Magnetic structure, phase diagram, and a new type of spin-flop transition dominated by higher order interaction in a localized 5f system U3Pd20Si6

The magnetic structure of the localized-5f uranium intermetallic compound U3Pd20Si6 has been determined by means of a neutron diffraction experiment. Our data demonstrate that this compound has a collinear coupling of the sublattice ordering of the uranium spins on the 4a and 8c sites. We conclude that higher-order exchange and/or quadrupole interactions are necessary to stabilize this unique collinear structure. We discovered a new type of spin-flop transition against the uniaxial anisotropy induced by this collinear coupling

Excitations in Spin Chains and Specific-Heat Anomalies in Yb(4)As(3)

An explanation is given for the observed magnetic-field dependence of the low-temperature specific heat coefficient of Yb(4)As(3). It is based on a recently developed model for that material which can explain the observed heavy-fermion behaviour. According to it the Yb(3+)-ions are positioned in a net of parallel chains with an effective spin coupling of the order of J = 25 K. The magnetic-field dependence can be understood by including a weak magnetic coupling J' between adjacent chains. The data require a ratio J'/J of about 10^{-4}. In that case the experimental results can be reproduced very well by the theory.Comment: 5 pages, 5 PostScript-figures, needs LaTeX2e and the graphics-packag

Thermal Properties of Heavy Fermion Compound YbP

Low-temperature specific heat and its field-dependence up to 16 T was measured in a stoichiometric single crystal of YbP. A sharp peak was observed at {\it T}$_{\rm N}$ = 0.53 K in zero magnetic field. Application of external field seems to induce a new magnetic phase above 11 T. The field dependence of the transition temperature in the high-field phase is different from that of the low field phase. The linear coefficient of the electronic specific heat is estimated as 120 mJ/mole K$^{2}$ from low temperature specfic heat, suggesting heavy Fermion state in YbP.Comment: to be published in J.Phys.Soc.Jpn on May, 200

Suppression of ferromagnetism in CeSi_1.81 under temperature and pressure

We have studied the pressure dependence of the magnetization of single crystalline CeSi_1.81. At ambient pressure ferromagnetism develops below T_C = 9.5 Below ~ 5 K an additional shoulder in low-field hysteresis loops and a metamagnetic crossover around 4 T suggest the appearance of an additional magnetic modulation to the ferromagnetic state. The suppression of the magnetic order in CeSi_1.81 as function of temperature at ambient pressure and as function of pressure at low temperature are in remarkable qualitative agreement. The continuous suppression of the ordered moment at p ~ 13.1 kbar suggests the existence of a ferromagnetic quantum critical point in this material.Comment: 9 pages, 9 figures, to be published in Physical Review

Anomalous Anisotropic Magnetoresistance in Heavy-Fermion PrFe4P12

We have investigated the anisotropy of the magnetoresistance in the Pr-based HF compound PrFe4P12. The large anisotropy of effective mass and its strong field dependence have been confirmed by resistivity measurements. Particularly for H||[111], where the effective mass is most strongly enhanced, the non-Fermi liquid behavior has been observed. Also, we have found the angular dependence of the magnetoresistance sharply enhanced at H||[111], which is evidently correlated with both the non-Fermi liquid behavior and the high-field ordered state (B-phase).Comment: 3 pages, 3 figures. J. Phys. Soc. Jpn. Vol.77, No.8, in pres

Crystalline electric field effects in the electrical resistivity of PrOs4_4Sb12_{12}

The temperature $T$ and magnetic field $H$ dependencies of the electrical resistivity $\rho$ of the recently discovered heavy fermion superconductor \PrOsSb{} have features that are associated with the splitting of the Pr$^{3+}$ Hund's rule multiplet by the crystalline electric field (CEF). These features are apparently due to magnetic exchange and aspherical Coulomb scattering from the thermally populated CEF-split Pr$^{3+}$ energy levels. The $\rho(T)$ data in zero magnetic field can be described well by calculations based on CEF theory for various ratios of magnetic exchange and aspherical Coulomb scattering, and yield CEF parameters that are qualitatively consistent with those previously derived from magnetic susceptibility, specific heat, and inelastic neutron scattering measurements. Calculated $\rho(H)$ isotherms for a $\Gamma_{3}$ ground state qualitatively account for the `dome-shaped' feature in the measured $\rho(H)$ isotherms.Comment: 8 pages, 2 figures, submitted to Journal of Physics: Condensed Matte

Change of Electronic Structure Induced by Magnetic Transitions in CeBi

The temperature dependence of the electronic structure of CeBi arising from two types of antiferromagnetic transitions based on optical conductivity ($\sigma(\omega)$) was observed. The $\sigma(\omega)$ spectrum continuously and discontinuously changes at 25 and 11 K, respectively. Between these temperatures, two peaks in the spectrum rapidly shift to the opposite energy sides as the temperature changes. Through a comparison with the band calculation as well as with the theoretical $\sigma(\omega)$ spectrum, this peak shift was explained by the energy shift of the Bi $6p$ band due to the mixing effect between the Ce $4f \Gamma_8$ and Bi $6p$ states. The single-layer antiferromagnetic ($+-$) transition from the paramagnetic state was concluded to be of the second order. The marked changes in the $\sigma(\omega)$ spectrum at 11 K, however, indicated the change in the electronic structure was due to a first-order-like magnetic transition from a single-layer to a double-layer ($++--$) antiferromagnetic phase.Comment: 4 pages, to be published in J. Phys. Soc. Jpn. 73 Aug. (2004

Magnetoelastic effects in low-dimensional magnetic systems

We consider a new realization of magnetoelastic interactions in low-dimensional magnetic systems. We show that low-dimensional spin systems are unstable with respect to the spontaneous appearance of alternating distortions of the positions of the three-dimensional nonmagnetic atoms (ligands), that surround the magnetic ions. Those distortions are supplemented by the spontaneous onset of alternating effective g factors of the magnetic ions in the phase with short-range interactions. We discuss the possibility of observing the effect in an uniform external magnetic field, which in the situation considered produces both magnetization and staggered magnetization of the magnetic subsystem. The connection of the proposed theory with recent experiments on effectively low-dimensional magnetic systems (organic spin chains, heavy-fermion compounds, rare-earth molybdates) is discussed

Detection of Neutron Scattering from Phase IV of Ce0.7La0.3B6: A Confirmation of the Octupole Order

We have performed a single crystal neutron scattering experiment on Ce0.7La0.3B6 to investigate the order parameter of phase IV microscopically. Below the phase transition temperature 1.5 K of phase IV, weak but distinct superlattice reflections at the scattering vector (h/2,h/2,l/2) (h, l = odd number) have been observed by neutron scattering for the first time. The intensity of the superlattice reflections is stronger for high scattering vectors, which is quite different from the usual magnetic form factor of magnetic dipoles. This result directly evidences that the order parameter of phase IV has a complex magnetization density, consistent with the recent experimental and theoretical prediction in which the order parameter is the magnetic octupoles Tbeta with Gamma5 symmetry of point group Oh. Neutron scattering experiments using short wavelength neutrons, as done in this study, could become a general method to study the high-rank multipoles in f electron systems.Comment: 4 pages, 4 figure