2,024 research outputs found
Production of long-lived atomic vapor inside high-density buffer gas
Atomic vapor of four different paramagnetic species: gold, silver, lithium,
and rubidium, is produced and studied inside several buffer gases: helium,
nitrogen, neon, and argon. The paramagnetic atoms are injected into the buffer
gas using laser ablation. Wires with diameters 25 m, 50 m, and 100
m are used as ablation targets for gold and silver, bulk targets are used
for lithium and rubidium. The buffer gas cools and confines the ablated atoms,
slowing down their transport to the cell walls. Buffer gas temperatures between
20 K and 295 K, and densities between cm and
cm are explored. Peak paramagnetic atom densities of cm
are routinely achieved. The longest observed paramagnetic vapor density decay
times are 110 ms for silver at 20 K and 4 ms for lithium at 32 K. The
candidates for the principal paramagnetic-atom loss mechanism are impurities in
the buffer gas, dimer formation and atom loss on sputtered clusters.Comment: Some minor editorial changes and corrections, added reference
Quantum theory of an atom laser originating from a Bose-Einstein condensate or a Fermi gas in the presence of gravity
We present a 3D quantum mechanical theory of radio-frequency outcoupled atom
lasers from trapped atomic gases in the presence of the gravitational force.
Predictions for the total outcoupling rate as a function of the radio-frequency
and for the beam wave function are given. We establish a sum rule for the
energy integrated outcoupling, which leads to a separate determination of the
coupling strength between the atoms and the radiation field.
For a non-interacting Bose-Einstein condensate analytic solutions are derived
which are subsequently extended to include the effects of atomic interactions.
The interactions enhance interference effects in the beam profile and modify
the outcoupling rate of the atom laser. We provide a complete quantum
mechanical solution which is in line with experimental findings and allows to
determine the validity of commonly used approximative methods.
We also extend the formalism to a fermionic atom laser and analyze the effect
of superfluidity on the outcoupling of atoms.Comment: 13 pages, 8 figures, slightly expanded versio
Theoretical study of molecular electronic excitations and optical transitions of C60
We report results on ab initio calculations of excited states of the
fullerene molecule by using configuration interaction (CI) approach with singly
excited determinants (SCI). We have used both the experimental geometry and the
one optimized by the density functional method and worked with basis sets at
the cc-pVTZ and aug-cc-pVTZ level. Contrary to the early SCI semiempirical
calculations, we find that two lowest electron
optical lines are situated at relatively high energies of ~5.8 eV (214 nm) and
~6.3 eV (197 nm). These two lines originate from two transitions: from HOMO to (LUMO+1) () and from (HOMO--1)
to LUMO (). The lowest molecular excitation, which is the level, is found at ~2.5 eV. Inclusion of doubly excited determinants
(SDCI) leads only to minor corrections to this picture. We discuss possible
assignment of absorption bands at energies smaller than 5.8 eV (or
larger than 214 nm).Comment: 6 pages, 1 figure, 9 Table
On the mutual polarization of two He-4 atoms
We propose a simple method based on the standard quantum-mechanical
perturbation theory to calculate the mutual polarization of two atoms He^4.Comment: 9 pages, 1 table; the article is revised and the calculation is
essentially refined; v4: final version, the Introduction is delete
Strong fragmentation of low-energy electromagnetic excitation strength in Sn
Results of nuclear resonance fluorescence experiments on Sn are
reported. More than 50 transitions with MeV were
detected indicating a strong fragmentation of the electromagnetic excitation
strength. For the first time microscopic calculations making use of a complete
configuration space for low-lying states are performed in heavy odd-mass
spherical nuclei. The theoretical predictions are in good agreement with the
data. It is concluded that although the E1 transitions are the strongest ones
also M1 and E2 decays contribute substantially to the observed spectra. In
contrast to the neighboring even Sn, in Sn the
component of the two-phonon quintuplet built on top of
the 1/2 ground state is proved to be strongly fragmented.Comment: 4 pages, 3 figure
The GREAT triggerless total data readout method
Recoil decay tagging (RDT) is a very powerful method for the spectroscopy of exotic nuclei. RDT is a delayed coincidence technique between detectors usually at the target position and at the focal plane of a spectrometer. Such measurements are often limited by dead time. This paper describes a novel triggerless data acquisition method, which is being developed for the Gamma Recoil Electron Alpha Tagging (GREAT) spectrometer, that overcomes this limitation by virtually eliminating dead time. Our solution is a total data readout (TDR) method where all channels run independently and are associated in software to reconstruct events. The TDR method allows all the data from both target position and focal plane to be collected with practically no dead-time losses. Each data word is associated with a timestamp generated from a global 100-MHz clock. Events are then reconstructed in real time in the event builder using temporal and spatial associations defined by the physics of the experimen
Lower Rydberg series of methane : A combined coupled cluster linear response and molecular quantum defect orbital calculation
Vertical excitation energies as well as related absolute photoabsorption oscillator strength data are very scarce in the literature for methane. In this study, we have characterized the three existing series of low-lying Rydberg states of CH4 by computing coupled cluster linear response (CCLR) vertical excitation energies together with oscillator strengths in the molecular-adapted quantum defect orbital formalism from a distorted Cs geometry selected on the basis of outer valence green function calculations. The present work provides a wide range of data of excitation energies and absolute oscillator strengths which correspond to the Rydberg series converging to the three lower ionization potential values of the distorted methane molecule, in energy regions for which experimentally measured data appear to be [email protected] [email protected] [email protected]
Infrared emission spectrum and potentials of and states of Xe excimers produced by electron impact
We present an investigation of the Xe excimer emission spectrum
observed in the near infrared range about 7800 cm in pure Xe gas and in
an Ar (90%) --Xe (10%) mixture and obtained by exciting the gas with energetic
electrons. The Franck--Condon simulation of the spectrum shape suggests that
emission stems from a bound--free molecular transition never studied before.
The states involved are assigned as the bound state with atomic limit and the dissociative state with limit. Comparison with the spectrum simulated by using theoretical
potentials shows that the dissociative one does not reproduce correctly the
spectrum features.Comment: 4 pages, 3 figures, submitted to Phys. Rev. Let
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