83 research outputs found

    Absence of Edge Localized Moments in the Doped Spin-Peierls System CuGe1x_{1-x}Six_{x}O3_3

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    We report the observation of nuclear quadrupole resonance (NQR) of Cu from the sites near the doping center in the spin-Peierls system CuGe1x_{1-x}Six_{x}O3_3. The signal appears as the satellites in the Cu NQR spectrum, and has a suppressed nuclear spin-lattice relaxation rate indicative of a singlet correlation rather than an enhanced magnetic correlation near the doping center. Signal loss of Cu nuclei with no neighboring Si is also observed. We conclude from these observations that the doping-induced moments are not in the vicinity of the doping center but rather away from it.Comment: 4 pages, 4 figures, accepted for publication in Phys. Rev. Let

    Phase Inhomogeneity of the Itinerant Ferromagnet MnSi at High Pressures

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    The pressure induced quantum phase transition of the weakly itinerant ferromagnet MnSi is studied using zero-field 29Si^{29}Si NMR spectroscopy and relaxation. Below P1.2GPaP^*\approx 1.2GPa, the intensity of the signal and the nuclear spin-lattice relaxation is independent of pressure, even though the amplitude of the magnetization drops by 20% from the ambient pressure amplitude. For P>PP>P^*, the decreasing intensity within the experimentally detectable bandwidth signals the onset of an inhomogeneous phase that persists to the highest pressure measured, P1.75GPaP\ge 1.75GPa, which is well beyond the known critical pressure Pc=1.46GPaP_c=1.46GPa. Implications for the non-Fermi Liquid behavior observed for P>PcP>P_c are discussed.Comment: 4 pages, 4 figure

    Unconventional ferromagnetic and spin-glass states of the reentrant spin glass Fe0.7Al0.3

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    Spin excitations of single crystal Fe0.7Al0.3 were investigated over a wide range in energy and reciprocal space with inelastic neutron scattering. In the ferromagnetic phase, propagating spin wave modes become paramagnon-like diffusive modes beyond a critical wave vector q0, indicating substantial disorder in the long-range ordered state. In the spin glass phase, spin dynamics is strongly q-dependent, suggesting remnant short-range spin correlations. Quantitative model for S(energy,q) in the ``ferromagnetic'' phase is determined.Comment: 4 pages, 5 figure

    Itinerant-Electron Magnet of the Pyrochlore Lattice: Indium-Doped YMn2Zn20

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    We report on a ternary intermetallic compound, "YMn2Zn20", comprising a pyrochlore lattice made of Mn atoms. A series of In-doped single crystals undergo no magnetic long-range order down to 0.4 K, in spite of the fact that the Mn atom carries a local magnetic moment at high temperatures, showing Curie-Weiss magnetism. However, In-rich crystals exhibit spin-glass transitions at approximately 10 K due to a disorder arising from the substitution, while, with decreasing In content, the spin-glass transition temperature is reduced to 1 K. Then, heat capacity divided by temperature approaches a large value of 280 mJ K-2 mol-1, suggesting a significantly large mass enhancement for conduction electrons. This heavy-fermion-like behavior is not induced by the Kondo effect as in ordinary f-electron compounds, but by an alternative mechanism related to the geometrical frustration on the pyrochlore lattice, as in (Y,Sc)Mn2 and LiV2O4, which may allow spin entropy to survive down to low temperatures and to couple with conduction electrons.Comment: 5 pages, 4 figures, J. Phys. Soc. Jpn., in pres

    Bulk screening in core level photoemission from Mott-Hubbard and Charge-Transfer systems

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    We report bulk-sensitive hard X-ray (hνh\nu = 5.95 KeV) core level photoemission spectroscopy (PES) of single crystal V1.98_{1.98}Cr0.02_{0.02}O3_{3} and the high-TcT_c cuprate Bi2_2Sr2_{2}CaCu2_{2}O8+δ_{8+\delta} (Bi2212). V1.98_{1.98}Cr0.02_{0.02}O3_{3} exhibits low binding energy "satellites" to the V 2p2p "main lines" in the metallic phase, which are suppressed in the antiferromagnetic insulator phase. In contrast, the Cu 2p2p spectra of Bi2212 do not show temperature dependent features, but a comparison with soft X-ray PES indicates a large increase in the 2p53d92p^5 3d^9 "satellites" or 3d93d^9 weight in the bulk. Cluster model calculations, including full multiplet structure and a screening channel derived from the coherent band at the Fermi energy, give very satisfactory agreement with experiments

    Coexistence of double alternating antiferromagnetic chains in (VO)_2P_2O_7 : NMR study

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    Nuclear magnetic resonance (NMR) of 31P and 51V nuclei has been measured in a spin-1/2 alternating-chain compound (VO)_2P_2O_7. By analyzing the temperature variation of the 31P NMR spectra, we have found that (VO)_2P_2O_7 has two independent spin components with different spin-gap energies. The spin gaps are determined from the temperature dependence of the shifts at 31P and 51V sites to be 35 K and 68 K, which are in excellent agreement with those observed in the recent inelastic neutron scattering experiments [A.W. Garrett et al., Phys. Rev. Lett. 79, 745 (1997)]. This suggests that (VO)_2P_2O_7 is composed of two magnetic subsystems showing distinct magnetic excitations, which are associated with the two crystallographically-inequivalent V chains running along the b axis. The difference of the spin-gap energies between the chains is attributed to the small differences in the V-V distances, which may result in the different exchange alternation in each magnetic chain. The exchange interactions in each alternating chain are estimated and are discussed based on the empirical relation between the exchange interaction and the interatomic distance.Comment: 10 pages, 11 embedded eps figures, REVTeX, Submitted to Phys. Rev.

    Magnetic fluctuations in frustrated Laves hydrides R(Mn_{1-x}Al_{x})_{2}H_{y}

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    By neutron scattering, we have studied the spin correlations and spin fluctuations in frustrated Laves hydrides, where magnetic disorder sets in the topologically frustrated Mn lattice. Below the transition towards short range magnetic order, static spin clusters coexist with fluctuating and alsmost uncorrelated spins. The magnetic response shows a complexe lineshape, connected with the presence of the magnetic inhomogeneities. Its analysis shows the existence of two different processes, relaxation and local excitations, for the spin fluctuations below the transition. The paramagnetic fluctuations are discussed in comparison with classical spin glasses, cluster glasses, and non Fermi liquid itinerant magnets

    Nonlinear magnetic susceptibility and aging phenomena in reentrant ferromagnet: Cu0.2_{0.2}Co0.8_{0.8}Cl2_{2}-FeCl3_{3} graphite bi-intercalation compound

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    Linear and nonlinear dynamic properties of a reentrant ferromagnet Cu0.2_{0.2}Co0.8_{0.8}Cl2_{2}-FeCl3_{3} graphite bi-intercalation compound are studied using AC and DC magnetic susceptibility. This compound undergoes successive phase transitions at the transition temperatures ThT_{h} (= 16 K), TcT_{c} (= 9.7 K), and TRSGT_{RSG} (= 3.5 K). The static and dynamic behaviors of the reentrant spin glass phase below TRSGT_{RSG} are characterized by those of normal spin glass phase with critical exponent β\beta = 0.57 ±\pm 0.10, a dynamic critical exponent xx = 8.5 ±\pm 1.8, and an exponent pp (= 1.55 ±\pm 0.13) for the de Almeida -Thouless line. A prominent nonlinear susceptibility is observed between TRSGT_{RSG} and TcT_{c} and around ThT_{h}, suggesting a chaotic nature of the ferromagnetic phase (TRSGTTcT_{RSG} \leq T \leq T_{c}) and the helical spin ordered phase (TcTThT_{c} \leq T \leq T_{h}). The aging phenomena are observed both in the RSG and FM phases, with the same qualitative features as in normal spin glasses. The aging of zero-field cooled magnetization indicates a drastic change of relaxation mechanism below and above TRSGT_{RSG}. The time dependence of the absorption χ\chi^{\prime \prime} is described by a power law form (tb\approx t^{-b^{\prime \prime}}) in the ferromagnetic phase, where b0.074±0.016b^{\prime \prime} \approx 0.074 \pm 0.016 at ff = 0.05 Hz and TT = 7 K. No ωt\omega t-scaling law for χ\chi^{\prime \prime} [(ωt)b\approx (\omega t)^{-b^{\prime \prime}}] is observed.Comment: 14 pages, 16 figures, and 2 table

    MicroRNA-196b is an independent prognostic biomarker in patients with pancreatic cancer

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    microRNA-196bは膵癌において異常高発現しており,多変量解析で不良な予後に相関した.その阻害剤は膵癌細胞株において抗腫瘍効果を示すことから,microRNA-196bは診断バイオマーカーおよび治療標的となることが示唆された

    Support for UNRWA's survival

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    The United Nations Relief and Works Agency for Palestine Refugees in the Near East (UNRWA) provides life-saving humanitarian aid for 5·4 million Palestine refugees now entering their eighth decade of statelessness and conflict. About a third of Palestine refugees still live in 58 recognised camps. UNRWA operates 702 schools and 144 health centres, some of which are affected by the ongoing humanitarian disasters in Syria and the Gaza Strip. It has dramatically reduced the prevalence of infectious diseases, mortality, and illiteracy. Its social services include rebuilding infrastructure and homes that have been destroyed by conflict and providing cash assistance and micro-finance loans for Palestinians whose rights are curtailed and who are denied the right of return to their homeland
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