3,113 research outputs found

    Novel phase diagram of superconductor NaxCoO2-yH2O in a 75 % relative humidity

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    We succeeded in synthesizing the powder samples of bilayer-hydrate sodium cobalt oxide superconductors NaxCoO2-yH2O with Tc = 0 ~ 4.6 K by systematically changing the keeping duration in a 75 % relative humidity atmosphere after intercalation of water molecules. From the magnetic measurements, we found that the one-day duration sample does not show any superconductivity down to 1.8 K, and that the samples kept for 2 ~ 7 days show superconductivity, in which Tc increases up to 4.6 K with increasing the duration. Tc and the superconducting volume fraction are almost invariant between 7 days and 1month duration. The 59Co NQR spectra indicate a systematic change in the local charge distribution on the CoO2 plane with change in duration.Comment: 4 pages, 5 figures, submitted to Journal of the Physical Society of Japa

    Superconductivity Phase Diagram of Na(x)CoO(2).1.3H(2)O

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    Although the microscopic origin of the superconductivity in high Tc copper oxides remains the subject of active inquiry, several of their electronic characteristics are well established as universal to all the known materials, forming the experimental foundation that all theories must address. The most fundamental of those characteristics is the dependence of the superconducting transition temperature on the degree of electronic band filling. Since the discovery of cuprate superconductivity in 1986 (1), the search for other families of superconductors that might help shed light on the superconducting mechanism of the cuprates has been of great interest. The recent report of superconductivity near 4K in the triangular lattice, layered sodium cobalt oxyhydrate, Na0.35CoO2.1.3H2O, is the best indication that superconductors related to the cuprates may be found (2). Here we show that the superconducting transition temperature of this compound displays the same kind of band-filling behavior that is observed in the cuprates. Specifically, that the optimal superconducting Tc occurs in a narrow range of band filling, and decreases for both underdoped and overdoped materials, in dramatic analogy to the phase diagram of the cuprate superconductors. Our results suggest that characterization of the detailed electronic and magnetic behavior of these new materials may help establish which of the many special characteristics of the cuprates is fundamental to their high Tc superconductivity.Comment: revised, publication information adde

    Spin and Charge Josephson effects between non-uniform superconductors with coexisting helimagnetic order

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    We consider the spin and charge Josephson current between two non-uniform Fulde-Ferrel-Larkin-Ovchinnikov superconductors with helimagnetic order. We demonstrate that the presence of the helimagnetic phase generates a spin Josephson effect and leads to additional contributions to both single-particle and Josephson charge current. It is shown that for such systems the AC effect differs more radically from the DC effect than in the case of a BCS superconductor with helimagnetic order considered earlier in the literature [M. L. Kuli\'c and I. M. Kuli\'c, Phys. Rev. B {\bf 63}, 104503 (2001)] where a spin Josephson current has also been found. In our system the most interesting effect occurs in the presence of an external magnetic field and in absence of voltage, where we show that the charge Josephson current can be tuned to zero while the spin Josephson current is non-vanishing. This provides a well controlled mechanism to generate a spin supercurrent in absence of charge currents.Comment: final versio

    Anomalous magnetic properties near Mott transition in Kagom\'e lattice Hubbard model

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    We investigate the characteristics of the metallic phase near the Mott transition in the Kagom\'e lattice Hubbard model using the cellular dynamical mean field theory. By calculating the specific heat and spin correlation functions, we demonstrate that the quasiparticles show anomalous properties in the metallic phase close to the Mott transition. We find clear evidence for the multi-band heavy quasiparticles in the specific heat, which gives rise to unusual temperature dependence of the spin correlation functions.Comment: 2 pages, 3 figures, accepted for publication in J. Mag. Mag. Mater. (Proceedings of the ICM, Kyoto, Japan, August 2006

    Electronic Collective Modes and Superconductivity in Layered Conductors

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    A distinctive feature of layered conductors is the presence of low-energy electronic collective modes of the conduction electrons. This affects the dynamic screening properties of the Coulomb interaction in a layered material. We study the consequences of the existence of these collective modes for superconductivity. General equations for the superconducting order parameter are derived within the strong-coupling phonon-plasmon scheme that account for the screened Coulomb interaction. Specifically, we calculate the superconducting critical temperature Tc taking into account the full temperature, frequency and wave-vector dependence of the dielectric function. We show that low-energy plasmons may contribute constructively to superconductivity. Three classes of layered superconductors are discussed within our model: metal-intercalated halide nitrides, layered organic materials and high-Tc oxides. In particular, we demonstrate that the plasmon contribution (electronic mechanism) is dominant in the first class of layered materials. The theory shows that the description of so-called ``quasi-two-dimensional superconductors'' cannot be reduced to a purely 2D model, as commonly assumed. While the transport properties are strongly anisotropic, it remains essential to take into account the screened interlayer Coulomb interaction to describe the superconducting state of layered materials.Comment: Final version (minor changes) 14 pages, 6 figure

    Behavior of a frustrated quantum spin chain with bond dimerization

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    We clarified behavior of the excitation gap in a frustrated S=1/2 quantum spin chain with bond dimerization by using the numerical diagonalization of finite systems and a variational approach. The model interpolates between the independent dimer model and the S=1 spin chain by changing a strength of the dimerization. The energy gap is minimum at the fully-frustrated point, where a localized kink and a freely mobile anti-kink govern the low-lying excitations. Away from the point, a kink and an antikink form a bound state by an effective triangular potential between them. The consequential gap enhancement and the localization length of the bound state is obtained exactly in the continuous limit. The gap enhancement obeys a power law with exponent 2/3. The method and the obtained results are common to other frustrated double spin-chain systems, such as the one-dimensional J_1 - J_2 model, or the frustrated ladder model.Comment: 11 pages, REVTeX, 8 figures in eps-fil

    Breached pairing superfluidity: Possible realization in QCD

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    We propose a wide universality class of gapless superfluids, and analyze a limit that might be realized in quark matter at intermediate densities. In the breached pairing color superconducting phase heavy ss-quarks, with a small Fermi surface, pair with light uu or dd quarks. The groundstate has a superfluid and a normal Fermi component simultaneously. We expect a second order phase transition, as a function of increasing density, from the breached pairing phase to the conventional color-flavor locked (CFL) phase.Comment: 5 pages, latex, 1 figure; added references; Comment on Ref. [10] change

    Including nonlocality in exchange-correlation kernel from time-dependent current density functional theory: Application to the stopping power of electron liquids

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    We develop a scheme for building the scalar exchange-correlation (xc) kernel of time-dependent density functional theory (TDDFT) from the tensorial kernel of time-dependent {\em current} density functional theory (TDCDFT) and the Kohn-Sham current density response function. Resorting to the local approximation to the kernel of TDCDFT results in a nonlocal approximation to the kernel of TDDFT, which is free of the contradictions that plague the standard local density approximation (LDA) to TDDFT. As an application of this general scheme, we calculate the dynamical xc contribution to the stopping power of electron liquids for slow ions to find that our results are in considerably better agreement with experiment than those obtained using TDDFT in the conventional LDA.Comment: 6 pages, 3 figures, accepted to Phys. Rev.

    Interior Gap Superfluidity

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    We propose a new state of matter in which the pairing interactions carve out a gap within the interior of a large Fermi ball, while the exterior surface remains gapless. This defines a system which contains both a superfluid and a normal Fermi liquid simultaneously, with both gapped and gapless quasiparticle excitations. This state can be realized at weak coupling. We predict that a cold mixture of two species of fermionic atoms with different mass will exhibit this state. For electrons in appropriate solids, it would define a material that is simultaneously superconducting and metallic.Comment: 5 page
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