894 research outputs found
Giant nonlinear conduction and thyristor-like negative derivative resistance in BaIrO3 single crystals
We synthesized single-crystalline samples of monoclinic BaIrO3 using a molten
flux method, and measured their magnetization, resistivity, Seebeck coefficient
and nonlinear voltage-current characteristics. The magnetization rapidly
increases below a ferromagnetic transition temperature TC of 180 K, where the
resistivity concomitantly shows a hump-type anomaly, followed by a sharp
increase below 30 K. The Seebeck coefficient suddenly increases below TC, and
shows linear temperature dependence below 50 K. A most striking feature of this
compound is that the anomalously giant nonlinear conduction is observed below
30 K, where a small current density of 20 A/cm2 dramatically suppresses the
sharp increase in resistivity to induce a metallic conduction down to 4 K.Comment: 10 pages, 4 figures Submitted to Physical Review Letter
Notice Requirements: Common Themes and Differences in the Regulatory and Legislative Responses to Data Security Breaches
Angle Dependent Magnetoresistance of the Layered Organic Superconductor \kappa-(ET)2Cu(NCS)2: Simulation and Experiment
The angle-dependences of the magnetoresistance of two different isotopic
substitutions (deuterated and undeuterated) of the layered organic
superconductor \kappa-(ET)2Cu(NCS)2 are presented. The angle dependent
magnetoresistance oscillations (AMRO) arising from the quasi-one-dimensional
(Q1D) and quasi-two-dimensional (Q2D) Fermi surfaces in this material are often
confused. By using the Boltzman transport equation extensive simulations of the
AMRO are made that reveal the subtle differences between the different species
of oscillation. No significant differences are observed in the electronic
parameters derived from quantum oscillations and AMRO for the two isotopic
substitutions. The interlayer transfer integrals are determined for both
isotopic substitutions and a slight difference is observed which may account
for the negative isotope effect previously reported [1]. The success of the
semi-classical simulations suggests that non-Fermi liquid effects are not
required to explain the interlayer-transport in this system.Comment: 15 pages, 16 figure
Substitution Effect by Deuterated Donors on Superconductivity in -(BEDT-TTF)Cu[N(CN)]Br
We investigate the superconductivity in the deuterated BEDT-TTF molecular
substitution system
-[(h8-BEDT-TTF)(d8-BEDT-TTF)]Cu[N(CN)]Br, where h8
and d8 denote fully hydrogenated and deuterated molecules, respectively.
Systematic and wide range ( = 0 -- 1) substitution can control chemical
pressure finely near the Mott boundary, which results in the modification of
the superconductivity. After cooling slowly, the increase of
observed up to 0.1 is evidently caused by the chemical pressure
effect. Neither reduction of nor suppression of
superconducting volume fraction is found below 0.5. This demonstrates
that the effect of disorder by substitution is negligible in the present
system. With further increase of , both and superconducting
volume fraction start to decrease toward the values in = 1.Comment: J. Phys. Soc. Jp
Efficient Online Timed Pattern Matching by Automata-Based Skipping
The timed pattern matching problem is an actively studied topic because of
its relevance in monitoring of real-time systems. There one is given a log
and a specification (given by a timed word and a timed automaton
in this paper), and one wishes to return the set of intervals for which the log
, when restricted to the interval, satisfies the specification
. In our previous work we presented an efficient timed pattern
matching algorithm: it adopts a skipping mechanism inspired by the classic
Boyer--Moore (BM) string matching algorithm. In this work we tackle the problem
of online timed pattern matching, towards embedded applications where it is
vital to process a vast amount of incoming data in a timely manner.
Specifically, we start with the Franek-Jennings-Smyth (FJS) string matching
algorithm---a recent variant of the BM algorithm---and extend it to timed
pattern matching. Our experiments indicate the efficiency of our FJS-type
algorithm in online and offline timed pattern matching
Isotope effect in superconductors with coexisting interactions of phonon and nonphonon mechanisms
We examine the isotope effect of superconductivity in systems with coexisting
interactions of phonon and nonphonon mechanisms in addition to the direct
Coulomb interaction. The interaction mediated by the spin fluctuations is
discussed as an example of the nonphonon interaction. Extended formulas for the
transition temperature Tc and the isotope-effect coefficient alpha are derived
for cases (a) omega_np omega_D, where omega_np is
an effective cutoff frequency of the nonphonon interaction that corresponds to
the Debye frequency omega_D in the phonon interaction. In case (a), it is found
that the nonphonon interaction does not change the condition for the inverse
isotope effect, i.e., mu^* > lambda_ph/2, but it modifies the magnitude of
alpha markedly. In particular, it is found that a giant isotope shift occurs
when the phonon and nonphonon interactions cancel each other largely. For
instance, strong critical spin fluctuations may give rise to the giant isotope
effect. In case (b), it is found that the inverse isotope effect occurs only
when the nonphonon interaction and the repulsive Coulomb interaction, in total
effect, work as repulsive interactions against the superconductivity. We
discuss the relevance of the present result to some organic superconductors,
such as kappa-(ET)2Cu(NCS)2 and Sr2RuO4 superconductors, in which inverse
isotope effects have been observed, and briefly to high-Tc cuprates, in which
giant isotope effects have been observed.Comment: 4 pages, 2 figures, (with jpsj2.cls, ver.1.2), v2:linguistic
correction
Evidence for structural and electronic instabilities at intermediate temperatures in -(BEDT-TTF)X for X=Cu[N(CN)]Cl, Cu[N(CN)]Br and Cu(NCS): Implications for the phase diagram of these quasi-2D organic superconductors
We present high-resolution measurements of the coefficient of thermal
expansion of the quasi-twodimensional
(quasi-2D) salts -(BEDT-TTF)X with X = Cu(NCS), Cu[N(CN)]Br
and Cu[N(CN)]Cl. At intermediate temperatures (B), distinct anomalies
reminiscent of second-order phase transitions have been found at
K and 45 K for the superconducting X = Cu(NCS) and Cu[N(CN)]Br salts,
respectively. Most interestingly, we find that the signs of the uniaxial
pressure coefficients of are strictly anticorrelated with those of
. We propose that marks the transition to a spin-density-wave
(SDW) state forming on minor, quasi-1D parts of the Fermi surface. Our results
are compatible with two competing order parameters that form on disjunct
portions of the Fermi surface. At elevated temperatures (C), all compounds show
anomalies that can be identified with a kinetic, glass-like
transition where, below a characteristic temperature , disorder in the
orientational degrees of freedom of the terminal ethylene groups becomes frozen
in. We argue that the degree of disorder increases on going from the X =
Cu(NCS) to Cu[N(CN)]Br and the Cu[N(CN)]Cl salt. Our results
provide a natural explanation for the unusual time- and cooling-rate
dependencies of the ground-state properties in the hydrogenated and deuterated
Cu[N(CN)]Br salts reported in the literature.Comment: 22 pages, 7 figure
Pulse profile modelling of thermonuclear burst oscillations - II: Handling variability
Pulse profile modelling is a relativistic ray-tracing technique that can be used to infer masses, radii, and geometric parameters of neutron stars. In a previous study, we looked at the performance of this technique when applied to thermonuclear burst oscillations from accreting neutron stars. That study showed that ignoring the variability associated with burst oscillation sources resulted in significant biases in the inferred mass and radius, particularly for the high count rates that are nominally required to obtain meaningful constraints. In this follow-on study, we show that the bias can be mitigated by slicing the bursts into shorter segments where variability can be neglected, and jointly fitting the segments. Using this approach, the systematic uncertainties on the mass and radius are brought within the range of the statistical uncertainty. With about 106 source counts, this yields uncertainties of approximately 10 per cent for both the mass and radius. However, this modelling strategy requires substantial computational resources. We also confirm that the posterior distributions of the mass and radius obtained from multiple bursts of the same source can be merged to produce outcomes comparable to that of a single burst with an equivalent total number of counts
Preparation of Microcrystals of Piroxicam Monohydrate by Antisolvent Precipitation via Microfabricated Metallic Membranes with Ordered Pore Arrays
Microcrystals of piroxicam (PRX) monohydrate with a narrow size distribution were prepared from acetone/PRX solutions by antisolvent crystallization via metallic membranes with ordered pore arrays. Crystallization was achieved by controlled addition of the feed solution through the membrane pores into a well-stirred antisolvent. A complete transformation of an anhydrous form I into a monohydrate form of PRX was confirmed by Raman spectroscopy and differential scanning calorimetry. The size of the crystals was 7–34 μm and was controlled by the PRX concentration in the feed solution (15–25 g L¯¹), antisolvent/solvent volume ratio (5–30), and type of antisolvent (Milli-Q water or 0.1–0.5 wt % aqueous solutions of hydroxypropyl methyl cellulose (HPMC), poly(vinyl alcohol) or Pluronic P-123). The smallest crystals were obtained by injecting 25 g L¯¹ PRX solution through a stainless-steel membrane with a pore size of 10 μm into a 0.06 wt % HPMC solution stirred at 1500 rpm using an antisolvent/solvent ratio of 20. HPMC provided better steric stabilization of microcrystals against agglomeration than poly(vinyl alcohol) and Pluronic P-123, due to hydrogen bonding interactions with PRX and water. A continuous production of large PRX monohydrate microcrystals with a volume-weighted mean diameter above 75 μm was achieved in a continuous stirred membrane crystallizer. Rapid pouring of Milli-Q water into the feed solution resulted in a mixture of highly polydispersed prism-shaped and needle-shaped crystals
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