Coherent transport in a two-electron quantum dot molecule

We investigate the dynamics of two interacting electrons confined to a pair of coupled quantum dots driven by an external AC field. By numerically integrating the two-electron Schroedinger equation in time, we find that for certain values of the strength and frequency of the AC field we can cause the electrons to be localised within the same dot, in spite of the Coulomb repulsion between them. Reducing the system to an effective two-site model of Hubbard type and applying Floquet theory leads to a detailed understanding of this effect. This demonstrates the possibility of using appropriate AC fields to manipulate entangled states in mesoscopic devices on extremely short timescales, which is an essential component of practical schemes for quantum information processing.Comment: 4 pages, 3 figures; the section dealing with the perturbative treatment of the Floquet states has been substantially expanded to make it easier to follo

Recurrence of fidelity in near integrable systems

Within the framework of simple perturbation theory, recurrence time of quantum fidelity is related to the period of the classical motion. This indicates the possibility of recurrence in near integrable systems. We have studied such possibility in detail with the kicked rotor as an example. In accordance with the correspondence principle, recurrence is observed when the underlying classical dynamics is well approximated by the harmonic oscillator. Quantum revivals of fidelity is noted in the interior of resonances, while classical-quantum correspondence of fidelity is seen to be very short for states initially in the rotational KAM region.Comment: 13 pages, 6 figure

Harmonic generation in ring-shaped molecules

We study numerically the interaction between an intense circularly polarized laser field and an electron moving in a potential which has a discrete cylindrical symmetry with respect to the laser pulse propagation direction. This setup serves as a simple model, e.g., for benzene and other aromatic compounds. From general symmetry considerations, within a Floquet approach, selection rules for the harmonic generation [O. Alon Phys. Rev. Lett. 80 3743 (1998)] have been derived recently. Instead, the results we present in this paper have been obtained solving the time-dependent Schroedinger equation ab initio for realistic pulse shapes. We find a rich structure which is not always dominated by the laser harmonics.Comment: 15 pages including 7 figure

High-order Harmonic Generation and Dynamic Localization in a driven two-level system, a non-perturbative solution using the Floquet-Green formalism

We apply the Floquet-Green operator formalism to the case of a harmonically-driven two-level system. We derive exact expressions for the quasi-energies and the components of the Floquet eigenstates with the use of continued fractions. We study the avoided crossings structure of the quasi-energies as a function of the strength of the driving field and give an interpretation in terms of resonant multi-photon processes. From the Floquet eigenstates we obtain the time-evolution operator. Using this operator we study Dynamic Localization and High-order Harmonic Generation in the non-perturbative regime

Transmission Properties of the oscillating delta-function potential

We derive an exact expression for the transmission amplitude of a particle moving through a harmonically driven delta-function potential by using the method of continued-fractions within the framework of Floquet theory. We prove that the transmission through this potential as a function of the incident energy presents at most two real zeros, that its poles occur at energies $n\hbar\omega+\varepsilon^*$ ($0<Re(\varepsilon^*)<\hbar\omega$), and that the poles and zeros in the transmission amplitude come in pairs with the distance between the zeros and the poles (and their residue) decreasing with increasing energy of the incident particle. We also show the existence of non-resonant "bands" in the transmission amplitude as a function of the strength of the potential and the driving frequency.Comment: 21 pages, 12 figures, 1 tabl

Changes in Floquet state structure at avoided crossings: delocalization and harmonic generation

Avoided crossings are common in the quasienergy spectra of strongly driven nonlinear quantum wells. In this paper we examine the sinusoidally driven particle in a square potential well to show that avoided crossings can alter the structure of Floquet states in this system. Two types of avoided crossings are identified: on type leads only to temporary changes (as a function of driving field strength) in Floquet state structure while the second type can lead to permanent delocalization of the Floquet states. Radiation spectra from these latter states show significant increase in high harmonic generation as the system passes through the avoided crossing.Comment: 8 pages with 10 figures submitted to Physical Review

Floquet scattering in parametric electron pumps

A Floquet scattering approach to parametric electron pumps is presented and compared with Brouwer's adiabatic scattering approach [Phys. Rev. B 58, R10135 (1998)] for a simple scattering model with two harmonically oscillating delta-function barriers. For small strength of oscillating potentials these two approaches give exactly equivalent results while for large strength, these clearly deviate from each other. The validity of the adiabatic theory is also discussed by using the Wigner delay time obtained from the Floquet scattering matrix.Comment: 10 pages, 7 figure

Exact exchange-correlation potential for a time-dependent two electron system

We obtain an exact solution of the time-dependent Schroedinger equation for a two-electron system confined to a plane by an isotropic parabolic potential whose curvature is periodically modulated in time. From this solution we compute the exact time-dependent exchange correlation potential v_xc which enters the Kohn-Sham equation of time-dependent density functional theory. Our exact result provides a benchmark against which various approximate forms for v_xc can be compared. Finally v_xc is separated in an adiabatic and a pure dynamical part and it is shown that, for the particular system studied, the dynamical part is negligible.Comment: 23 pages, 6 figure

Floquet Formalism of Quantum Pumps

We review Floquet formalism of quantum electron pumps. In the Floquet formalism the quantum pump is regarded as a time dependent scattering system, which allows us to go beyond the adiabatic limit. It can be shown that the well-known adiabatic formula given by Brouwer can be derived from the adiabatic limit of Floquet formalism. We compare various physical properties of the quantum pump both in the adiabatic and in the non-adiabatic regime using the Floquet theory.Comment: Latex2e 16 pages, 6 figures. A review paper to appear in Int. J. Mod. Phys.

Nonperturbative Coherent Population Trapping: An Analytic Model

Coherent population trapping is shown to occur in a driven symmetric double-well potential in the strong-field regime. The system parameters have been chosen to reproduce the $0^{-}\leftrightarrow 3^{+}$ transition of the inversion mode of the ammonia molecule. For a molecule initially prepared in its lower doublet we find that, under certain circumstances, the $3^{+}$ level remains unpopulated, and this occurs in spite of the fact that the laser field is resonant with the $0^{-}\leftrightarrow 3^{+}$ transition and intense enough so as to strongly mix the $0^{+}$ and $0^{-}$ ground states. This counterintuitive result constitutes a coherent population trapping phenomenon of nonperturbative origin which cannot be accounted for with the usual models. We propose an analytic nonperturbative model which accounts correctly for the observed phenomenon.Comment: 5 pages, 2 figure