623 research outputs found

    Spin- and time-resolved photoemission studies of thin Co2FeSi Heusler alloy films

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    We have studied the possibly half metallic Co2FeSi full Heusler alloy by means of spin- and time-resolved photoemission spectroscopy. For excitation, the second and fourth harmonic of femtosecond Ti:sapphire lasers were used, with photon energies of 3.1 eV and 5.9 eV, respectively. We compare the dependence of the measured surface spin polarization on the particular photoemission mechanism, i.e. 1-photon-photoemission (1PPE) or 2-photon photoemission (2PPE). The observed differences in the spin polarization can be explained by a spin-dependent lifetime effect occurring in the 2-photon absorption process. The difference in escape depth of the two methods in this context suggests that the observed reduction of spin polarization (compared to the bulk) cannot be attributed just to the outermost surface layer but takes place at least 4-6 nm away from the surface.Comment: 7 pages, 3 figures; submitted to Journal of Magnetism and Magnetic Material

    Experimental time-resolved photoemission and ab initio study of lifetimes of excited electrons in Mo and Rh

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    We have studied the relaxation dynamics of optically excited electrons in molybdenum and rhodium by means of time resolved two-photon photoemission spectroscopy (TR-2PPE) and ab initio electron self-energy calculations performed within the GW and GW+T approximations. Both theoretical approaches reproduce qualitatively the experimentally observed trends and differences in the lifetimes of excited electrons in molybdenum and rhodium. For excitation energies exceeding the Fermi energy by more than 1 eV, the GW+T theory yields lifetimes in quantitative agreement with the experimental results. As one of the relevant mechanisms causing different excited state lifetime in Mo and Rh we identify the occupation of the 4d bands. An increasing occupation of the 4d bands results in an efficient decrease of the lifetime even for rather small excitation energies of a few 100 meV.Comment: 8 pages, 10 figure

    Une genre de nouvelle discrimination chromatique

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    Une mode comme celle des baskets rouges est un prétexte à distinguer les classes sociales. On pourrait continuer d'imaginer pour chaque groupe de femmes et d'hommes une couleur qui correspondrait au mieux à leurs aspirations et finirait par les décrire, au pied de la lettre. Pour démontrer que l'écriture inclusive devrait être aussi variée que les couleurs possibles de chaussures, ce récit distingue douze types de formulation non hétérosexiste adaptés sur mesure à autant de catégories d'individus.A trend such as the red sneakers one is a pretext to distinguish between social classes. We could keep on imagining for every group of women and men a colour matching as much as possible what they aspire to be, and at the end, which could literally describe them. To prove that gender-neutral language [or inclusive writing] should be as multifarious as the possibilities of shoes' colour, this narrative distinguish between twelve types of non-heterosexist phrasing, made to measure to so many categories of persons

    Love kills: Simulations in Penna Ageing Model

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    The standard Penna ageing model with sexual reproduction is enlarged by adding additional bit-strings for love: Marriage happens only if the male love strings are sufficiently different from the female ones. We simulate at what level of required difference the population dies out.Comment: 14 pages, including numerous figure

    Dynamics of Excited Electrons in Copper and Ferromagnetic Transition Metals: Theory and Experiment

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    Both theoretical and experimental results for the dynamics of photoexcited electrons at surfaces of Cu and the ferromagnetic transition metals Fe, Co, and Ni are presented. A model for the dynamics of excited electrons is developed, which is based on the Boltzmann equation and includes effects of photoexcitation, electron-electron scattering, secondary electrons (cascade and Auger electrons), and transport of excited carriers out of the detection region. From this we determine the time-resolved two-photon photoemission (TR-2PPE). Thus a direct comparison of calculated relaxation times with experimental results by means of TR-2PPE becomes possible. The comparison indicates that the magnitudes of the spin-averaged relaxation time \tau and of the ratio \tau_\uparrow/\tau_\downarrow of majority and minority relaxation times for the different ferromagnetic transition metals result not only from density-of-states effects, but also from different Coulomb matrix elements M. Taking M_Fe > M_Cu > M_Ni = M_Co we get reasonable agreement with experiments.Comment: 23 pages, 11 figures, added a figure and an appendix, updated reference

    Deterministic spatio-temporal control of nano-optical fields in optical antennas and nano transmission lines

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    We show that pulse shaping techniques can be applied to tailor the ultrafast temporal response of the strongly confined and enhanced optical near fields in the feed gap of resonant optical antennas (ROAs). Using finite-difference time-domain (FDTD) simulations followed by Fourier transformation, we obtain the impulse response of a nano structure in the frequency domain, which allows obtaining its temporal response to any arbitrary pulse shape. We apply the method to achieve deterministic optimal temporal field compression in ROAs with reduced symmetry and in a two-wire transmission line connected to a symmetric dipole antenna. The method described here will be of importance for experiments involving coherent control of field propagation in nanophotonic structures and of light-induced processes in nanometer scale volumes.Comment: 5 pages, 5 figure

    Structure and electronic properties of the (3×3\sqrt{3}\times \sqrt{3})R30R30^{\circ} SnAu2_2/Au(111) surface alloy

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    We have investigated the atomic and electronic structure of the (3×3\sqrt{3}\times \sqrt{3})R30R30^{\circ} SnAu2_2/Au(111) surface alloy. Low energy electron diffraction and scanning tunneling microscopy measurements show that the native herringbone reconstruction of bare Au(111) surface remains intact after formation of a long range ordered (3×3\sqrt{3}\times \sqrt{3})R30R30^{\circ} SnAu2_22/Au(111) surface alloy. Angle-resolved photoemission and two-photon photoemission spectroscopy techniques reveal Rashba-type spin-split bands in the occupied valence band with comparable momentum space splitting as observed for the Au(111) surface state, but with a hole-like parabolic dispersion. Our experimental findings are compared with density functional theory (DFT) calculation that fully support our experimental findings. Taking advantage of the good agreement between our DFT calculations and the experimental results, we are able to extract that the occupied Sn-Au hybrid band is of (s, d)-orbital character while the unoccupied Sn-Au hybrid bands are of (p, d)-orbital character. Hence, we can conclude that the Rashba-type spin splitting of the hole-like Sn-Au hybrid surface state is caused by the significant mixing of Au d- to Sn s-states in conjunction with the strong atomic spin-orbit coupling of Au, i.e., of the substrate.Comment: Copyright: https://journals.aps.org/authors/transfer-of-copyright-agreement; All copyrights by AP
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