14,933 research outputs found

    Density of bulk trap states in organic semiconductor crystals: discrete levels induced by oxygen in rubrene

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    The density of trap states in the bandgap of semiconducting organic single crystals has been measured quantitatively and with high energy resolution by means of the experimental method of temperature-dependent space-charge-limited-current spectroscopy (TD-SCLC). This spectroscopy has been applied to study bulk rubrene single crystals, which are shown by this technique to be of high chemical and structural quality. A density of deep trap states as low as ~ 10^{15} cm^{-3} is measured in the purest crystals, and the exponentially varying shallow trap density near the band edge could be identified (1 decade in the density of states per ~25 meV). Furthermore, we have induced and spectroscopically identified an oxygen related sharp hole bulk trap state at 0.27 eV above the valence band.Comment: published in Phys. Rev. B, high quality figures: http://www.cpfs.mpg.de/~krellner

    Milli-second Oscillations in the Persistent and Bursting Flux of Aql X-1 During an Outburst

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    The Rossi X-Ray Timing Explorer observed the soft X-Ray transient Aql X-1 during its outburst in February and March 1997. We report the discovery of quasi-periodic oscillations (QPOs) in its persistent flux with frequencies in the range of 740 to 830 Hz, Q-value of over 100, and a fractional RMS amplitude of (6.8 +- 0.6)%, and nearly coherent oscillations (NCOs) during a Type-I burst with a frequency of 549 Hz. The frequency of the QPOs in the persistent flux is correlated with the mass accretion rate on time scale of hours, but not on time scale of days. This is most likely the manifestation in a single source of the kHz QPO puzzle observed among many sources, i.e., on the one hand, individual sources show a correlation between the QPO frequency and the inferred mass accretion rate, on the other hand, the dozen or so sources with luminosities spanning two decades have essentially the same QPO frequencies. We propose that this multi-valued QPO frequency and mass accretion rate correlation indicates the existence of many similar regimes of the accretion disk. These regimes, with a very similar energy spectrum and QPO frequency, are distinguished from each other by the mass accretion rate or the total X-ray flux. The NCOs during the burst can be made almost perfectly coherent by taking into account a large frequency derivative. This strongly suggests that this frequency is related to the neutron star spin frequency. The large frequency derivative is attributable to the expansion or contraction of the neutron star photosphere during the burst.Comment: 6 pages, LaTex (aas2pp4), Accepted for publication in ApJ Let

    New Constraints on Neutralino Dark Matter in the Supersymmetric Standard Model

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    We investigate the prospects for neutralino dark matter within the Supersymmetric Standard Model (SSM) including the constraints from universal soft supersymmetry breaking and radiative breaking of the electroweak symmetry. The latter is enforced by using the one-loop Higgs effective potential which automatically gives the one-loop corrected Higgs boson masses. We perform an exhaustive search of the allowed five-dimensional parameter space and find that the neutralino relic abundance Ωχh02\Omega_\chi h^2_0 depends most strongly on the ratio ξ0m0/m1/2\xi_0\equiv m_0/m_{1/2}. For ξ01\xi_0\gg1 the relic abundance is almost always much too large, whereas for ξ01\xi_0\ll1 the opposite occurs. For ξ01\xi_0\sim1 there are wide ranges of the remaining parameters for which Ωχ1\Omega_\chi\sim1. We also determine that m_{\tilde q}\gsim250\GeV and m_{\tilde l}\gsim100\GeV are necessary in order to possibly achieve Ωχ1\Omega_\chi\sim1. These lower bounds are much weaker than the corresponding ones derived previously when radiative breaking was {\it not} enforced.Comment: 12 pages plus 6 figures (not included), CERN-TH.6584/92, CTP-TAMU-56/92, UAHEP921

    Accurate Neutralino Relic Density Computations in Supergravity Models

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    We investigate the question of the proper thermal averaging of neutralino annihilation amplitudes which possess poles and thresholds, as they impact on the calculated neutralino relic density and therefore on the cosmological viability of supersymmetric models. We focus on two typical resonances, namely the ZZ boson and the lightest Higgs boson (hh). In the context of supergravity models with radiative electroweak symmetry breaking, an exploration of the whole parameter space of the model is possible and the overall relevance of these sophisticated analyses can be ascertained. As an example we chose the minimal SU(5)SU(5) supergravity model since the presence of such poles is essential to obtain a cosmologically acceptable model. We find that the proper thermal averaging is important for individual points in parameter space and that the fraction of cosmologically acceptable points is increased somewhat by the accurate procedure. However, qualitatively the new set of points is very similar to that obtained previously using the usual series approximations to the thermal average. We conclude that all phenomenological analyses based on the previously determined cosmologically allowed set remain valid.Comment: 15 pages, 9 figures (available upon request as uuencoded file or separate ps files), tex (harvmac) CTP-TAMU-14/9

    Metabolic Changes Following a 1-Year Diet and Exercise Intervention in Patients With Type 2 Diabetes

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    Objective—To characterize the relationships among longterm improvements in peripheral insulin sensitivity (glucose disposal rate [GDR]), fasting glucose, and free fatty acids (FFAs) and concomitant changes in weight and adipose tissue mass and distribution induced by lifestyle intervention in obese individuals with type 2 diabetes. Research Design And Methods—We measured GDR, fasting glucose, and FFAs during a euglycemic clamp and adipose tissue mass and distribution, organ fat, and adipocyte size by dual-energy X-ray absorptiometry, CT scan, and adipose tissue biopsy in 26 men and 32 women in the Look-AHEAD trial before and after 1 year of diet and exercise aimed at weight loss. Results—Weight and fasting glucose decreased significantly (P _ 0.0001) and significantly more in men than in women (_12 vs. _8% and _16 vs. _7%, respectively; P _ 0.05), while FFAs during hyperinsulinemia decreased and GDR increased significantly (P _ 0.00001) and similarly in both sexes (_53 vs. _41% and 63 vs. 43%; P _ NS). Men achieved a more favorable fat distribution by losing more from upper compared with lower and from deeper compared with superficial adipose tissue depots (P _ 0.01). Decreases in weight and adipose tissue mass predicted improvements in GDR but not in fasting glucose or fasting FFAs; however, decreases in FFAs during hyperinsulinemia significantly determined GDR improvements. Hepatic fat was the only regional fat measure whose change contributed independently to changes in metabolic variables. Conclusions—Patients with type 2 diabetes undergoing a 1-year lifestyle intervention had significant improvements in GDR, fasting glucose, FFAs and adipose tissue distribution. However, changes in overall weight (adipose tissue mass) and hepatic fat were the most important determinants of metabolic improvements.Jeanine B. Albu, Leonie K. Heilbronn, David E. Kelley, Steven R. Smith, Koichiro Azuma, Evan S. Berk, F. Xavier Pi-Sunyer, Eric Ravussin, and the Look AHEAD Adipose Research Grou

    Urinary ATP and visualization of intracellular bacteria: a superior diagnostic marker for recurrent UTI in renal transplant recipients?

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    Renal transplant recipients (RTR) are highly susceptible to urinary tract infections (UTIs) with over 50% of patients having at least one UTI within the first year. Yet it is generally acknowledged that there is considerable insensitivity and inaccuracy in routine urinalysis when screening for UTIs. Thus a large number of transplant patients with genuine urine infections may go undiagnosed and develop chronic recalcitrant infections, which can be associated with graft loss and morbidity. Given a recent study demonstrating ATP is released by urothelial cells in response to bacteria exposure, possibly acting at metabotropic P2Y receptors mediating a proinflammatory response, we have investigated alternative, and possibly more appropriate, urinalysis techniques in a cohort of RTRs.Mid-stream urine (MSU) samples were collected from 53 outpatient RTRs. Conventional leukocyte esterase and nitrite dipstick tests, and microscopic pyuria counts (in 1 ?l), ATP concentration measurements, and identification of intracellular bacteria in shed urothelial cells, were performed on fresh unspun samples and compared to ‘gold-standard’ bacterial culture results.Of the 53 RTRs, 22% were deemed to have a UTI by ‘gold-standard’ conventional bacteria culture, whereas 87%, 8% and 4% showed evidence of UTIs according to leukocyte esterase dipstick, nitrite dipstick, and a combination of both dipsticks, respectively. Intracellular bacteria were visualized in shed urothelial cells of 44% of RTRs, however only 1 of the 23 RTRs (44%) was deemed to have a UTI by conventional bacteria culture. A significant association of the ‘gold-standard’ test with urinary ATP concentration combined with visualization of intracellular bacteria in shed urothelial cells was determined using the Fisher’s exact test.It is apparent that standard bedside tests for UTIs give variable results and that seemingly quiescent bacteria in urothelial cells are very common in RTRs and may represent a focus of subclinical infection. Furthermore, our results suggest urinary ATP concentration combined with detection of intracellular bacteria in shed urinary epithelial cells may be a sensitive means by which to detect ‘occult’ infection in RTRs

    Low self-control promotes the willingness to sacrifice in close relationships

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    Although previous theories and research have suggested that human behavior is automatically driven by selfish impulses (e.g., vengeance rather than forgiveness), the present research tested the hypothesis that in close relationships, people's impulsive inclination is to be prosocial and to sacrifice for their partner-to pursue the interests of the partner or of the relationship at some costs for the self. Results from four studies demonstrated that people with low self-control, relative to those with high self-control, reported greater willingness to sacrifice for their close others. Furthermore, Study 4 demonstrated that communal orientation was more strongly associated with sacrifice among participants with low self-control than participants with high self-control. This moderational pattern supports the hypothesis that communal orientation functions as a default approach to sacrifice in the context of close relationships. Taken together, these findings suggest that under certain crucial conditions in close relationships, gut-level impulses are more likely than deliberative considerations to promote prorelationship behavior. © The Author(s) 2013
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