409 research outputs found
Hybridization-Driven Orthorhombic Lattice Instability in URu2Si2
We have measured the elastic constant (C11-C12)/2 in URu2Si2 by means of
high-frequency ultrasonic measurements in pulsed magnetic fields H || [001] up
to 61.8 T in a wide temperature range from 1.5 to 116 K. We found a reduction
of (C11-C12)/2 that appears only in the temperature and magnetic field region
in which URu2Si2 exhibits a heavy-electron state and hidden-order. This change
in (C11-C12)/2 appears to be a response of the 5f-electrons to an orthorhombic
and volume conservative strain field \epsilon_xx-\epsilon_yy with
{\Gamma}3-symmetry. This lattice instability is likely related to a
symmetry-breaking band instability that arises due to the hybridization of the
localized f electrons with the conduction electrons, and is probably linked to
the hidden-order parameter of this compound.Comment: 5 pages, 4 figure
Diffraction from Ordered States of Higher Multipoles
Possible ways of identification are discussed of an electronic order of
higher multipoles such as octupoles and hexadecapoles. A particularly powerful
method is resonant X-ray scattering (RXS) using quadrupolar resonance processes
called E2.The characteristic azimuthal angle dependence of
CeLaB is interpreted as evidence of antiferro-octupole
order. For PrRuP, eightfold pattern against azimuthal angle is
predicted if its metal-insulator transition is a consequence of a hexadecapole
order. In non-resonant superlattice Bragg scattering, hexadecapole contribution
may also be identified because of absence of quadrupole component.Comment: Invited paper to be published in Proc. Hiroshima Workshop on Novel
Functional Materials with Multinary Freedoms (Physica B, 2006
Magnetic phase diagram of antiferroquadrupole ordering in HoB2C2
The magnetic phase diagram for antiferro-quadrupole (AFQ) ordering in
tetragonal HoBC has been investigated by measurements of elastic
constants , and in fields along the basal -
plane as well as the principal [001]-axis. The hybrid magnet (GAMA) in Tsukuba
Magnetic Laboratory was employed for high field measurements up to 30 T. The
AFQ phase is no longer observed above 26.3 T along the principal [001] axis in
contrast to the relatively small critical field of 3.9 T in fields applied
along the basal [110] axis. The quadrupolar intersite interaction of
and/or is consistent with the anisotropy in the magnetic phase diagram
of the AFQ phase in HoBC.Comment: Phys. Rev. B. (2005) in press. approx 8 pages, 10 figure
Lattice Distortion and Octupole Ordering Model in CexLa1-xB6
Possible order parameters of the phase IV in CexLa1-xB6 are discussed with
special attention to the lattice distortion recently observed. A
\Gamma_{5u}-type octupole order with finite wave number is proposed as the
origin of the distortion along the [111] direction. The \Gamma_8 crystalline
electric field (CEF) level splits into three levels by a mean field with the
\Gamma_{5u} symmetry. The ground and highest singlets have the same quadrupole
moment, while the intermediate doublet has an opposite sign. It is shown that
any collinear order of \Gamma_{5u}-type octupole moment accompanies the
\Gamma_{5g}-type ferro-quadrupole order, and the coupling of the quadrupole
moment with the lattice induces the distortion. The cusp in the magnetization
at the phase transition is reproduced, but the internal magnetic field due to
the octupole moment is smaller than the observed one by an order of magnitude.Comment: 5 pages, 4 figures, submitted to J. Phys. Soc. Jp
Detection of Neutron Scattering from Phase IV of Ce0.7La0.3B6: A Confirmation of the Octupole Order
We have performed a single crystal neutron scattering experiment on
Ce0.7La0.3B6 to investigate the order parameter of phase IV microscopically.
Below the phase transition temperature 1.5 K of phase IV, weak but distinct
superlattice reflections at the scattering vector (h/2,h/2,l/2) (h, l = odd
number) have been observed by neutron scattering for the first time. The
intensity of the superlattice reflections is stronger for high scattering
vectors, which is quite different from the usual magnetic form factor of
magnetic dipoles. This result directly evidences that the order parameter of
phase IV has a complex magnetization density, consistent with the recent
experimental and theoretical prediction in which the order parameter is the
magnetic octupoles Tbeta with Gamma5 symmetry of point group Oh. Neutron
scattering experiments using short wavelength neutrons, as done in this study,
could become a general method to study the high-rank multipoles in f electron
systems.Comment: 4 pages, 4 figure
Evidence for Octupole Order in CeLaB from Resonant X-ray Scattering
The azimuthal angle dependence observed in the resonant X-ray scattering in
phase IV of CeLaB is analyzed theoretically. It is shown
that the peculiar angle dependence observed in the E2 channel is consistent
with the Gamma_{5u}-type octupole order with principal axis along (111) and
equivalent directions. Under the assumption that the four equivalent octupole
domains are nearly equally populated in the sample, the observed angle
dependences are reproduced by calculation for both sigma-sigma' and sigma-pi'
polarizations. The calculation for various symmetries of order parameters
excludes unambiguously other order parameters than the Gamma_{5u}-type
octupole.Comment: 4 pages, 2 figures, 3 tables, in JPSJ forma
Invariant Form of Hyperfine Interaction with Multipolar Moments - Observation of Octupolar Moments in NpO and CeB by NMR -
The invariant form of the hyperfine interaction between multipolar moments
and the nuclear spin is derived, and applied to discuss possibilities to
identify the antiferro-octupolar (AFO) moments by NMR experiments. The ordered
phase of NpO and the phase IV of CeLaB are studied in
detail. Recent O NMR for polycrystalline samples of NpO are
discussed theoretically from our formulation. The observed feature of the
splitting of O NMR spectrum into a sharp line and a broad line, their
intensity ratio, and the magnetic field dependence of the shift and of the
width can be consistently explained on the basis of the triple \bq AFO
ordering model proposed by Paix\~{a}o {\it et. al.} Thus, the present theory
shows that the O NMR spectrum gives a strong support to the model. The 4
O sites in the fcc NpO become inequivalent due to the secondary triple
\bq ordering of AF-quadrupoles: one cubic and three non-cubic sites. It turns
out that the hyperfine field due to the antiferro-dipole and AFO moments
induced by the magnetic field, and the quadrupolar field at non-cubic sites are
key ingredients to understand the observed spectrum. The controversial problem
of the nature of phase IV in CeLaB is also studied. It is
pointed out that there is a unique feature in the NMR spectra, if the
() AFO ordering is
realized in CeLaB. Namely, the hyperfine splitting of a B
atom pair on the sites crosses zero on the
plane when the magnetic field is rotated around the axis.Comment: 22 pages, 2 figure
Quadrupolar effect and rattling motion in heavy fermion superconductor PrOs_4Sb_{12}
The elastic properties of a filled skutterudite PrOs_4Sb_{12} with a heavy
Fermion superconductivity at T_C=1.85 K have been investigated. The elastic
softening of (C_{11}-C_{12})/2 and C_{44} with lowering temperature down to T_C
indicates that the quadrupolar fluctuation due to the CEF state plays a role
for the Cooper paring in superconducting phase of PrOs_4Sb_{12}. A Debye-type
dispersion in the elastic constants around 30 K revealed a thermally activated
Gamma_{23} rattling due to the off-center Pr-atom motion obeying
tau=tau_{0}exp(E/k_{B}T) with an attempt time tau_0=8.8*10^{-11} sec and an
activation energy E=168 K. It is remarkable that the charge fluctuation of the
off-center motion with Gamma_{23} symmetry may mix with the quadrupolar
fluctuation and enhance the elastic softening of (C_{11}-C_{12})/2 just above
T_C.Comment: 5 pages, 4 figures, to be published to Phys. Rev.
Spectral Correlation in Incommensurate Multi-Walled Carbon Nanotubes
We investigate the energy spectra of clean incommensurate double-walled
carbon nanotubes, and find that the overall spectral properties are described
by the so-called critical statistics of Anderson metal-insulator transition. In
the energy spectra, there exist three different regimes characterized by
Wigner-Dyson, Poisson, and semi-Poisson distributions. This feature implies
that the electron transport in incommensurate multi-walled nanotubes can be
either diffusive, ballistic, or intermediate between them, depending on the
position of the Fermi energy.Comment: final version to appear in Phys. Rev. Let
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