Symmetry selective third harmonic generation from plasmonic metacrystals

Nonlinear processes are often governed by selection rules imposed by the symmetries of the molecular configurations. The most well-known examples include the role of mirror symmetry breaking for the generation of even harmonics, and the selection rule related to the rotation symmetry in harmonic generation for fundamental beams with circular polarizations. While the role of mirror symmetry breaking in second harmonic generation has been extensively studied in plasmonic systems, the investigation on selection rules pertaining to circular polarization states of harmonic generation has been limited to crystals, i.e. symmetries at the atomic level. Here we demonstrate the rotational symmetry dependent third harmonic generation from nonlinear plasmonic metacrystals. We show that the selection rule can be imposed by the rotational symmetry of meta-crystals embedded into an isotropic organic nonlinear thin film. The results presented here may open new avenues for designing symmetry-dependent nonlinear optical responses with tailored plasmonic nanostructures.Comment: 13 pages, 3 figure

Exploiting dynamic scheduling for VM-based code obfuscation

Code virtualization built upon virtual machine (VM) technologies is emerging as a viable method for implementing code obfuscation to protect programs against unauthorized analysis. State-of-the-art VM-based protection approaches use a fixed scheduling structure where the program follows a single, static execution path for the same input. Such approaches, however, are vulnerable to certain scenarios where the attacker can reuse knowledge extracted from previously seen software to crack applications using similar protection schemes. This paper presents DSVMP, a novel VM-based code obfuscation approach for software protection. DSVMP brings together two techniques to provide stronger code protection than prior VM-based schemes. Firstly, it uses a dynamic instruction scheduler to randomly direct the program to execute different paths without violating the correctness across different runs. By randomly choosing the program execution paths, the application exposes diverse behavior, making it much more difficult for an attacker to reuse the knowledge collected from previous runs or similar applications to perform attacks. Secondly, it employs multiple VMs to further obfuscate the relationship between VM bytecode and their interpreters, making code analysis even harder. We have implemented DSVMP in a prototype system and evaluated it using a set of widely used applications. Experimental results show that DSVMP provides stronger protection with comparable runtime overhead and code size when compared to two commercial VMbased code obfuscation tools

Giant nonlinear optical activity of achiral origin in planar metasurfaces with quadratic and cubic nonlinearities

3D chirality is shown to be unnecessary for introducing strong circular dichroism for harmonic generations. Specifically, near-unity circular dichroism for both second-harmonic generation and third-harmonic generations is demonstrated on suitably designed ultrathin plasmonic metasurfaces with only 2D planar chirality. The study opens up new routes for designing chip-type biosensing platform, which may allow for highly sensitive detection of bio- and chemical molecules with weak chirality

VMGuards:A Novel Virtual Machine Based Code Protection System with VM Security as the First Class Design Concern

Process-level virtual machine (PVM) based code obfuscation is a viable means for protecting software against runtime code tampering and unauthorized code reverse engineering. PVM-based approaches rely on a VM to determine how instructions of the protected code region are scheduled and executed. Therefore, it is crucial to protect the VM against runtime code tampering that alters the instructions and behavior of the VM. This paper presents VMGuards, a novel PVM-based code protection system that puts the security of VM as the first class design concern. Our approach advances prior work by promoting security of the VM as the first class design constraint. We achieve this by introducing two new instruction sets to protect the internal implementations of critical code segments and the host runtime environment where the VM runs in. Our new instruction sets not only have an identical code structure as standard virtual instructions, but also provide additional information to allow the VM to check whether the critical internal implementation or the runtime environment is affected. We evaluate our approach by using a set of real-life applications. Experimental results show that our approach provides stronger and more fine-grained protection when compared to the state-of-the-art with little extra overhead

Third Harmonic Generation Enhanced by Multipolar Interference in Complementary Silicon Metasurfaces

Nonlinear harmonic generation in metasurfaces has shown great promise for applications such as novel light sources, nonlinear holography, and nonlinear imaging. In particular, dielectric metasurfaces have shown multifold enhancement of the harmonic efficiency in comparison to their plasmonic counterparts due to lower optical loss and much higher damage threshold. In this work, we propose to enhance the efficiency of the third harmonic generation in a complementary silicon nonlinear metasurface, consisting of nanoapertures of cross-like shape in the silicon film. The efficiency enhancement is based on a multipolar interference between the magnetic dipole and electric quadrupole, resulting in significant near-field enhancement and a large mode volume of the nonlinear interaction. The measured efficiency of third harmonic generation from the silicon metasurface is 100× higher than that from a planar silicon film of the same thickness. Numerical analysis of the near-field resonant modes confirms the multipolar mechanism of nonlinear enhancement. Enhanced third harmonic generation by multipolar interference in complementary dielectric nanostructure opens a new route for developing high-efficiency nonlinear metasurfaces

Metasurface holograms reaching 80% efficiency

Surfaces covered by ultrathin plasmonic structures—so-called metasurfaces—have recently been shown to be capable of completely controlling the phase of light, representing a new paradigm for the design of innovative optical elements such as ultrathin flat lenses, directional couplers for surface plasmon polaritons and wave plate vortex beam generation. Among the various types of metasurfaces, geometric metasurfaces, which consist of an array of plasmonic nanorods with spatially varying orientations, have shown superior phase control due to the geometric nature of their phase profile. Metasurfaces have recently been used to make computer-generated holograms, but the hologram efficiency remained too low at visible wavelengths for practical purposes. Here, we report the design and realization of a geometric metasurface hologram reaching diffraction efficiencies of 80% at 825 nm and a broad bandwidth between 630 nm and 1,050 nm. The 16-level-phase computer-generated hologram demonstrated here combines the advantages of a geometric metasurface for the superior control of the phase profile and of reflectarrays for achieving high polarization conversion efficiency. Specifically, the design of the hologram integrates a ground metal plane with a geometric metasurface that enhances the conversion efficiency between the two circular polarization states, leading to high diffraction efficiency without complicating the fabrication process. Because of these advantages, our strategy could be viable for various practical holographic applications