Investigation of ββ\beta\beta decay in 150^{150}Nd and 148^{148}Nd to the excited states of daughter nuclei

Double beta decay of $^{150}$Nd and $^{148}$Nd to the excited states of daughter nuclei have been studied using a 400 cm$^3$ low-background HPGe detector and an external source consisting of 3046 g of natural Nd$_2$O$_3$ powder. The half-life for the two-neutrino double beta decay of $^{150}$Nd to the excited 0$^+_1$ state in $^{150}$Sm is measured to be $T_{1/2}=[1.33^{+0.36}_{-0.23}(stat)^{+0.27}_{-0.13}(syst)]\cdot 10^{20}$ y. For other $(0\nu + 2\nu)$ transitions to the 2$^+_1$, 2$^+_2$, 2$^+_3$, and 0$^+_2$ levels in $^{150}$Sm, limits are obtained at the level of $\sim (2-8)\cdot 10^{20}$ y. In the case of $^{148}$Nd only limits for the $(0\nu + 2\nu)$ transitions to the 2$^+_1$, 0$^+_1$, and 2$^+_2$ excited states in $^{148}$Sm were obtained and are at the level of \sim (4-8)\cdot 10^{20}$ y.Comment: 13 pages, 6 figure

Search for β+\beta^+EC and ECEC processes in 112^{112}Sn

Limits on $\beta^+$EC (here EC denotes electron capture) and ECEC processes in $^{112}$Sn have been obtained using a 380 cm$^3$ HPGe detector and an external source consisting of 53.355 g enriched tin (94.32% of $^{112}$Sn). A limit with 90% C.L. on the $^{112}$Sn half-life of $4.7\times 10^{20}$ y for the ECEC(0$\nu$) transition to the $0^+_3$ excited state in $^{112}$Cd (1871.0 keV) has been established. This transition is discussed in the context of a possible enhancement of the decay rate by several orders of magnitude given that the ECEC$(0\nu)$ process is nearly degenerate with an excited state in the daughter nuclide. Prospects for investigating such a process in future experiments are discussed. The limits on other $\beta^+$EC and ECEC processes in $^{112}$Sn were obtained on the level of $(0.6-8.7)\times 10^{20}$ y at the 90% C.L.Comment: 14 pages, 4 figure

Phase stability, ordering tendencies, and magnetism in single-phase fcc Au-Fe nanoalloys

Bulk Au-Fe alloys separate into Au-based fcc and Fe-based bcc phases, but L1$_0$ and L1$_2$ orderings were reported in single-phase Au-Fe nanoparticles. Motivated by these observations, we study the structural and ordering energetics in this alloy by combining density functional theory (DFT) calculations with effective Hamiltonian techniques: a cluster expansion with structural filters, and the configuration-dependent lattice deformation model. The phase separation tendency in Au-Fe persists even if the fcc-bcc decomposition is suppressed. The relative stability of disordered bcc and fcc phases observed in nanoparticles is reproduced, but the fully ordered L1$_0$ AuFe, L1$_2$ Au$_3$Fe, and L1$_2$ AuFe$_3$ structures are unstable in DFT. However, a tendency to form concentration waves at the corresponding [001] ordering vector is revealed in nearly-random alloys in a certain range of concentrations. This incipient ordering requires enrichment by Fe relative to the equiatomic composition, which may occur in the core of a nanoparticle due to the segregation of Au to the surface. Effects of magnetism on the chemical ordering are also discussed.Comment: 23 pages, 11 figure

First test of an enriched 116^{116}CdWO4_4 scintillating bolometer for neutrinoless double-beta-decay searches

For the first time, a cadmium tungstate crystal scintillator enriched in $^{116}$Cd has been succesfully tested as a scintillating bolometer. The measurement was performed above ground at a temperature of 18 mK. The crystal mass was 34.5 g and the enrichment level ~82 %. Despite a substantial pile-up effect due to above-ground operation, the detector demonstrated a high energy resolution (2-7 keV FWHM in 0.2-2.6 MeV $\gamma$ energy range), a powerful particle identification capability and a high level of internal radiopurity. These results prove that cadmium tungstate is an extremely promising detector material for a next-generation neutrinoless double-beta decay bolometric experiment, like that proposed in the CUPID project (CUORE Upgrade with Particle IDentification)

Searches for neutrinoless double beta decay

Neutrinoless double beta decay is a lepton number violating process whose observation would also establish that neutrinos are their own anti-particles. There are many experimental efforts with a variety of techniques. Some (EXO, Kamland-Zen, GERDA phase I and CANDLES) started take data in 2011 and EXO has reported the first measurement of the half life for the double beta decay with two neutrinos of $^{136}$Xe. The sensitivities of the different proposals are reviewed.Comment: 8 pages, prepared for TAUP 201

Double beta decay: present status

The present status of double beta decay experiments (including the search for $2\beta^{+}$, EC$\beta^{+}$ and ECEC processes) are reviewed. The results of the most sensitive experiments are discussed. Average and recommended half-life values for two-neutrino double beta decay are presented. Conservative upper limits on effective Majorana neutrino mass and the coupling constant of the Majoron to the neutrino are established as $< 0.75$ eV and $<g_{ee} > < 1.9 \cdot 10^{-4}$, respectively. Proposals for future double beta decay experiments with a sensitivity for the $$ at the level of (0.01-0.1) eV are considered.Comment: 33 pages included 7 figures and 14 tables; an extended version of the invited talk at 13th Lomonosov Conference of Elementary Particle Physics, 23-29 August, 2007, Moscow, Russi

Improvement of radiopurity level of enriched 116^{116}CdWO4_4 and ZnWO4_4 crystal scintillators by recrystallization

As low as possible radioactive contamination of a detector plays a crucial role to improve sensitivity of a double beta decay experiment. The radioactive contamination of a sample of $^{116}$CdWO$_4$ crystal scintillator by thorium was reduced by a factor $\approx 10$, down to the level 0.01 mBq/kg ($^{228}$Th), by exploiting the recrystallization procedure. The total alpha activity of uranium and thorium daughters was reduced by a factor $\approx 3$, down to 1.6 mBq/kg. No change in the specific activity (the total $\alpha$ activity and $^{228}$Th) was observed in a sample of ZnWO$_4$ crystal produced by recrystallization after removing $\approx 0.4$ mm surface layer of the crystal.Comment: 14 pages, 5 figures and 2 table

Searches for neutrinoless double beta decay

Neutrinoless double beta decay is a lepton number violating process whose observation would also establish that neutrinos are their own anti-particles. There are many experimental efforts with a variety of techniques. Some (EXO, Kamland-Zen, GERDA phase I and CANDLES) started take data in 2011 and EXO has reported the first measurement of the half life for the double beta decay with two neutrinos of $^{136}$Xe. The sensitivities of the different proposals are reviewed.Comment: 8 pages, prepared for TAUP 201