A hybrid model for Rydberg gases including exact two-body correlations

A model for the simulation of ensembles of laser-driven Rydberg-Rydberg interacting multi-level atoms is discussed. Our hybrid approach combines an exact two-body treatment of nearby atom pairs with an effective approximate treatment for spatially separated pairs. We propose an optimized evolution equation based only on the system steady state, and a time-independent Monte Carlo technique is used to efficiently determine this steady state. The hybrid model predicts features in the pair correlation function arising from multi-atom processes which existing models can only partially reproduce. Our interpretation of these features shows that higher-order correlations are relevant already at low densities. Finally, we analyze the performance of our model in the high-density case.Comment: significantly expanded and revised version (more observables, high-density regime); 9 pages, 8 figure

Ab initio quantum models for thin-film x-ray cavity QED

We develop two ab initio quantum approaches to thin-film x-ray cavity quantum electrodynamics with spectrally narrow x-ray resonances, such as those provided by M\"ossbauer nuclei. The first method is based on a few-mode description of the cavity, and promotes and extends existing phenomenological few-mode models to an ab initio theory. The second approach uses analytically-known Green's functions to model the system. The two approaches not only enable one to ab initio derive the effective few-level scheme representing the cavity and the nuclei in the low-excitation regime, but also provide a direct avenue for studies at higher excitation, involving non-linear or quantum phenomena. The ab initio character of our approaches further enables direct optimizations of the cavity structure and thus of the photonic environment of the nuclei, to tailor the effective quantum optical level scheme towards particular applications. To illustrate the power of the ab initio approaches, we extend the established quantum optical modeling to resonant cavity layers of arbitrary thickness, which is essential to achieve quantitative agreement for cavities used in recent experiments. Further, we consider multi-layer cavities featuring electromagnetically induced transparency, derive their quantum optical few-level systems ab initio, and identify the origin of discrepancies in the modeling found previously using phenomenological approaches as arising from cavity field gradients across the resonant layers.Comment: 41 pages, 20 figures, added clarifications and minor correction

Coherent X-ray−optical control of nuclear excitons

Coherent control of quantum dynamics is key to a multitude of fundamental studies and applications. In the visible or longer-wavelength domains, near-resonant light fields have become the primary tool with which to control electron dynamics. Recently, coherent control in the extreme-ultraviolet range was demonstrated, with a few-attosecond temporal resolution of the phase control. At hard-X-ray energies (above 5–10 kiloelectronvolts), Mössbauer nuclei feature narrow nuclear resonances due to their recoilless absorption and emission of light, and spectroscopy of these resonances is widely used to study the magnetic, structural and dynamical properties of matter. It has been shown that the power and scope of Mössbauer spectroscopy can be greatly improved using various control techniques. However, coherent control of atomic nuclei using suitably shaped near-resonant X-ray fields remains an open challenge. Here we demonstrate such control, and use the tunable phase between two X-ray pulses to switch the nuclear exciton dynamics between coherent enhanced excitation and coherent enhanced emission. We present a method of shaping single pulses delivered by state-of-the-art X-ray facilities into tunable double pulses, and demonstrate a temporal stability of the phase control on the few-zeptosecond timescale. Our results unlock coherent optical control for nuclei, and pave the way for nuclear Ramsey spectroscopy and spin-echo-like techniques, which should not only advance nuclear quantum optics, but also help to realize X-ray clocks and frequency standards. In the long term, we envision time-resolved studies of nuclear out-of-equilibrium dynamics, which is a long-standing challenge in Mössbauer science

Spectral narrowing of x-ray pulses for precision spectroscopy with nuclear resonances

Spectroscopy of nuclear resonances offers a wide range of applications due to the remarkable energy resolution afforded by their narrow linewidths. However, progress toward higher resolution is inhibited at modern x-ray sources because they deliver only a tiny fraction of the photons on resonance, with the remainder contributing to an off-resonant background. We devised an experimental setup that uses the fast mechanical motion of a resonant target to manipulate the spectrum of a given x-ray pulse and to redistribute off-resonant spectral intensity onto the resonance. As a consequence, the resonant pulse brilliance is increased while the off-resonant background is reduced. Because our method is compatible with existing and upcoming pulsed x-ray sources, we anticipate that this approach will find applications that require ultranarrow x-ray resonances

Analysis of Outcomes in Ischemic vs Nonischemic Cardiomyopathy in Patients With Atrial Fibrillation A Report From the GARFIELD-AF Registry

IMPORTANCE Congestive heart failure (CHF) is commonly associated with nonvalvular atrial fibrillation (AF), and their combination may affect treatment strategies and outcomes