328 research outputs found
Genetic optimization of attosecond-pulse generation in light-field synthesizers
We demonstrate control over attosecond pulse generation and shaping by
numerically optimizing the synthesis of few-cycle to sub-cycle driver
waveforms. The optical waveform synthesis takes place in an ultrabroad spectral
band covering the ultraviolet-infrared domain. These optimized driver waves are
used for ultrashort single and double attosecond pulse production (with tunable
separation) revealing the potentials of the light wave synthesizer device
demonstrated by Wirth et al. [Science 334, 195 (2011)]. The results are also
analyzed with respect to attosecond pulse propagation phenomena
Attosecond control of electrons emitted from a nanoscale metal tip
Attosecond science is based on steering of electrons with the electric field
of well-controlled femtosecond laser pulses. It has led to, for example, the
generation of XUV light pulses with a duration in the sub-100-attosecond
regime, to the measurement of intra-molecular dynamics by diffraction of an
electron taken from the molecule under scrutiny, and to novel ultrafast
electron holography. All these effects have been observed with atoms or
molecules in the gas phase. Although predicted to occur, a strong light-phase
sensitivity of electrons liberated by few-cycle laser pulses from solids has
hitherto been elusive. Here we show a carrier-envelope (C-E) phase-dependent
current modulation of up to 100% recorded in spectra of electrons laser-emitted
from a nanometric tungsten tip. Controlled by the C-E phase, electrons
originate from either one or two sub-500as long instances within the 6-fs laser
pulse, leading to the presence or absence of spectral interference. We also
show that coherent elastic re-scattering of liberated electrons takes place at
the metal surface. Due to field enhancement at the tip, a simple laser
oscillator suffices to reach the required peak electric field strengths,
allowing attosecond science experiments to be performed at the 100-Megahertz
repetition rate level and rendering complex amplified laser systems
dispensable. Practically, this work represents a simple, exquisitely sensitive
C-E phase sensor device, which can be shrunk in volume down to ~ 1cm3. The
results indicate that the above-mentioned novel attosecond science techniques
developed with and for atoms and molecules can also be employed with solids. In
particular, we foresee sub-femtosecond (sub-) nanometre probing of (collective)
electron dynamics, such as plasmon polaritons, in solid-state systems ranging
in size from mesoscopic solids via clusters to single protruding atoms.Comment: Final manuscript version submitted to Natur
Carrier-envelope phase effects on the strong-field photoemission of electrons from metallic nanostructures
Sharp metallic nanotapers irradiated with few-cycle laser pulses are emerging
as a source of highly confined coherent electron wavepackets with attosecond
duration and strong directivity. The possibility to steer, control or switch
such electron wavepackets by light is expected to pave the way towards direct
visualization of nanoplasmonic field dynamics and real-time probing of electron
motion in solid state nanostructures. Such pulses can be generated by
strong-field induced tunneling and acceleration of electrons in the near-field
of sharp gold tapers within one half-cycle of the driving laser field. Here, we
show the effect of the carrier-envelope phase of the laser field on the
generation and motion of strong-field emitted electrons from such tips. This is
a step forward towards controlling the coherent electron motion in and around
metallic nanostructures on ultrashort length and time scales
The direct evaluation of attosecond chirp from a streaking measurement
We derive an analytical expression, from classical electron trajectories in a
laser field, that relates the breadth of a streaked photoelectron spectrum to
the group-delay dispersion of an isolated attosecond pulse. Based on this
analytical expression, we introduce a simple, efficient and robust procedure to
instantly extract the attosecond pulse's chirp from the streaking measurement.Comment: 4 figure
Two-color ionization of hydrogen by short intense pulses
Photoelectron energy spectra resulting by the interaction of hydrogen with
two short pulses having carrier frequencies, respectively, in the range of the
infrared and XUV regions have been calculated. The effects of the pulse
duration and timing of the X-ray pulse on the photoelectron energy spectra are
discussed. Analysis of the spectra obtained for very long pulses show that
certain features may be explained in terms of quantum interferences in the time
domain. It is found that, depending on the duration of the X-ray pulse, ripples
in the energy spectra separated by the infrared photon energy may appear.
Moreover, the temporal shape of the low frequency radiation field may be
inferred by the breadth of the photoelectron energy spectra.Comment: 12 pages, 8 figure
Attosecond double-slit experiment
A new scheme for a double-slit experiment in the time domain is presented.
Phase-stabilized few-cycle laser pulses open one to two windows (``slits'') of
attosecond duration for photoionization. Fringes in the angle-resolved energy
spectrum of varying visibility depending on the degree of which-way information
are observed. A situation in which one and the same electron encounters a
single and a double slit at the same time is discussed. The investigation of
the fringes makes possible interferometry on the attosecond time scale. The
number of visible fringes, for example, indicates that the slits are extended
over about 500as.Comment: 4 figure
Giant half-cycle attosecond pulses
Half-cycle picosecond pulses have been produced from thin photo-conductors,
when applying an electric field across the surface and switching on conduction
by a short laser pulse. Then the transverse current in the wafer plane emits
half-cycle pulses in normal direction, and pulses of 500 fs duration and 1e6
V/m peak electric field have been observed. Here we show that single half-cycle
pulses of 50 as duration and up to 1e13 V/m can be produced when irradiating a
double foil target by intense few-cycle laser pulses. Focused onto an
ultra-thin foil, all electrons are blown out, forming a uniform sheet of
relativistic electrons. A second layer, placed at some distance behind,
reflects the drive beam, but lets electrons pass straight. Under oblique
incidence, beam reflection provides the transverse current, which emits intense
half-cycle pulses. Such a pulse may completely ionize even heavier atoms. New
types of attosecond pump-probe experiments will become possible.Comment: 5 pages, 4 figures, to be presented at LEI2011-Light at Extreme
Intensities and China-Germany Symposium on Laser Acceleratio
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