The fate of orbitons coupled to phonons

The key feature of an orbital wave or orbiton is a significant dispersion, which arises from exchange interactions between orbitals on distinct sites. We study the effect of a coupling between orbitons and phonons in one dimension using continuous unitary transformations (CUTs). Already for intermediate values of the coupling, the orbiton band width is strongly reduced and the spectral density is dominated by an orbiton-phonon continuum. However, we find sharp features within the continuum and an orbiton-phonon anti-bound state above. Both show a significant dispersion and should be observable experimentally.Comment: 7 pages, 7 figures; strongly enlarged, comprehensive revised version according to the referees' suggestions, in pres

Spin-Waves in the Mid-Infrared Spectrum of Antiferromagnetic YBa2_2Cu3_3O6.0_{6.0}

The mid-infrared spin-wave spectrum of antiferromagnetic YBa$_2$Cu$_3$O$_{6.0}$\ was determined by infrared transmission and reflection measurements (\bbox{k} \!\! \parallel c) at $T\!=\!10\!$~K.\@ Excitation of single magnons of the optical branch was observed at $E_{\text{op}}\!=\!178.0\!$~meV.\@ Two further peaks at $346\!$~meV ($\approx\!1.94\,E_{\text{op}}$) and $470\!$~meV ($\approx\!2.6\,E_{\text{op}}$) both belong to the two-magnon spectrum. Linear spin wave theory is in good agreement with the measured two-magnon spectrum, and allows to determine the exchange constant $J$ to be about $120\!$~meV, whereas the intrabilayer coupling $J_{12}$ is approximately $0.55\,J$.Comment: 3 figures in uuencoded for

Unifying Magnons and Triplons in Stripe-Ordered Cuprate Superconductors

Based on a two-dimensional model of coupled two-leg spin ladders, we derive a unified picture of recent neutron scattering data of stripe-ordered La_(15/8)Ba_(1/8)CuO_4, namely of the low-energy magnons around the superstructure satellites and of the triplon excitations at higher energies. The resonance peak at the antiferromagnetic wave vector Q_AF in the stripe-ordered phase corresponds to a saddle point in the dispersion of the magnetic excitations. Quantitative agreement with the neutron data is obtained for J= 130-160 meV and J_cyc/J = 0.2-0.25.Comment: 4 pages, 4 figures included updated version taking new data into account; factor in spectral weight corrected; Figs. 2 and 4 change

Mott-Hubbard exciton in the optical conductivity of YTiO3 and SmTiO3

In the Mott-Hubbard insulators YTiO3 and SmTiO3 we study optical excitations from the lower to the upper Hubbard band, d^1d^1 -> d^0d^2. The multi-peak structure observed in the optical conductivity reflects the multiplet structure of the upper Hubbard band in a multi-orbital system. Absorption bands at 2.55 and 4.15 eV in the ferromagnet YTiO3 correspond to final states with a triplet d^2 configuration, whereas a peak at 3.7 eV in the antiferromagnet SmTiO3 is attributed to a singlet d^2 final state. A strongly temperature-dependent peak at 1.95 eV in YTiO3 and 1.8 eV in SmTiO3 is interpreted in terms of a Hubbard exciton, i.e., a charge-neutral (quasi-)bound state of a hole in the lower Hubbard band and a double occupancy in the upper one. The binding to such a Hubbard exciton may arise both due to Coulomb attraction between nearest-neighbor sites and due to a lowering of the kinetic energy in a system with magnetic and/or orbital correlations. Furthermore, we observe anomalies of the spectral weight in the vicinity of the magnetic ordering transitions, both in YTiO3 and SmTiO3. In the G-type antiferromagnet SmTiO3, the sign of the change of the spectral weight at T_N depends on the polarization. This demonstrates that the temperature dependence of the spectral weight is not dominated by the spin-spin correlations, but rather reflects small changes of the orbital occupation.Comment: Strongly extended version; new data of SmTiO3 included; detailed discussion of temperature dependence include

Optical spectroscopy of (La,Ca)14Cu24O41 spin ladders: comparison of experiment and theory

Transmission and reflectivity of La_x Ca_14-x Cu_24 O_41 two-leg spin-1/2 ladders were measured in the mid-infrared regime between 500 and 12000 1/cm. This allows us to determine the optical conductivity sigma_1 directly and with high sensitivity. Here we show data for x=4 and 5 with the electrical field polarized parallel to the rungs (E||a) and to the legs (E||c). Three characteristic peaks are identified as magnetic excitations by comparison with two different theoretical calculations.Comment: 4 pages, 2 figures, submitted to SCES 200

Optical absorption spectra in SrCu_2O_3 two-leg spin ladder

We calculate the phonon-assisted optical-absorption spectra in SrCu_2O_3 two-leg spin-ladder systems. The results for two models proposed for SrCu_2O_3 are compared. In the model including the effects of a cyclic four-spin interaction, the shoulder structure appears at 978 cm^{-1} and the peak appears at 1975 cm^{-1} in the spectrum for polarization of the electric field parallel to the legs. In the other model which describes a pure two-leg ladder, the peak appears around the lower edge of the spectrum at 1344 cm^{-1}. The feature can be effective in determining the proper model for SrCu_2O_3.Comment: 5 pages, 5 figures, to appear in PRB vol. 67 (2003

Group delay in THz spectroscopy with ultra-wideband log-spiral antennae

We report on the group delay observed in continuous-wave terahertz spectroscopy based on photomixing with phase-sensitive homodyne detection. We discuss the different contributions of the experimental setup to the phase difference \Delta\phi(\nu) between transmitter arm and receiver arm. A simple model based on three contributions yields a quantitative description of the overall behavior of \Delta\phi(\nu). Firstly, the optical path-length difference gives rise to a term linear in frequency. Secondly, the ultra-wideband log-spiral antennae effectively radiate and receive in a frequency-dependent active region, which in the most simple model is an annular area with a circumference equal to the wavelength. The corresponding term changes by roughly 6 pi between 100 GHz and 1 THz. The third contribution stems from the photomixer impedance. In contrast, the derivative (d\Delta\phi / d\nu) is dominated by the contribution of periodic modulations of \Delta\phi(\nu) caused by standing waves, e.g., in the photomixers' Si lenses. Furthermore, we discuss the Fourier-transformed spectra, which are equivalent to the waveform in a time-domain experiment. In the time domain, the group delay introduced by the log-spiral antennae gives rise to strongly chirped signals, in which low frequencies are delayed. Correcting for the contributions of antennae and photomixers yields sharp peaks or "pulses" and thus facilitates a time-domain-like analysis of our continuous-wave data.Comment: 7 pages, 7 figure

Optically probing symmetry breaking in the chiral magnet Cu2OSeO3

We report on the linear optical properties of the chiral magnet Cu2OSeO3, specifically associated with the absence of inversion symmetry, the chiral crystallographic structure, and magnetic order. Through spectroscopic ellipsometry, we observe local crystal-field excitations below the charge-transfer gap. These crystal-field excitations are optically allowed due to the lack of inversion symmetry at the Cu sites. Optical polarization rotation measurements were used to study the structural chirality and magnetic order. The temperature dependence of the natural optical rotation, originating in the chiral crystal structure, provides evidence for a finite magneto-electric effect in the helimagnetic phase. We find a large magneto-optical susceptibility on the order of V(540nm)~10^4 rad/(T*m) in the helimagnetic phase and a maximum Faraday rotation of ~165deg/mm in the ferrimagnetic phase. The large value of V can be explained by considering spin cluster formation and the relative ease of domain reorientation in this metamagnetic material. The magneto-optical activity allows us to map the magnetic phase diagram, including the skyrmion lattice phase. In addition to this, we probe and discuss the nature of the various magnetic phase transitions in Cu2OSeO3.Comment: 9 pages, 10 figure

Self-normalizing phase measurement in multimode terahertz spectroscopy based on photomixing of three lasers

Photomixing of two near-infrared lasers is well established for continuous-wave terahertz spectroscopy. Photomixing of three lasers allows us to measure at three terahertz frequencies simultaneously. Similar to Fourier spectroscopy, the spectral information is contained in an nterferogram, which is equivalent to the waveform in time-domain spectroscopy. We use one fixed terahertz frequency \nu_ref to monitor temporal drifts of the setup, i.e., of the optical path-length difference. The other two frequencies are scanned for broadband high-resolution spectroscopy. The frequency dependence of the phase is obtained with high accuracy by normalizing it to the data obtained at \nu_ref, which eliminates drifts of the optical path-length difference. We achieve an accuracy of about 1-2 microns or 10^{-8} of the optical path length. This method is particularly suitable for applications in nonideal environmental conditions outside of an air-conditioned laboratory.Comment: 5 pages, 5 figure