961 research outputs found
Plasmons on the edge of MoS2 nanostructures
Using ab initio calculations we predict the existence of one-dimensional
(1D), atomically confined plasmons at the edges of a zigzag MoS2 nanoribbon.
The strongest plasmon originates from a metallic edge state localized on the
sulfur dimers decorating the Mo edge of the ribbon. A detailed analysis of the
dielectric function reveals that the observed deviations from the ideal 1D
plasmon behavior result from single-particle transitions between the metallic
edge state and the valence and conduction bands of the MoS2 sheet. The Mo and S
edges of the ribbon are clearly distinguishable in calculated spatially
resolved electron energy loss spectrum owing to the different plasmonic
properties of the two edges. The edge plasmons could potentially be utilized
for tuning the photocatalytic activity of MoS2 nanoparticles
Spatially resolved quantum plasmon modes in metallic nano-films from first principles
Electron energy loss spectroscopy (EELS) can be used to probe plasmon
excitations in nanostructured materials with atomic-scale spatial resolution.
For structures smaller than a few nanometers quantum effects are expected to be
important, limiting the validity of widely used semi-classical response models.
Here we present a method to identify and compute spatially resolved plasmon
modes from first principles based on a spectral analysis of the dynamical
dielectric function. As an example we calculate the plasmon modes of 0.5-4 nm
thick Na films and find that they can be classified as (conventional) surface
modes, sub-surface modes, and a discrete set of bulk modes resembling standing
waves across the film. We find clear effects of both quantum confinement and
non-local response. The quantum plasmon modes provide an intuitive picture of
collective excitations of confined electron systems and offer a clear
interpretation of spatially resolved EELS spectra.Comment: 7 pages, 7 figure
An Investigation of Energy Storage Possibilities in Single Family Houses for Smart Grid Purposes
Aerobic anti-gravity exercise in patients with Charcot-Marie-Tooth disease types 1A and X:A pilot study
Phenylketonuria - the effects on quality of life and plasma concentrations of phenylalanine and tyrosine of two different amino-acid-suplementations in different concentrations
Herregårdshaven på Sønderskov: Havens historie og udvikling set i havekunstnerisk perspektiv
Cand.hort.arch. Kirsten Lund-Andersen gennemgår i denne artikel haven på Sønderskovs historie fra 1400-tallet til i dag i relation til udviklingen i havekunst og -historie
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