2,881 research outputs found
Excited State Relaxation in Vacuum Deposited and Solution Processed Films of Merocyanine/Fulerene Blends
Exciton dynamics in merocyanine/fulerene blend films made by vacuum deposition and solution processing
techniques were investigated by means of steady-state and time resolved fluorescence and
absorption spectroscopy. Intermolecular charge transfer states are formed during several ps in neat
merocianine films, which determine their fluorescence properties. Fullerene additives cause formation of
new heterogeneous charge transfer states. Even a small fullerene concentration significantly influences
the exciton dynamics by quenching inherent merocianine fluorescent states and causing appearance of new
fluorescence bands caused by the charge transfer states between merocyanine and fullerene molecules. All
fluorescence bands are quenched in films with high fulerence concentration due to the charge carrier generation,
and the quenching effect is stronger in vacuum deposited films.
When you are citing the document, use the following link http://essuir.sumdu.edu.ua/handle/123456789/3529
Collisionless energy absorption in the short-pulse intense laser-cluster interaction
In a previous Letter [Phys. Rev. Lett. 96, 123401 (2006)] we have shown by
means of three-dimensional particle-in-cell simulations and a simple
rigid-sphere model that nonlinear resonance absorption is the dominant
collisionless absorption mechanism in the intense, short-pulse laser cluster
interaction. In this paper we present a more detailed account of the matter. In
particular we show that the absorption efficiency is almost independent of the
laser polarization. In the rigid-sphere model, the absorbed energy increases by
many orders of magnitude at a certain threshold laser intensity. The
particle-in-cell results display maximum fractional absorption around the same
intensity. We calculate the threshold intensity and show that it is
underestimated by the common over-barrier ionization estimate.Comment: 12 pages, 13 figures, RevTeX
Ensemble inequivalence in systems with long-range interactions
Ensemble inequivalence has been observed in several systems. In particular it
has been recently shown that negative specific heat can arise in the
microcanonical ensemble in the thermodynamic limit for systems with long-range
interactions. We display a connection between such behaviour and a mean-field
like structure of the partition function. Since short-range models cannot
display this kind of behaviour, this strongly suggests that such systems are
necessarily non-mean field in the sense indicated here. We illustrate our
results showing an application to the Blume-Emery-Griffiths model. We further
show that a broad class of systems with non-integrable interactions are indeed
of mean-field type in the sense specified, so that they are expected to display
ensemble inequivalence as well as the peculiar behaviour described above in the
microcanonical ensemble.Comment: 12 pages, no figure
Domain wall mobility in nanowires: transverse versus vortex walls
The motion of domain walls in ferromagnetic, cylindrical nanowires is
investigated numerically by solving the Landau-Lifshitz-Gilbert equation for a
classical spin model in which energy contributions from exchange, crystalline
anisotropy, dipole-dipole interaction, and a driving magnetic field are
considered. Depending on the diameter, either transverse domain walls or vortex
walls are found. The transverse domain wall is observed for diameters smaller
than the exchange length of the given material. Here, the system behaves
effectively one-dimensional and the domain wall mobility agrees with a result
derived for a one-dimensional wall by Slonczewski. For low damping the domain
wall mobility decreases with decreasing damping constant. With increasing
diameter, a crossover to a vortex wall sets in which enhances the domain wall
mobility drastically. For a vortex wall the domain wall mobility is described
by the Walker-formula, with a domain wall width depending on the diameter of
the wire. The main difference is the dependence on damping: for a vortex wall
the domain wall mobility can be drastically increased for small values of the
damping constant up to a factor of .Comment: 5 pages, 6 figure
General-Relativistic Thomas-Fermi model
A system of self-gravitating massive fermions is studied in the framework of
the general-relativistic Thomas-Fermi model. We study the properties of the
free energy functional and its relation to Einstein's field equations. A
self-gravitating fermion gas we then describe by a set of Thomas-Fermi type
self-consistency equations.Comment: 7 pages, LaTex, to appear in Gen. Rel. Gra
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