Impurity intrusion in radio-frequency micro-plasma jets operated in ambient air

Space and time resolved concentrations of helium metastable atoms in an atmospheric pressure radio-frequency micro-plasma jet were measured using tunable diode laser absorption spectroscopy. Spatial profiles as well as lifetime measurements show significant influences of air entering the discharge from the front nozzle and of impurities originating from the gas supply system. Quenching of metastables was used to deduce quantitative concentrations of intruding impurities. The impurity profile along the jet axis was determined from optical emission spectroscopy as well as their dependance on the feed gas flow through the jet.Comment: Journal of Physics D: Applied Physics (accepted), 6 page

On the fidelity of two pure states

The fidelity of two pure states (also known as transition probability) is a symmetric function of two operators, and well-founded operationally as an event probability in a certain preparation-test pair. Motivated by the idea that the fidelity is the continuous quantum extension of the combinatorial equality function, we enquire whether there exists a symmetric operational way of obtaining the fidelity. It is shown that this is impossible. Finally, we discuss the optimal universal approximation by a quantum operation.Comment: LaTeX2e, 8 pages, submitted to J. Phys. A: Math. and Ge

New Indicators for AGN Power: The Correlation Between [O IV] lambda 25.89 micron and Hard X-ray Luminosity for Nearby Seyfert Galaxies

We have studied the relationship between the [O IV] lambda 25.89 micron emission line luminosities, obtained from Spitzer spectra, the X-ray continua in the 2-10 keV band, primarily from ASCA, and the 14-195 keV band obtained with the SWIFT/Burst Alert Telescope (BAT), for a sample of nearby (z < 0.08) Seyfert galaxies. For comparison, we have examined the relationship between the [O III] 5007, the 2-10 keV and the 14-195 keV luminosities for the same set of objects. We find that both the [O IV] and [O III] luminosities are well-correlated with the BAT luminosities. On the other hand, the [O III] luminosities are better-correlated with 2-10 keV luminosities than are those of [O IV]. When comparing [O IV] and [O III] luminosities for the different types of galaxies, we find that the Seyfert 2's have significantly lower [O III] to [O IV] ratios than the Seyfert 1's. We suggest that this is due to more reddening of the narrow line region (NLR) of the Seyfert 2's. Assuming Galactic dust to gas ratios, the average amount of extra reddening corresponds to a hydrogen column density of ~ few times 10^21 cm^-2, which is a small fraction of the X-ray absorbing columns in the Seyfert 2's. The combined effects of reddening and the X-ray absorption are the probable reason why the [O III] versus 2-10 keV correlation is better than the [O IV] versus 2-10 keV, since the [O IV] emission line is much less affected by extinction. Overall, we find the [O IV] to be an accurate and truly isotropic indicator of the power of the AGN. This suggests that it can be useful in deconvolving the contribution of the AGN and starburst to the spectrum of Compton-thick and/or X-ray weak sources.Comment: Accepted for publication in the Astrophysical Journal. 31 pages, 6 figures, 4 table

Argon metastable dynamics in a filamentary jet micro-discharge at atmospheric pressure

Space and time resolved concentrations of Ar ($^{3}P_2$) metastable atoms at the exit of an atmospheric pressure radio-frequency micro-plasma jet were measured using tunable diode laser absorption spectroscopy. The discharge features a coaxial geometry with a hollow capillary as an inner electrode and a ceramic tube with metal ring as outer electrode. Absorption profiles of metastable atoms as well as optical emission measurements reveal the dynamics and the filamentary structure of the discharge. The average spatial distribution of Ar metastables is characterized with and without a target in front of the jet, showing that the target potential and therewith the electric field distribution substantially changes the filaments' expansion. Together with the detailed analysis of the ignition phase and the discharge's behavior under pulsed operation, the results give an insight into the excitation and de-excitation mechanisms

Heat kernel estimates and spectral properties of a pseudorelativistic operator with magnetic field

Based on the Mehler heat kernel of the Schroedinger operator for a free electron in a constant magnetic field an estimate for the kernel of E_A is derived, where E_A represents the kinetic energy of a Dirac electron within the pseudorelativistic no-pair Brown-Ravenhall model. This estimate is used to provide the bottom of the essential spectrum for the two-particle Brown-Ravenhall operator, describing the motion of the electrons in a central Coulomb field and a constant magnetic field, if the central charge is restricted to Z below or equal 86

Macroscopic Quantum Tunneling of Ferromagnetic Domain Walls

Quantum tunneling of domain walls out of an impurity potential in a mesoscopic ferromagnetic sample is investigated. Using improved expressions for the domain wall mass and for the pinning potential, we find that the cross-over temperature between thermal activation and quantum tunneling is of a different functional form than found previously. In materials like Ni or YIG, the crossover temperatures are around 5 mK. We also find that the WKB exponent is typically two orders of magnitude larger than current estimates. The sources for these discrepancies are discussed, and precise estimates for the transition from three-dimensional to one-dimensional magnetic behavior of a wire are given. The cross-over temperatures from thermal to quantum transitions and tunneling rates are calculated for various materials and sample sizes.Comment: 10 pages, 2 postscript figures, REVTe

Trading quantum for classical resources in quantum data compression

We study the visible compression of a source E of pure quantum signal states, or, more formally, the minimal resources per signal required to represent arbitrarily long strings of signals with arbitrarily high fidelity, when the compressor is given the identity of the input state sequence as classical information. According to the quantum source coding theorem, the optimal quantum rate is the von Neumann entropy S(E) qubits per signal. We develop a refinement of this theorem in order to analyze the situation in which the states are coded into classical and quantum bits that are quantified separately. This leads to a trade--off curve Q(R), where Q(R) qubits per signal is the optimal quantum rate for a given classical rate of R bits per signal. Our main result is an explicit characterization of this trade--off function by a simple formula in terms of only single signal, perfect fidelity encodings of the source. We give a thorough discussion of many further mathematical properties of our formula, including an analysis of its behavior for group covariant sources and a generalization to sources with continuously parameterized states. We also show that our result leads to a number of corollaries characterizing the trade--off between information gain and state disturbance for quantum sources. In addition, we indicate how our techniques also provide a solution to the so--called remote state preparation problem. Finally, we develop a probability--free version of our main result which may be interpreted as an answer to the question: ``How many classical bits does a qubit cost?'' This theorem provides a type of dual to Holevo's theorem, insofar as the latter characterizes the cost of coding classical bits into qubits.Comment: 51 pages, 7 figure

Core level photoelectron spectroscopy of heterogeneous reactions at liquid-vapor interfaces: Current status, challenges, and prospects

Liquid–vapor interfaces, particularly those between aqueous solutions and air, drive numerous important chemical and physical processes in the atmosphere and in the environment. X-ray photoelectron spectroscopy is an excellent method for the investigation of these interfaces due to its surface sensitivity, elemental and chemical specificity, and the possibility to obtain information on the depth distribution of solute and solvent species in the interfacial region. In this Perspective, we review the progress that was made in this field over the past decades and discuss the challenges that need to be overcome for investigations of heterogeneous reactions at liquid–vapor interfaces under close-torealistic environmental conditions. We close with an outlook on where some of the most exciting and promising developments might lie in this fiel

Sheared Ising models in three dimensions

The nonequilibrium phase transition in sheared three-dimensional Ising models is investigated using Monte Carlo simulations in two different geometries corresponding to different shear normals. We demonstrate that in the high shear limit both systems undergo a strongly anisotropic phase transition at exactly known critical temperatures T_c which depend on the direction of the shear normal. Using dimensional analysis, we determine the anisotropy exponent theta=2 as well as the correlation length exponents nu_parallel=1 and nu_perp=1/2. These results are verified by simulations, though considerable corrections to scaling are found. The correlation functions perpendicular to the shear direction can be calculated exactly and show Ornstein-Zernike behavior.Comment: 6 pages, 3 figure