Hyperfine quenching of the metastable 3P0,2^3P_{0,2} states in divalent atoms

Hyperfine quenching rates of the lowest-energy metastable $^3P_0$ and $^3P_2$ states of Mg, Ca, Sr, and Yb atoms are computed. The calculations are carried out using ab initio relativistic many-body methods. The computed lifetimes may be useful for designing novel ultra-precise optical clocks and trapping experiments with the $3P_2$ fermionic isotopes. The resulting natural widths of the $^3P_0 -> ^1S_0$ clock transition are 0.44 mHz for $^{25}$Mg, 2.2 mHz for $^{43}$Ca, 7.6 mHz for $^{87}$Sr, 43.5 mHz for $^{171}$Yb, and 38.5 mHz for $^{173}$Yb. Compared to the bosonic isotopes, the lifetime of the $3P_2$ states in fermionic isotopes is noticeably shortened by the hyperfine quenching but still remains long enough for trapping experiments.Comment: 10 pages, 1 figure, submitted to Phys. Rev.

On the feasibility of cooling and trapping metastable alkaline-earth atoms

Metastability and long-range interactions of Mg, Ca, and Sr in the lowest-energy metastable $^3P_2$ state are investigated. The calculated lifetimes are 38 minutes for Mg*, 118 minutes for Ca*, and 17 minutes for Sr*, supporting feasibility of cooling and trapping experiments. The quadrupole-quadrupole long-range interactions of two metastable atoms are evaluated for various molecular symmetries. Hund's case (c) 4_g potential possesses a large 100-1000 K potential barrier. Therefore magnetic trap losses can possibly be reduced using cold metastable atoms in a stretched M=2 state. Calculations were performed in the framework of ab initio relativistic configuration interaction method coupled with the random-phase approximation.Comment: 8 pages, 2 figures; to appear in PR

Multiconfiguration Dirac-Hartree-Fock energy levels and transition probabilities for 3d^5 in Fe IV

Multiconfiguration Dirac-Hartree-Fock electric quadrupole (E2) and magnetic dipole (M1) transition probabilities are reported for transitions between levels of 3d^5 in [Fe IV]. The accuracy of the ab initio energy levels and the agreement in the length and velocity forms of the line strength for the E2 transitions are used as indicators of accuracy. The present E2 and M1 transition probabilities are compared with earlier Breit-Pauli results and other theories. An extensive set of transition probabilites with indicators of accuracy are reported in Appendices A and B. Recommended values of A(E2) + A(M1) are listed in Appendix C.Comment: 16 pages, three appendices containing accuracy indicators and recommended values for E2 and M1 transition rate

Comments on ``The first detections of the Extragalactic Background Light at 3000, 5500, and 8000 A'' by Bernstein, Freedman and Madore

A critical discussion is presented of the data analysis applied by Bernstein, Freedman and Madore (2002 ApJ, 571, 56; and ApJ 571, 85) in their measurement of the Extragalactic Background Light. There are questionable assumptions in the analysis of the ground-based observations of the Zodiacal Light. The modeling of the Diffuse Galactic Light is based on an underestimated value of the dust column density along the line of sight. Comparison with the previously presented results from the same observations reveals a puzzling situation: in spite of a large difference in the atmospheric scattered light corrections the derived Extragalactic Background Light values are exactly the same. The claim of the paper of a ``detection of the Extragalactic Background Light'' appears premature.Comment: 6 pages, accepted for Ap

Properties of metastable alkaline-earth-metal atoms calculated using an accurate effective core potential

The first three electronically excited states in the alkaline-earth-metal atoms magnesium, calcium, and strontium comprise the (nsnp) triplet P^o_J (J=0,1,2) fine-structure manifold. All three states are metastable and are of interest for optical atomic clocks as well as for cold-collision physics. An efficient technique--based on a physically motivated potential that models the presence of the ionic core--is employed to solve the Schroedinger equation for the two-electron valence shell. In this way, radiative lifetimes, laser-induced clock shifts, and long-range interaction parameters are calculated for metastable Mg, Ca, and Sr.Comment: 13 pages, 9 table

The FERRUM project: Transition probabilities for forbidden lines in [FeII] and experimental metastable lifetimes

Accurate transition probabilities for forbidden lines are important diagnostic parameters for low-density astrophysical plasmas. In this paper we present experimental atomic data for forbidden [FeII] transitions that are observed as strong features in astrophysical spectra. Aims: To measure lifetimes for the 3d^6(^3G)4s a ^4G_{11/2} and 3d^6(^3D)4s b ^4D_{1/2} metastable levels in FeII and experimental transition probabilities for the forbidden transitions 3d^7 a ^4F_{7/2,9/2}- 3d^6(^3G)4s a ^4G_{11/2}. Methods: The lifetimes were measured at the ion storage ring facility CRYRING using a laser probing technique. Astrophysical branching fractions were obtained from spectra of Eta Carinae, obtained with the Space Telescope Imaging Spectrograph onboard the Hubble Space Telescope. The lifetimes and branching fractions were combined to yield absolute transition probabilities. Results: The lifetimes of the a ^4G_{11/2} and the b ^4D_{1/2} levels have been measured and have the following values, 0.75(10) s and 0.54(3) s respectively. Furthermore, we have determined the transition probabilities for two forbidden transitions of a ^4F_{7/2,9/2}- a ^4G_{11/2} at 4243.97 and 4346.85 A. Both the lifetimes and the transition probabilities are compared to calculated values in the literature.Comment: 5 pages, accepted for publication in A&

Optical and near infrared observations of SN 1998bu

Infrared and optical spectra of SN 1998bu at an age of one year after explosion are presented. The data show evidence for the radioactive decay of 56Co to 56Fe, long assumed to be the powering source for the supernova light curve past maximum light. The spectra provide direct evidence for at least 0.4 solar masses of iron being present in the ejecta of the supernova. The fits to the data also show that the widths of the emission lines increase with time. Photometric measurements in the H-band show that the supernova is not fading during the observation period. This is consistent with theoretical expectations.Comment: accepted A&A, 7 pages, 9 figure

Ionization Structure and Spectra of Iron in Gaseous Nebulae}

The emission spectra and the ionization structure of the low ionization stages of iron, Fe I--IV, in gaseous nebulae are studied. This work includes: (i) new atomic data: photoionization cross sections, total e-ion recombination rates, excitation collision strengths, and transition probabilities; (ii) detailed study of excitation mechanisms for the [Fe II], [Fe III], and [Fe IV] emission, and spectroscopic analysis of the observed IR, optical, and UV spectra; (iii) study of the physical structure and kinematics of the nebulae and their ionization fronts. Spectral analysis of the well observed Orion nebula is carried out as a test case, using extensive collisional-radiative and photoionization models. It is shown that the [Fe II] emission from the Orion nebula is predominantly excited via electron collisions in high density partially ionized zones; radiative fluorescence is relatively less effective. Further evidence for high density zones is derived from the [O I] and [Ni II] spectral lines, as well as from the kinematic measurements of ionic species in the nebula. The ionization structure of iron in Orion is modeled using the newly calculated atomic data, showing some significant differences from previous models. The new model suggests a fully ionized H II region at densities on the order of $10^3$ cm$^{-3}$, and a dynamic partially ionized H II/H I region at densities of $10^5-10^7$ \cm3. Photoionization models also indicate that the optical [O I] and [Fe II] emission originates in high density partially ionized regions within ionization fronts. The gas phase iron abundance in Orion is estimated from observed spectra.Comment: AAS LaTex, 60 pages 18 figures. Astrophysical Journal. in pres

[Fe IV] emission in ionized nebulae

This paper presents an analysis of [Fe IV] emission based on new identifications and previous measurements of [Fe IV] lines in 30 Doradus, IC 4846, M42, SMC N88A, and SBS 0335-052. The Fe abundances obtained by adding the abundances of the relevant Fe ions (mainly Fe^{++} and Fe^{3+}) are found to be lower, by factors in the range 2.6-5.9, than the Fe abundances implied by [Fe III] emission and an ionization correction factor derived from ionization models. The most likely explanation of this discrepancy is that either the collision strengths for [Fe IV] or the Fe ionization fractions predicted by models are unreliable. The available data neither allow one to distinguish between these two possibilities nor to exclude another possible explanation: that the discrepancy implies the presence of a gradient in the Fe abundance within the ionized gas. Further measurements of [Fe IV] lines and checks on the Fe^{3+} atomic data and ionization models are needed to reach a definitive conclusion. The discrepancy introduces an uncertainty in the determination of Fe abundances in ionized nebulae. This uncertainty has implications for our understanding of both the evolution of dust in ionized nebulae and the chemical history of low metallicity galaxies.Comment: 23 pages, 3 figures, accepted for publication in ApJ, a new table and several comments adde

Late Spectral Evolution of SN 1987A: I. Temperature and Ionization

The temperature and ionization of SN 1987A is modeled between 200 and 2000 days in its nebular phase, using a time-dependent model. We include all important elements, as well as the primary composition zones in the supernova. The energy input is provided by radioactive decay of Co-56, Co-57, and Ti-44. The thermalization of the resulting gamma-rays and positrons is calculated by solving the Spencer-Fano equation. Both the ionization and the individual level populations are calculated time-dependently. Adiabatic cooling is included in the energy equation. Charge transfer is important for determining the ionization and is included with available and estimated rates. Full, multilevel atoms are used for the observationally important ions. As input models to the calculations we use explosion models for SN 1987A calculated by Woosley et al and Nomoto et al. The most important result in this paper refers to the evolution of the temperature and ionization of the various abundance zones. The metal-rich core undergoes a thermal instability, often referred to as the IR-catastrophe, at 600 - 1000 days. The hydrogen-rich zones evolve adiabatically after 500 - 800 days, while in the helium region both adiabatic cooling and line cooling are of equal importance after ~1000 days. Freeze-out of the recombination is important in the hydrogen and helium zones. Concomitant with the IR-catastrophe, the bulk of the emission shifts from optical and near-IR lines to the mid- and far-IR. After the IR-catastrophe, the cooling is mainly due to far-IR lines and adiabatic expansion. Dust cooling is likely to be important in the zones where dust forms. We find that the dust condensation temperatures occur later than ~500 days in the oxygen-rich zones, and the most favorable zone for dust condensation is the iron core.Comment: 53 pages, including 10 figures; ApJ (Main Journal); scheduled for April 1, 1998, Vol. 49