2,521 research outputs found
Permalloy-based carbon nanotube spin-valve
In this Letter we demonstrate that Permalloy (Py), a widely used Ni/Fe alloy,
forms contacts to carbon nanotubes (CNTs) that meet the requirements for the
injection and detection of spin-polarized currents in carbon-based spintronic
devices. We establish the material quality and magnetization properties of Py
strips in the shape of suitable electrical contacts and find a sharp
magnetization switching tunable by geometry in the anisotropic
magnetoresistance (AMR) of a single strip at cryogenic temperatures. In
addition, we show that Py contacts couple strongly to CNTs, comparable to Pd
contacts, thereby forming CNT quantum dots at low temperatures. These results
form the basis for a Py-based CNT spin-valve exhibiting very sharp resistance
switchings in the tunneling magnetoresistance, which directly correspond to the
magnetization reversals in the individual contacts observed in AMR experiments.Comment: 3 page
Laserâinduced desorption of NO from NiO(100): Ab initio calculations of potential surfaces for intermediate excited states
In order to interpret the experimental results of the state resolved UVâlaserâinduced desorption of NO from NiO(100) (rotational and vibrational populations, velocity distributions of the desorbing NO molecules, etc.), we have performed ab initio complete active space selfâconsistent field (CASSCF) and configuration interaction (CI) calculations for the interaction potential between NO and the NiO(100) surface in the electronic ground state and for those excited states which are involved in the desorption process. The NiO(100)âNO distance and the tilt angle between the NO axis and the surface normal have been varied. A cluster model containing a NiO8â5âcluster embedded in a Madelung potential has been used for representing the NiO(100) surface. The excited states which are important for the desorption process, are charge transfer states of the substrateâadsorbate system, in which one electron is transferred from the surface into the NOâ2Ïâorbital. The potential curves of these excited charge transfer states show deep minima (4 eVâ5 eV) at surface/NO distances which are smaller than that in the ground state. The angular dependence of these potentials behaves similar as in the ground state. A semiempirical correction to the calculated excitation energies has been added which makes use of the bulk polarization of NiO. With this correction the charge transfer states are considerably stabilized. The lowest excitation energy amounts to about 4 eV which is in reasonable agreement with the onset of the laser desorption observed experimentally at about 3.5 eV. The density of the NOââlike states is rather high, so that probably several excited states are involved in the desorption process. The potential energy curves for all of these states are quite similar, but the transitions from the ground state into different excited charge transfer states show strongly differing oscillator strengths, which are also strongly dependent on the surface/NO distance. This fact is important for the dynamics of the deexcitation process in the sense of a selection criterion for the states involved. The magnitude of the oscillator strengths is large in comparison with the excitation of NO in the gas phase, which might be an indication for the possibility of optical excitation processes. One dimensional wave packet calculations on two potential energy curves using fixed lifetimes for the excited state in each calculation have been performed and enable us to estimate the mean lifetime of the excited state to be 15 fsâ€Ïâ€25 fs. This implies that the dynamics of the system is dominated by the attractive part of the excited state potential
On Convergence of the Inexact Rayleigh Quotient Iteration with the Lanczos Method Used for Solving Linear Systems
For the Hermitian inexact Rayleigh quotient iteration (RQI), the author has
established new local general convergence results, independent of iterative
solvers for inner linear systems. The theory shows that the method locally
converges quadratically under a new condition, called the uniform positiveness
condition. In this paper we first consider the local convergence of the inexact
RQI with the unpreconditioned Lanczos method for the linear systems. Some
attractive properties are derived for the residuals, whose norms are
's, of the linear systems obtained by the Lanczos method. Based on
them and the new general convergence results, we make a refined analysis and
establish new local convergence results. It is proved that the inexact RQI with
Lanczos converges quadratically provided that with a
constant . The method is guaranteed to converge linearly provided
that is bounded by a small multiple of the reciprocal of the
residual norm of the current approximate eigenpair. The results are
fundamentally different from the existing convergence results that always
require , and they have a strong impact on effective
implementations of the method. We extend the new theory to the inexact RQI with
a tuned preconditioned Lanczos for the linear systems. Based on the new theory,
we can design practical criteria to control to achieve quadratic
convergence and implement the method more effectively than ever before.
Numerical experiments confirm our theory.Comment: 20 pages, 8 figures. arXiv admin note: text overlap with
arXiv:0906.223
Rates and Characteristics of Intermediate Mass Ratio Inspirals Detectable by Advanced LIGO
Gravitational waves (GWs) from the inspiral of a neutron star (NS) or
stellar-mass black hole (BH) into an intermediate-mass black hole (IMBH) with
mass between ~50 and ~350 solar masses may be detectable by the planned
advanced generation of ground-based GW interferometers. Such intermediate mass
ratio inspirals (IMRIs) are most likely to be found in globular clusters. We
analyze four possible IMRI formation mechanisms: (1) hardening of an NS-IMBH or
BH-IMBH binary via three-body interactions, (2) hardening via Kozai resonance
in a hierarchical triple system, (3) direct capture, and (4) inspiral of a
compact object from a tidally captured main-sequence star; we also discuss
tidal effects when the inspiraling object is an NS. For each mechanism we
predict the typical eccentricities of the resulting IMRIs. We find that IMRIs
will have largely circularized by the time they enter the sensitivity band of
ground-based detectors. Hardening of a binary via three-body interactions,
which is likely to be the dominant mechanism for IMRI formation, yields
eccentricities under 10^-4 when the GW frequency reaches 10 Hz. Even among
IMRIs formed via direct captures, which can have the highest eccentricities,
around 90% will circularize to eccentricities under 0.1 before the GW frequency
reaches 10 Hz. We estimate the rate of IMRI coalescences in globular clusters
and the sensitivity of a network of three Advanced LIGO detectors to the
resulting GWs. We show that this detector network may see up to tens of IMRIs
per year, although rates of one to a few per year may be more plausible. We
also estimate the loss in signal-to-noise ratio that will result from using
circular IMRI templates for data analysis and find that, for the eccentricities
we expect, this loss is negligible.Comment: Accepted for publication in ApJ; revised version reflects changes
made to the article during the acceptance proces
Electrically Driven Light Emission from Individual CdSe Nanowires
We report electroluminescence (EL) measurements carried out on three-terminal
devices incorporating individual n-type CdSe nanowires. Simultaneous optical
and electrical measurements reveal that EL occurs near the contact between the
nanowire and a positively biased electrode or drain. The surface potential
profile, obtained by using Kelvin probe microscopy, shows an abrupt potential
drop near the position of the EL spot, while the band profile obtained from
scanning photocurrent microscopy indicates the existence of an n-type Schottky
barrier at the interface. These observations indicate that light emission
occurs through a hole leakage or an inelastic scattering induced by the rapid
potential drop at the nanowire-electrode interface.Comment: 12 pages, 4 figure
Constraints on post-depositional isotope modifications in East Antarctic firn from analysing temporal changes of isotope profiles
The isotopic composition of water in ice sheets is extensively used to infer past climate changes. In low-accumulation regions their interpretation is, however, challenged by poorly constrained effects that may influence the initial isotope signal during and after deposition of the snow. This is reflected in snow-pit isotope data from Kohnen Station, Antarctica, which exhibit a seasonal cycle but also strong interannual variations that contradict local temperature observations. These inconsistencies persist even after averaging many profiles and are thus not explained by local stratigraphic noise. Previous studies have suggested that post-depositional processes may significantly influence the isotopic composition of East Antarctic firn. Here, we investigate the importance of post-depositional processes within the open-porous firn (âłâŻ10âŻcm depth) at Kohnen Station by separating spatial from temporal variability. To this end, we analyse 22 isotope profiles obtained from two snow trenches and examine the temporal isotope modifications by comparing the new data with published trench data extracted 2 years earlier. The initial isotope profiles undergo changes over time due to downward advection, firn diffusion and densification in magnitudes consistent with independent estimates. Beyond that, we find further modifications of the original isotope record to be unlikely or small in magnitude (âȘâŻ1âŻâ° RMSD). These results show that the discrepancy between local temperatures and isotopes most likely originates from spatially coherent processes prior to or during deposition, such as precipitation intermittency or systematic isotope modifications acting on drifting or loose surface snow
Superconductivity enhanced conductance fluctuations in few layer graphene nanoribbons
We investigate the mesoscopic disorder induced rms conductance variance
in a few layer graphene nanoribbon (FGNR) contacted by two
superconducting (S) Ti/Al contacts. By sweeping the back-gate voltage, we
observe pronounced conductance fluctuations superimposed on a linear background
of the two terminal conductance G. The linear gate-voltage induced response can
be modeled by a set of inter-layer and intra-layer capacitances.
depends on temperature T and source-drain voltage .
increases with decreasing T and . When lowering , a
pronounced cross-over at a voltage corresponding to the superconducting energy
gap is observed. For |V_{sd}|\ltequiv \Delta the fluctuations are
markedly enhanced. Expressed in the conductance variance of one
graphene-superconducutor (G-S) interface, values of 0.58 e^2/h are obtained at
the base temperature of 230 mK. The conductance variance in the sub-gap region
are larger by up to a factor of 1.4-1.8 compared to the normal state. The
observed strong enhancement is due to phase coherent charge transfer caused by
Andreev reflection at the nanoribbon-superconductor interface.Comment: 15 pages, 5 figure
Non-volatile molecular memory elements based on ambipolar nanotube field effect transistors
We have fabricated air-stable n-type, ambipolar carbon nanotube field effect
transistors (CNFETs), and used them in nanoscale memory cells. N-type
transistors are achieved by annealing of nanotubes in hydrogen gas and
contacting them by cobalt electrodes. Scanning gate microscopy reveals that the
bulk response of these devices is similar to gold-contacted p-CNFETs,
confirming that Schottky barrier formation at the contact interface determines
accessibility of electron and hole transport regimes. The transfer
characteristics and Coulomb Blockade (CB) spectroscopy in ambipolar devices
show strongly enhanced gate coupling, most likely due to reduction of defect
density at the silicon/silicon-dioxide interface during hydrogen anneal. The CB
data in the ``on''-state indicates that these CNFETs are nearly ballistic
conductors at high electrostatic doping. Due to their nanoscale capacitance,
CNFETs are extremely sensitive to presence of individual charge around the
channel. We demonstrate that this property can be harnessed to construct data
storage elements that operate at the few-electron level.Comment: 6 pages text, 3 figures and 1 table of content graphic; available as
NanoLetters ASAP article on the we
The role of contacts in graphene transistors: A scanning photocurrent study
A near-field scanning optical microscope is used to locally induce
photocurrent in a graphene transistor with high spatial resolution. By
analyzing the spatially resolved photo-response, we find that in the n-type
conduction regime a p-n-p structure forms along the graphene device due to the
doping of the graphene by the metal contacts. The modification of the
electronic structure is not limited only underneath the metal electrodes, but
extends 0.2-0.3 um into the graphene channel. The asymmetric conduction
behavior of electrons and holes that is commonly observed in graphene
transistors is discussed in light of the potential profiles obtained from this
photocurrent imaging approach. Furthermore, we show that photocurrent imaging
can be used to probe single- / multi-layer graphene interfaces
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