109 research outputs found
Pressure-temperature phase diagram of the heavy-electron superconductor URu2Si2
The pressure-temperature phase diagram of the heavy-electron superconductor
URu2Si2 has been reinvestigated by ac-susceptibility and elastic
neutron-scattering (NS) measurements performed on a small single-crystalline
rod (2 mm in diameter, 6 mm in length) in a Cu-Be clamp-type high-pressure cell
(P < 1.1 GPa). At ambient pressure, this sample shows the weakest
antiferromagnetic (AF) Bragg reflections reported so far, corresponding to the
volume-averaged staggered moment of mord ~ 0.011 mB/U. Under applied pressure,
the AF scattering intensity exhibits a sharp increase at P ~ 0.7 GPa at low
temperatures. The saturation value of the AF scattering intensity above 0.7 GPa
corresponds to mord ~ 0.41 mB/U, which is in good agreement with that (~ 0.39
mB/U) observed above 1.5 GPa in our previous NS measurements. The
superconductivity is dramatically suppressed by the evolution of AF phase,
indicating that the superconducting state coexists only with the hidden order
phase. The presence of parasitic ferro- and/or antiferromagnetic phases with
transition temperatures T1star =120(5) K, T2star = 36(3) K and T3star = 16.5(5)
K and their relationship to the low-T ordered phases are also discussed.Comment: 6 pages, 7 figures, submitted to J. Magn. Magn. Mater. (ICM2006
Competition between hidden order and antiferromagnetism in URu_2Si_2 under uniaxial stress studied by neutron scattering
We have performed elastic neutron scattering experiments under uniaxial
stress sigma applied along the tetragonal [100], [110] and [001] directions for
the heavy electron compound URu2Si2. We found that antiferromagnetic (AF) order
with large moment is developed with sigma along the [100] and [110] directions.
If the order is assumed to be homogeneous, the staggered ordered moment mu_o
continuously increases from 0.02 mu_B (sigma=0) to 0.22 mu_B (0.25 GPa). The
rate of increase partial mu_o/partial sigma is ~ 1.0 mu_B/GPa, which is four
times larger than that for the hydrostatic pressure (partial mu_o/partial P sim
0.25 mu_B/GPa). Above 0.25 GPa, mu_o shows a tendency to saturate, similar to
the hydrostatic pressure behavior. For sigma||[001], mu_o shows only a slight
increase to 0.028 mu_B (sigma = 0.46 GPa) with a rate of ~ 0.02 mu_B/GPa,
indicating that the development of the AF state highly depends on the direction
of sigma. We have also found a clear hysteresis loop in the isothermal
mu_o(sigma) curve obtained for sigma||[110] under the zero-stress-cooled
condition at 1.4 K. This strongly suggests that the sigma-induced AF phase is
metastable, and separated from the "hidden order" phase by a first-order phase
transition. We discuss these experimental results on the basis of crystalline
strain effects and elastic energy calculations, and show that the c/a ratio
plays a key role in the competition between these two phases.Comment: 9 pages, 7 figures, to appear in Physical Review
Magnetic Quantum Phase Transitions in Kondo Lattices
The identification of magnetic quantum critical points in heavy fermion
metals has provided an ideal setting for experimentally studying quantum
criticality. Motivated by these experiments, considerable theoretical efforts
have recently been devoted to reexamine the interplay between Kondo screening
and magnetic interactions in Kondo lattice systems. A local quantum critical
picture has emerged, in which magnetic interactions suppress Kondo screening
precisely at the magnetic quantum critical point (QCP). The Fermi surface
undergoes a large reconstruction across the QCP and the coherence scale of the
Kondo lattice vanishes at the QCP. The dynamical spin susceptibility exhibits
scaling and non-trivial exponents describe the temperature and
frequency dependence of various physical quantities. These properties are to be
contrasted with the conventional spin-density-wave (SDW) picture, in which the
Kondo screening is not suppressed at the QCP and the Fermi surface evolves
smoothly across the phase transition. In this article we discuss recent
microscopic studies of Kondo lattices within an extended dynamical mean field
theory (EDMFT). We summarize the earlier work based on an analytical
-expansion renormalization group method, and expand on the more
recent numerical results. We also discuss the issues that have been raised
concerning the magnetic phase diagram. We show that the zero-temperature
magnetic transition is second order when double counting of the RKKY
interactions is avoided in EDMFT.Comment: 10 pages, 4 figures; references added; as published in JPCM in early
September, except for the correction to the legend for Figure
Neutron Scattering Study on Competition between Hidden Order and Antiferromagnetism in U(Ru_{1-x}Rh_x)_2Si_2 (x <= 0.05)
We have performed elastic and inelastic neutron scattering experiments on the
solid solutions U(Ru_{1-x}Rh_x)_2Si_2 for the Ru rich concentrations: x=0,
0.01, 0.02, 0.025, 0.03, 0.04 and 0.05. Hidden order is suppressed with
increasing x, and correspondingly the onset temperature T_m (~ 17.5 K at x=0)
of weak antiferromagnetic (AF) Bragg reflection decreases. For x=0.04 and 0.05,
no magnetic order is detected in the investigated temperature range down to 1.4
K. In the middle range, 0.02 <= x <= 0.03, we found that the AF Bragg
reflection is strongly enhanced. At x=0.02, this takes place at ~ 7.7 K (=T_M),
which is significantly lower than T_m (~ 13.7 K). T_M increases with increasing
x, and seems to merge with T_m at x=0.03. If the AF state is assumed to be
homogeneous, the staggered moment \mu_o estimated at 1.4 K increases from
0.02(2) \mu_B/U (x=0) to 0.24(1) \mu_B/U (x=0.02). The behavior is similar to
that observed under hydrostatic pressure (\mu_o increases to ~ 0.25 \mu_B/U at
1.0 GPa), suggesting that the AF evolution induced by Rh doping is due to an
increase in the AF volume fraction. We also found that the magnetic excitation
observed at Q=(1,0,0) below T_m disappears as T is lowered below T_M.Comment: 4 pages, 4 figures, submitted to J. Phys. Soc. Jp
Susceptibility Inhomogeneity and Non-Fermi-Liquid Behavior in Ce(Ru_{0.5}Rh_{0.5})_2Si_2
Magnetic susceptibility and muon spin rotation (\muSR) experiments have been
carried out to study the effect of structural disorder on the non-Fermi-liquid
(NFL) behavior of the heavy-fermion alloy Ce(Ru_{0.5}Rh_{0.5})_2Si_2. Analysis
of the bulk susceptibility in the framework of disorder-driven Griffiths-phase
and Kondo-disorder models for NFL behavior yields relatively narrow
distributions of characteristic spin fluctuation energies, in agreement with
\muSR linewidths that give the inhomogeneous spread in susceptibility. \muSR
and NMR data both indicate that disorder explains the "nearly NFL" behavior
observed above \sim2 K, but does not dominate the NFL physics found at low
temperatures and low magnetic fields.Comment: 6 pages, 4 figures, REVTeX, submitted to Phys. Rev.
Non-Fermi-Liquid Scaling in Ce(Ru_{0.5}Rh_{0.5})_2Si_2
We study the temperature and field dependence of the magnetic and transport
properties of the non-Fermi-liquid compound Ce(Ru_{1-x}Rh_x)_2Si_2 at x=0.5.
For fields 0.1T the experimental results show signatures of the
presence of Kondo-disorder, expected to be large at this concentration. For
larger fields, however, magnetic and transport properties are controlled by the
coupling of the conduction electrons to critical spin-fluctuations. The
temperature dependence of the susceptibility as well as the scaling properties
of the magnetoresistance are in very good agreement with the predictions of
recent dynamical mean-field theories of Kondo alloys close to a spin-glass
quantum critical point.Comment: 4 pages, 4 figures. Improved discussion. To appear in Phys. Rev. Let
Further analysis of the quantum critical point of CeLaRuSi
New data on the spin dynamics and the magnetic order of
CeLaRuSi are presented. The importance of the Kondo
effect at the quantum critical point of this system is emphasized from the
behaviour of the relaxation rate at high temperature and from the variation of
the ordered moment with respect to the one of the N\'eel temperature for
various .Comment: Contribution for the Festschrift on the occasion of Hilbert von
Loehneysen 60 th birthday. To be published as a special issue in the Journal
of Low Temperature Physic
Effect of Pressure on Tiny Antiferromagnetic Moment in the Heavy-Electron Compound URu_2Si_2
We have performed elastic neutron-scattering experiments on the
heavy-electron compound URu_2Si_2 for pressure P up to 2.8 GPa. We have found
that the antiferrmagnetic (100) Bragg reflection below T_m ~ 17.5 K is strongly
enhanced by applying pressure. For P < 1.1 GPa, the staggered moment mu_o at
1.4 K increases linearly from ~ 0.017(3) mu_B to ~ 0.25(2) mu_B, while T_m
increases slightly at a rate ~ 1 K/GPa, roughly following the transition
temperature T_o determined from macroscopic anomalies. We have also observed a
sharp phase transition at P_c ~ 1.5 GPa, above which a 3D-Ising type of
antiferromagnetic phase (mu_o ~ 0.4 mu_B) appears with a slightly reduced
lattice constant.Comment: RevTeX, 4 pages, 4 eps figures, accepted for publication in Phys.
Rev. Let
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