theoretical calculations). Zh.D. and S.M. acknowledge financial support from the Foundation for the advancement of theoretical physics “BASIS.” S.M. acknowledges financial support from the Russian Presidential Scholarship (SP-3938.2018.5

Large-scale on-chip integration of gate-voltage addressable hybrid superconductor-semiconductor quantum wells field effect nano-switch arrays

Stable, reproducible, scalable, addressable, and controllable hybrid superconductor-semiconductor (S-Sm) junctions and switches are key circuit elements and building blocks of gate-based quantum processors. The electrostatic field effect produced by the split gate voltages facilitates the realisation of nano-switches that can control the conductance or current in the hybrid S-Sm circuits based on 2D semiconducting electron systems. Here, we experimentally demonstrate a novel realisation of large-scale scalable, and gate voltage controllable hybrid field effect quantum chips. Each chip contains arrays of split gate field effect hybrid junctions, that work as conductance switches, and are made from In0.75Ga0.25As quantum wells integrated with Nb superconducting electronic circuits. Each hybrid junction in the chip can be controlled and addressed through its corresponding source-drain and two global split gate contact pads that allow switching between their (super)conducting and insulating states. We fabricate a total of 18 quantum chips with 144 field effect hybrid Nb- In0.75Ga0.25As 2DEG-Nb quantum wires and investigate the electrical response, switching voltage (on/off) statistics, quantum yield, and reproducibility of several devices at cryogenic temperatures. The proposed integrated quantum device architecture allows control of individual junctions in a large array on a chip useful for the development of emerging cryogenic nanoelectronics circuits and systems for their potential applications in fault-tolerant quantum technologies

Effect of Meissner Screening and Trapped Magnetic Flux on Magnetization Dynamics in Thick Nb/Ni₈₀Fe₂₀/Nb Trilayers

We investigate the influence of Meissner screening and trapped magnetic flux on magnetization dynamics for a Ni80Fe20 film sandwiched between two thick Nb layers (100 nm) using broadband (5–20 GHz) ferromagnetic resonance (FMR) spectroscopy. Below the superconducting transition Tc of Nb, significant zero-frequency line broadening (5–6 mT) and dc-resonance field shift (50 mT) to a low field are both observed if the Nb thickness is comparable to the London penetration depth of Nb films (≥100 nm). We attribute the observed peculiar behaviors to the increased incoherent precession near the Ni80Fe20/Nb interfaces and the effectively focused magnetic flux in the middle Ni80Fe20 caused by strong Meissner screening and (defect-)trapped flux of the thick adjacent Nb layers. This explanation is supported by static magnetic properties of the samples and comparison with FMR data on thick Nb/Ni80Fe20 bilayers. Great care should, therefore, be taken in the analysis of FMR response in ferromagnetic Josephson structures with thick superconductors, a fundamental property for high-frequency device applications of spin-polarized supercurrents

Unveiling unconventional magnetism at the surface of Sr2_2RuO4_4

Materials with strongly correlated electrons exhibit physical properties that are often difficult to predict as they result from the interactions of large numbers of electrons combined with several quantum degrees of freedom. The layered oxide perovskite Sr$_2$RuO$_4$ is a strongly correlated electron material that has been intensively investigated since its discovery due to its unusual physical properties. Whilst recent experiments have reopened the debate on the exact symmetry of the superconducting state in Sr$_2$RuO$_4$, a deeper understanding of the Sr$_2$RuO$_4$ normal state appears crucial as this is the background in which electron pairing occurs. Here, by using low-energy muon spin spectroscopy we discover the existence of magnetism at the surface of Sr$_2$RuO$_4$ in its normal state. We detect static weak dipolar fields yet manifesting below a relatively high onset temperature larger than 50 K, which reveals the unconventional nature of the observed magnetism. We relate the origin of this phase breaking time reversal symmetry to electronic ordering in the form of orbital loop currents that originate at the reconstructed Sr$_2$RuO$_4$ surface. Our observations set a reference for the discovery of the same magnetic phase in other materials and unveil an electronic ordering mechanism that can influence unconventional electron pairing with broken time reversal symmetry in those materials where the observed magnetic phase coexists with superconductivity.Comment: 20 pages, 5 figure

Quantized conductance in split gate superconducting quantum point contacts with InGaAs semiconducting two-dimensional electron systems

Quantum point contact or QPC -- a constriction in a semiconducting two-dimensional (2D) electron system with a quantized conductance -- has been found as the building block of novel spintronic, and topological electronic circuits. They can also be used as readout electronic, charge sensor or switch in quantum nanocircuits. A short and impurity-free constriction with superconducting contacts is a Cooper pairs QPC analogue known as superconducting quantum point contact (SQPC). The technological development of such quantum devices has been prolonged due to the challenges of maintaining their geometrical requirement and near-unity superconductor-semiconductor interface transparency. Here, we develop advanced nanofabrication, material and device engineering techniques and report on an innovative realisation of nanoscale SQPC arrays with split gate technology in semiconducting 2D electron systems, exploiting the special gate tunability of the quantum wells, and report the first experimental observation of conductance quantization in hybrid InGaAs-Nb SQPCs. We observe reproducible quantized conductance at zero magnetic fields in multiple quantum nanodevices fabricated in a single chip and systematically investigate the quantum transport of SQPCs at low and high magnetic fields for their potential applications in quantum metrology, for extremely accurate voltage standards, and fault-tolerant quantum technologies.N

Pair suppression caused by mosaic-twist defects in superconducting Sr 2 RuO 4 thin-films prepared using pulsed laser deposition

Funder: IBS Institute for Basic Science in Korea Grant No. IBS-R009-D1Abstract: Sr2RuO4 (SRO214) is a prototypical unconventional superconductor. However, since the discovery of its superconductivity a quarter of a century ago, the symmetry of the bulk and surface superconducting states in single crystal SRO214 remains controversial. Solving this problem is massively impeded by the fact that superconducting SRO214 is extremely challenging to achieve in thin-films as structural defects and impurities sensitively annihilate superconductivity. Here we report a protocol for the reliable growth of superconducting SRO214 thin-films by pulsed laser deposition and identify universal materials properties that are destructive to the superconducting state. We demonstrate that careful control of the starting material is essential in order to achieve superconductivity and use a single crystal target of Sr3Ru2O7 (SRO327). By systematically varying the SRO214 film thickness, we identify mosaic twist as the key in-plane defect that suppresses superconductivity. The results are central to the development of unconventional superconductivity

Fraunhofer patterns in magnetic Josephson junctions with non-uniform magnetic susceptibility

The development of superconducting memory and logic based on magnetic Josephson junctions relies on an understanding of junction properties and, in particular, the dependence of critical current on external magnetic flux (i.e. Fraunhofer patterns). With the rapid development of Josephson junctions with various forms of inhomogeneous barrier magnetism, Fraunhofer patterns are increasingly complex. In this paper we model Fraunhofer patterns for magnetic Josephson junctions in which the barrier magnetic susceptibility is position- and external magnetic field dependent. The model predicts anomalous Fraunhofer patterns in which local minima in the Josephson critical current can be nonzero and non-periodic with external magnetic flux due to an interference effect between highly magnetised and demagnetised regions