Lattice dynamics and the electron-phonon interaction in Ca2_2RuO4_4

We present a Raman scattering study of Ca$_2$RuO$_4$, in which we investigate the temperature-dependence of the lattice dynamics and the electron-phonon interaction below the metal-insulator transition temperature ({\it T}$_{\rm MI}$). Raman spectra obtained in a backscattering geometry with light polarized in the ab-plane reveal 9 B$_{1g}$ phonon modes (140, 215, 265, 269, 292, 388, 459, 534, and 683 cm$^{-1}$) and 9 A$_g$ phonon modes (126, 192, 204, 251, 304, 322, 356, 395, and 607 cm$^{-1}$) for the orthorhombic crystal structure (Pbca$-$D$_{2h}^{15}$). With increasing temperature toward {\it T}$_{\rm MI}$, the observed phonon modes shift to lower energies and exhibit reduced spectral weights, reflecting structural changes associated with the elongation of the RuO$_6$ octahedra. Interestingly, the phonons exhibit significant increases in linewidths and asymmetries for {\it T} $>$ {\it T}$_{\rm N}$. These results indicate that there is an increase in the effective number of electrons and the electron-phonon interaction strengths as the temperature is raised through {\it T}$_{\rm N}$, suggesting the presence of orbital fluctuations in the temperature regime {\it T}$_{\rm N}$ $<$ {\it T} $<$ {\it T}$_{\rm MI}$.Comment: 6 pages, 4 figure

Mechanism of hopping transport in disordered Mott insulators

By using a combination of detailed experimental studies and simple theoretical arguments, we identify a novel mechanism characterizing the hopping transport in the Mott insulating phase of Ca$_{2-x}$Sr$_x$RuO$_4$ near the metal-insulator transition. The hopping exponent $\alpha$ shows a systematic evolution from a value of $\alpha=1/2$ deeper in the insulator to the conventional Mott value $\alpha=1/3$ closer to the transition. This behavior, which we argue to be a universal feature of disordered Mott systems close to the metal-insulator transition, is shown to reflect the gradual emergence of disorder-induced localized electronic states populating the Mott-Hubbard gap.Comment: 5 pages, 3 figures, To be published in Physical Review Letter

Active Galaxies and Cluster Gas

Two lines of evidence indicate that active galaxies, principally radio galaxies, have heated the diffuse hot gas in clusters. The first is the general need for additional heating to explain the steepness of the X-ray luminosity--temperature relation in clusters, the second is to solve the cooling flow problem in cluster cores. The inner core of many clusters is radiating energy as X-rays on a timescale much shorter than its likely age. Although the temperature in this region drops by a factor of about 3 from that of the surrounding gas, little evidence is found for gas much cooler than that. Some form of heating appears to be taking place, probably by energy transported outward from the central accreting black hole or radio source. How that energy heats the gas depends on poorly understood transport properties (conductivity and viscosity) of the intracluster medium. Viscous heating is discussed as a possibility. Such heating processes have consequences for the truncation of the luminosity function of massive galaxies.Comment: 14 pages, 16 fig, Feb 2004 talk for Phil Trans Roy So

Orbital ordering transition in Ca2_2RuO4_4 observed with resonant x-ray diffraction

Resonant x-ray diffraction performed at the $\rm L_{II}$ and $\rm L_{III}$ absorption edges of Ru has been used to investigate the magnetic and orbital ordering in Ca$_2$RuO$_4$ single crystals. A large resonant enhancement due to electric dipole $2p\to 4d$ transitions is observed at the wave-vector characteristic of antiferromagnetic ordering. Besides the previously known antiferromagnetic phase transition at $\rm T_{N}=110$ K, an additional phase transition, between two paramagnetic phases, is observed around 260 K. Based on the polarization and azimuthal angle dependence of the diffraction signal, this transition can be attributed to orbital ordering of the Ru $t_{2g}$ electrons. The propagation vector of the orbital order is inconsistent with some theoretical predictions for the orbital state of Ca$_2$RuO$_4$.Comment: to appear in PR

High resolution soft X-ray spectroscopy of the elliptical galaxy NGC 5044. Results from the reflection grating spectrometer on-board XMM-Newton

The results from an X-ray spectroscopic study of the giant elliptical galaxy NGC5044 in the center of a galaxy group are presented. The line dominated soft X-ray spectra (mainly Fe-L and O VIII Ly_a) from the diffuse gas are resolved for the first time in this system with the Reflection Grating Spectrometers on-board XMM-Newton and provide a strong constraint on the temperature structure. The spectra integrated over 2' (\sim 20kpc) in full-width can be described by a two temperature plasma model of 0.7keV and 1.1keV. Most of the latter component is consistent with originating from off-center regions. Compared to the isobaric cooling flow prediction, the observation shows a clear cut-off below a temperature of 0.6 +-0.1keV. Furthermore, the Fe and O abundances within the central 10--20kpc in radius are accurately measured to be 0.55+-0.05 and 0.25+-0.1 times the solar ratios, respectively. The observed cut-off temperature of this galaxy and other central galaxies in galaxy groups and clusters are compared with the scale of the galaxy and properties of the surrounding intra-cluster medium. Based on this comparison, the origin of the lack of predicted cool emission is discussed.Comment: Accepted for publication in Astronomy & Astrophysic

Possible Multiple Gap Superconductivity with Line Nodes in Heavily Hole-Doped Superconductor KFe2As2 Studied by 75As-NQR and Specific Heat

We report the 75As nuclear quadrupole resonance (NQR) and specific heat measurements of the heavily hole-doped superconductor KFe2As2 (Tc = 3.5 K). The spin-lattice relaxation rate 1/T1 in the superconducting state exhibits quite gradual temperature dependence with no coherence peak below Tc. The quasi-particle specific heat C_QP/T shows small specific heat jump which is about 30% of electronic specific heat coefficient just below Tc. In addition, it suggests the existence of low-energy quasi-particle excitation at the lowest measurement temperature T = 0.4 K \simeq Tc/10. These temperature dependence of 1/T1 and C_QP/T can be explained by multiple nodal superconducting gap scenario rather than multiple fully-gapped s_\pm-wave one within simple gap analysis.Comment: 5 pages, 5 figures, to be published in J. Phys. Soc. Jpn. No.8 issue (2009

X-ray Diagnostics of Thermal Conditions of the Hot Plasmas in the Centaurus Cluster

X-ray data of the Centaurus cluster, obtained with {\it XMM-Newton} for 45 ksec, were analyzed. Deprojected EPIC spectra from concentric thin shell regions were reproduced equally well by a single-phase plasma emission model, or by a two-phase model developed by {\it ASCA}, both incorporating cool (1.7--2.0 keV) and hot ($\sim 4$ keV) plasma temperatures. However, EPIC spectra with higher statistics, accumulated over 3-dimentional thick shell regions, were reproduced better by the two-phase model than by the singe-phase one. Therefore, hot and cool plasma phases are inferred to co-exist in the cluster core region within $\sim 70$ kpc. The iron and silicon abundances of the plasma were reconfirmed to increase significantly towards the center, while that of oxygen was consistent with being radially constant. The implied non-solar abundance ratios explains away the previously reported excess X-ray absorption from the central region. Although an additional cool ($\sim 0.7$ keV) emission was detected within $\sim 20$ kpc of the center, the RGS data gave tight upper limits on any emission with a tempeartures below $\sim 0.5$ keV. These results are compiled into a magnetosphere model, which interprets the cool phase as confined within closed magnetic loops anchored to the cD galaxy. When combined with so-called Rosner-Tucker-Vaiana mechanism which applies to solar coronae, this model can potentially explain basic properties of the cool phase, including its temperature and thermal stability.Comment: 53 pages, 11 figures, accepted for publication in Astrophysical Journa

Pressure-Tuned Collapse of the Mott-Like State in Ca_{n+1}Ru_nO_{3n+1} (n=1,2): Raman Spectroscopic Studies

We report a Raman scattering study of the pressure-induced collapse of the Mott-like phases of Ca_3Ru_2O_7 (T_N=56 K) and Ca_2RuO_4 (T_N=110 K). The pressure-dependence of the phonon and two-magnon excitations in these materials indicate: (i) a pressure-induced collapse of the antiferromagnetic (AF) insulating phase above P* ~ 55 kbar in Ca_3Ru_2O_7 and P* ~ 5-10 kbar in Ca_2RuO_4, reflecting the importance of Ru-O octahedral distortions in stabilizing the AF insulating phase; and (ii) evidence for persistent AF correlations above the critical pressure of Ca_2RuO_4, suggestive of phase separation involving AF insulator and ferromagnetic metal phases.Comment: 3 figure

An ASCA Study of the Heavy Element Distribution in Clusters of Galaxies

We perform a spatially resolved X-ray spectroscopic study of a set of 11 relaxed clusters of galaxies observed by the ROSAT/PSPC and ASCA/SIS. Using a method which corrects for the energy dependent effects of the ASCA PSF based on ROSAT images, we constrain the spatial distribution of Ne, Si, S and Fe in each cluster. Theoretical prescriptions for the chemical yields of Type Ia and II supernovae, then allow determination of the Fe enrichment from both types of supernovae as a function of radius within each cluster. Using optical measurements from the literature, we also determine the iron mass-to-light ratio (IMLR) separately for Fe synthesized in both types of supernovae. For clusters with the best photon statistics, we find that the total Fe abundance decreases significantly with radius, while the Si abundance is either flat or decreases less rapidly, resulting in an increasing Si/Fe ratio with radius. This result indicates a greater predominance of Type II SNe enrichment at large radii in clusters. We suggest that the high Si/Fe ratios in the outskirts of rich clusters may arise from enrichment by Type II SNe released to ICM via galactic star burst driven winds. Abridged.Comment: 17 pages, ApJ in press (Nov. 2000), a study of systematics is adde

Commensurate Itinerant Antiferromagnetism in BaFe2As2: 75As-NMR Studies on a Self-Flux Grown Single Crystal

We report results of 75As nuclear magnetic resonance (NMR) experiments on a self-flux grown single crystal of BaFe2As2. A first-order antiferromagnetic (AF) transition near 135 K was detected by the splitting of NMR lines, which is accompanied by simultaneous structural transition as evidenced by a sudden large change of the electric field gradient tensor at the As site. The NMR results lead almost uniquely to the stripe spin structure in the AF phase. The data of spin-lattice relaxation rate indicate development of anisotropic spin fluctuations of the stripe-type with decreasing temperature in the paramagnetic phase.Comment: 7 pages, 7 figures, accepted for publication in J. Phys. Soc. Jp