290 research outputs found
Assembly of Colloidal Aggregates by Electrohydrodynamic Flow: Kinetic Experiments and Scaling Analysis
Electric fields generate transverse flows near electrodes that sweep colloidal particles into densely packed assemblies. We interpret this behavior in terms of electrohydrodynamic motion stemming from distortions of the field by the particles that alter the body force distribution in the electrode charge polarization layer. A scaling analysis shows how the action of the applied electric field generates fluid motion that carries particles toward one another. The resulting fluid velocity is proportional to the square of the applied field and decreases inversely with frequency. Experimental measurements of the particle aggregation rate accord with the electrohydrodynamic theory over a wide range of voltages and frequencies
Spin dynamics in high- superconductors
Key features of antiferromagnetic dynamical correlations in high-
superconductors cuprates are discussed. In underdoped regime, the sharp
resonance peak, occuring exclusively in the SC state, is accompanied by a
broader contribution located around 30 meV which remains above .
Their interplay may induce incommensurate structure in the superconducting
state.Comment: HTS99 Proceedings Miami (January 7-11 1999
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Precipitation and Deposition of Aluminum-Containing Phases in Tank Wastes
In the first phase of our study, we focused on the use of simple organics to raise the solubility of aluminum oxyhydroxides in high alkaline aqueous solvents. In a limited survey of common organic acids, we determined that citric acid had the highest potential to achieve our goal. However, our subsequent investigation revealed that the citric acid appeared to play two roles in the solutions: first, raising the concentration of aluminum in highly alkaline solutions by breaking up or inhibiting ''seed'' polycations and thereby delaying the nucleation and growth of particles; and second, stabilizing nanometer-sized particles in suspension when nucleation did occur. The results of this work were recently published in Langmuir: D.M. Dabbs, U. Ramachandran, S. Lu, J. Liu, L.-Q. Wang, I.A. Aksay, ''Inhibition of Aluminum Oxyhydroxide Precipitation with Citric Acid'' Langmuir, 21, 11690-11695 (2005). The second phase of our work involved the solvation of silicon, again in solutions of high alkalinity. Citric acid, due to its unfavorable pKa values, was not expected to be useful with silicon-containing solutions. Here, the use of polyols was determined to be effective in maintaining silicon-containing particles under high pH conditions but at smaller size with respect to standard suspensions of silicon-containing particles. There were a number of difficulties working with highly alkaline silicon-containing solutions, particularly in solutions at or near the saturation limit. Small deviations in pH resulted in particle formation or dissolution in the absence of the organic agents. One of the more significant observations was that the polyols appeared to stabilize small particles of silicon oxyhydroxides across a wider range of pH, albeit this was difficult to quantify due to the instability of the solutions
Superconductivity-Induced Anomalies in the Spin Excitation Spectra of Underdoped YBa_2 Cu_3 O_{6+x}
Polarized and unpolarized neutron scattering has been used to determine the
effect of superconductivity on the magnetic excitation spectra of YBa_2 Cu_3
O_{6.5} (T_c = 52K) and YBa_2 Cu_3 O_{6.7} (T_c = 67K). Pronounced enhancements
of the spectral weight centered around 25 meV and 33 meV, respectively, are
observed below T_c in both crystals, compensated predominantly by a loss of
spectral weight at higher energies. The data provide important clues to the
origin of the 40 meV magnetic resonance peak in YBa_2 Cu_3 O_7.Comment: LaTex, 4 pages, 4 ps figures. to appear in Phys. Rev. Let
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Aluminum-Containing Phases in Tank Waste: Precipitation and Deposition of Aluminum-Containing Phases
Aluminosilicate deposit buildup experienced during the tank waste volume-reduction process at the Savannah River Site (SRS) required an evaporator to be shut down in October 1999. Recent investigations illustrated the accumulation 7 wt% uranium, 3% was 235U and absent of neutron poisons, within these deposits and presented a criticality concern. The Waste Processing Technology Section of Westinghouse Savannah River Company at SRS is now collaborating with a team from Pacific Northwest National Laboratory in efforts to identify the phases controlling uranium solubility and understand the conditions under which they precipitate
Evaluation of YBa₂Cu₃O₇₋ₓ Bulk Superconductors for High Field Magnet Applications
Processing of YBCO single crystals was carried out by solidification of semi-liquid YBCO composition using a seeding technique. Microstructural characterization of the pinning centers was investigated by transmission electron microscopy. Characterization of single crystals was carried out, relating grain size and shape to the corresponding flux profiles. Current densities were calculated based on measured trapped fields. Once circulating currents were established, flux pumping and quenching experiments were conducted. These large single crystals will be incorporated into electromagnetic forming devices for use in the military and commercial aircraft manufacturing and service industries
High energy spin excitations in YBa_2 Cu_3 O_{6.5}
Inelastic neutron scattering has been used to obtain a comprehensive
description of the absolute dynamical spin susceptibility
of the underdoped superconducting cuprate YBa_2 Cu_3 O_{6.5} ()
over a wide range of energies and temperatures ( and ). Spin excitations of two different
symmetries (even and odd under exchange of two adjacent CuO_2 layers) are
observed which, surprisingly, are characterized by different temperature
dependences. The excitations show dispersive behavior at high energies.Comment: 15 pages, 5 figure
Quantum Impurities and the Neutron Resonance Peak in : Ni versus Zn
The influence of magnetic (S=1) and nonmagnetic (S=0) impurities on the spin
dynamics of an optimally doped high temperature superconductor is compared in
two samples with almost identical superconducting transition temperatures:
YBa(CuNi)O (T=80 K) and
YBa(CuZn)O (T=78 K). In the Ni-substituted
system, the magnetic resonance peak (which is observed at E40 meV in
the pure system) shifts to lower energy with a preserved E/T ratio
while the shift is much smaller upon Zn substitution. By contrast Zn, but not
Ni, restores significant spin fluctuations around 40 meV in the normal state.
These observations are discussed in the light of models proposed for the
magnetic resonance peak.Comment: 3 figures, submitted to PR
Effect of Nonmagnetic Impurities on the Magnetic Resonance Peak in YBa2Cu3O7
The magnetic excitation spectrum of a YBa_2 Cu_3 O_7 crystal containing 0.5%
of nonmagnetic (Zn) impurities has been determined by inelastic neutron
scattering. Whereas in the pure system a sharp resonance peak at E ~ 40 meV is
observed exclusively below the superconducting transition temperature T_c, the
magnetic response in the Zn-substituted system is broadened significantly and
vanishes at a temperature much higher than T_c. The energy-integrated spectral
weight observed near q = (pi,pi) increases with Zn substitution, and only about
half of the spectral weight is removed at T_c
İzmir‐Ankara suture as a Triassic to Cretaceous plate boundary – data from central Anatolia
The İzmir‐Ankara suture represents part of the boundary between Laurasia and Gondwana along which a wide Tethyan ocean was subducted. In northwest Turkey, it is associated with distinct oceanic subduction‐accretion complexes of Late Triassic, Jurassic and Late Cretaceous ages. The Late Triassic and Jurassic accretion complexes consist predominantly of basalt with lesser amounts of shale, limestone, chert, Permian (274 Ma zircon U‐Pb age) metagabbro and serpentinite, which have undergone greenschist facies metamorphism. Ar‐Ar muscovite ages from the phyllites range from 210 Ma down to 145 Ma with a broad southward younging. The Late Cretaceous subduction‐accretion complex, the ophiolitic mélange, consists of basalt, radiolarian chert, shale and minor amounts of recrystallized limestone, serpentinite and greywacke, showing various degrees of blueschist facies metamorphism and penetrative deformation. Ar‐Ar phengite ages from two blueschist metabasites are ca. 80 Ma (Campanian). The ophiolitic mélange includes large Jurassic peridotite‐gabbro bodies with plagiogranites with ca. 180 Ma U‐Pb zircon ages. Geochronological and geological data show that Permian to Cretaceous oceanic lithosphere was subducted north under the Pontides from the Late Triassic to the Late Cretaceous. This period was characterized generally by subduction‐accretion, except in the Early Cretaceous, when subduction‐erosion took place. In the Sakarya segment all the subduction accretion complexes, as well as the adjacent continental sequences, are unconformably overlain by Lower Eocene red beds. This, along with the stratigraphy of the Sakarya Zone indicate that the hard collision between the Sakarya Zone and the Anatolide‐Tauride Block took place in Paleocene
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