Possibilities for Beam Stripping Solutions at a Rare Isotope Accelerator (RIA)

As part of the DOE RIA R&D effort we investigated the possibilities and problems of beam strippers in the different heavy ion accelerator components of a possible Rare Isotope Accelerator (RIA) facility. We focused on two beam stripping positions in the RIA heavy ion driver where benchmark currents of up to 5 particle μA 238-U were projected at energies of 10.5 MeV/u and 85 MeV/u respectively. In order to select feasible stripper materials, data from experiments with Uranium beams at Texas A&M and GSI were evaluated. Based on these results thermal estimates for a possible design were calculated and cooling simulations with commercially available software performed. Additionally, we performed simulations with the GEANT4 code on evaluating the radiation environment for our beam stripping solution at the 85 MeV/u position in the RIA driver

Boron-Rich Benzene and Pyrene Derivatives for the Detection of Thermal Neutrons

A synthetic methodology is developed to generate boron rich aromatic small molecules based on benzene and pyrene moieties for the detection of thermal neutrons. The prepared aromatic compounds have a relatively high boron content up to 7.4 wt%, which is important for application in neutron detection as 10B (20% of natural abundance boron) has a large neutron induced reaction cross-section. This is demonstrated by preparing blends of the synthesized molecules with fluorescent dopants in poly(vinyltoluene) matrices resulting in comparable scintillation light output and neutron capture as state-of-the art commercial scintillators, but with the advantage of much lower cost. The boron-rich benzene and pyrene derivatives are prepared by Suzuki conditions using both microwave and traditional heating, affording yields of 40-93%. This new procedure is simple and straightforward, and has the potential to be scaled up

Status of the LUNA experiment

Luna is a pilot project initially focused on the 3He(3He, 2p)4He cross section measurement within the thermal energy region of the Sun (15–27 keV). A compact high current 50 kV ion accelerator facility including a windowless gas target system, a beam calorimeter and four detector telescopes has been built, tested and installed underground at Laboratori Nazionali del Gran Sasso. In these conditions, thanks to the cosmic ray suppression, we could attain a background level of less than 1 event per week, a rate similar to the one expected from 3He(3He, 2p)4He at the lower edge of the Sun thermal energy region

Charge state studies of low energy heavy ions passing through hydrogen and helium gas

Studies of the charge state distribution of low energy (< 1.5 MeV/u), low Z (< 13) heavy ions passing through hydrogen and helium gas of varying target pressure have been performed using separate windowless gas target systems at TRIUMF and the University of Naples. Semi-empirical relationships have been deduced to estimate the equilibrium charge state distributions as a function of beam energy. From these distributions, cross-sections for the relevant charge changing reactions have been deduced. (C) 2002 Elsevier Science B.V. All rights reserved

Recoil separators for radiative capture using radioactive ion beams

Radiative capture reactions involving the fusion of hydrogen or helium are ubiquitous in the stellar history of the universe, and are some of the most important reactions in the processes that govern nucleosynthesis and energy generation in both static and explosive scenarios. However, radiative capture reactions pose some of the most difficult experimental challenges due to extremely small cross sections. With the advent of recoil separators and techniques in inverse kinematics, it is now possible to measure radiative capture reactions on very short-lived radioactive nuclei, and in the presence of high experimental backgrounds. In this paper we review the experimental needs for making measurements of astrophysical importance on radiative capture reactions. We also review some of the important historical advances in the field of recoil separators as well as describe current techniques and performance milestones, including descriptions of some of the separators most recently working at radioactive ion beam facilities, such as DRAGON at TRIUMF and the DRS at the Holifield Radioactive Ion Beam Facility. We will also summarize some of the scientific highlight measurements at the RIB facilities

Total kinetic energy and fragment mass distributions from fission of Th-232 and U-233

Properties of fission in Th-232 and U-233 were studied at the Los Alamos Neutron Science Center at incident neutron energies from subthermal to 40 MeV. Fission fragments are observed in coincidence using a twin ionization chamber with Frisch grids. The average total kinetic energy released from fission and fragment mass distributions are calculated from observations of energy deposited and conservation of mass and momentum. Accurate experimental measurements of these parameters are necessary to better understand the fission process in isotopes relevant to the thorium fuel cycle, in which Th-232 is used as a fertile material to generate the fissile isotope of U-233. This process mirrors the uranium breeder process used to produce Pu-239 with several potential advantages including the comparative greater abundance of thorium, inherent nuclear weapons proliferation resistance, and reduced actinide production. Thus, there is increased interest in the thorium fuel cycle to meet future energy demands and improve safety and security while increasing profitability for the nuclear power industry. This research is ongoing and preliminary results are presented

Underground nuclear astrophysics studies with CASPAR

The drive of low-energy nuclear astrophysics laboratories is to study the reactions of importance to stellar burning processes and elemental production through stellar nucleosynthesis, over the energy range of astrophysical interest. As laboratory measurements approach the stellar burning window, the rapid drop off of cross-sections is a significant barrier and drives the need to lower background interference. The natural background suppression of underground accelerator facilities enables the extension of current experimental data to lower energies. An example of such reactions of interest are those thought to be sources of neutrons for the s-process, the major production mechanism for elements above the iron peak. The reactions 13C(α,n)16O and 22Ne(α,n)25Mg are the proposed initial focus of the new nuclear astrophysics accelerator laboratory (CASPAR) currently under construction at the Sanford Underground Research Facility, Lead, South Dakot

Underground nuclear astrophysics studies with CASPAR

The drive of low-energy nuclear astrophysics laboratories is to study the reactions of importance to stellar burning processes and elemental production through stellar nucleosynthesis, over the energy range of astrophysical interest. As laboratory measurements approach the stellar burning window, the rapid drop off of cross-sections is a significant barrier and drives the need to lower background interference. The natural background suppression of underground accelerator facilities enables the extension of current experimental data to lower energies. An example of such reactions of interest are those thought to be sources of neutrons for the s-process, the major production mechanism for elements above the iron peak. The reactions 13C(α,n)16O and 22Ne(α,n)25Mg are the proposed initial focus of the new nuclear astrophysics accelerator laboratory (CASPAR) currently under construction at the Sanford Underground Research Facility, Lead, South Dakot

Final Technical Report for DOE Project: Beam Stripping Solutions for RIA Colorado School of Mines Possibilities for Beam Stripping Solutions at a Rare Isotope Accelerator (RIA) Faculty: Uwe. Greife

Executive Summary As part of the DOE RIA R&amp;D effort we investigated the possibilities and problems of beam strippers in the different heavy ion accelerator components of a possible Rare Isotope Accelerator (RIA) facility. We focused on two beam stripping positions in the RIA heavy ion driver where benchmark currents of up to 5 particle µA 238 U were projected at energies of 10.5 MeV/u and 85 MeV/u respectively. In order to select feasible stripper materials, data from experiments with Uranium beams at Texas A&amp;M and GSI were evaluated. Based on these results 3 3 thermal estimates for a possible design were calculated and cooling simulations with commercially available software performed. Additionally, we performed simulations with the GEANT4 code on evaluating the radiation environment for our beam stripping solution at the 85 MeV/u position in the RIA driver