Crystal growth and in-plane optical properties of Tl2_2Ba2_2Can−1_{n-1}Cun_nOx_x (n=1,2,3) superconductors

Single crystals of thallium-based cuprates with the general formula Tl$_{2}$Ba$_{2}$Ca$_{n-1}$Cu$_{n}$O$_{x}$(n=1,2,3) have been grown by the flux method. The superconducting transition temperatures determined by the ac magnetic susceptibility are 92 K, 109 K, and 119 K for n=1,2,3 respectively. X-ray diffraction measurements and EDX compositional analysis were described. We measured in-plane optical reflectance from room temperature down to 10 K, placing emphasis on Tl-2223. The reflectance roughly has a linear-frequency dependence above superconducting transition temperature, but displays a pronounced knee structure together with a dip-like feature at higher frequency below T$_c$. Correspondingly, the ratio of the reflectances below and above T$_{c}$ displays a maximum and a minimum near those feature frequencies. In particular, those features in Tl2223 appear at higher energy scale than Tl2212, and Tl2201. The optical data are analyzed in terms of spectral function. We discussed the physical consequences of the data in terms of both clean and dirty limit.Comment: 8 pages, 13 figures, to be published in Phys. Rev.

Magnetic transitions in CaMn7O12 : a Raman observation of spin-phonon couplings

The quadruple Calcium manganite (CaMn7O12) is a multiferroic material that exhibits a giant magnetically-induced ferroelectric polarization which makes it very interesting for magnetoelectric applications. Here, we report the Raman spectroscopy study on this compound of both the phonon modes and the low energy excitations from 4 K to room temperature. A detailed study of the Raman active phonon excitations shows that three phonon modes evidence a spin-phonon coupling at TN2 = 50 K. In particular, we show that the mode at 432 cm-1 associated to Mn(B)O6 (B position of the perovskite) rotations around the [111] cubic diagonal is impacted by the magnetic transition at 50 K and its coupling to the new modulation of the Mn spin in the (a,b) plane. At low energies, two large low energy excitations are observed at 25 and 47 cm-1. The first one disappears at 50 K and the second one at 90 K. We have associated these excitations to electro-magneto-active modes

η\eta collective mode as A1g_{1g} Raman resonance in cuprate superconductors

We discuss the possible existence a spin singlet excitation with charge $\pm2$ ($\eta$-mode) originating the $A_{1g}$ Raman resonance in cuprate superconductors. This $\eta$-mode relates the $d$-wave superconducting singlet pairing channel to a $d$-wave charge channel. We show that the $\eta$ boson forms a particle-particle bound state below the $2\Delta$ threshold of the particle-hole continuum where $\Delta$ is the maximum $d$-wave gap. Within a generalized random phase approximation and Bethe-Salpether approximation study, we find that this mode has energies similar to the resonance observed by Inelastic Neutron Scattering (INS) below the superconducting (SC) coherent peak at $2\Delta$ in various SC cuprates compounds. We show that it is a very good candidate for the resonance observed in Raman scattering below the $2\Delta$ peak in the $A_{1g}$ symmetry. Since the $\eta$-mode sits in the $S=0$ channel, it may be observable via Raman, X -ray or Electron Energy Loss Spectroscopy probes

Extended mid-infrared emission from VV 114: probing the birth of a ULIRG

We present our 5-16 micron spectro-imaging observations of VV114, an infrared luminous early-stage merger, taken with the ISOCAM camera on-board ISO. We find that only 40% of the mid-infrared (MIR) flux is associated with a compact nuclear region, while the rest of the emission originates from a rather diffuse component extended over several kpc. This is in stark contrast with the very compact MIR starbursts usually seen in luminous infrared galaxies. A secondary peak of MIR emission is associated with an extra-nuclear star forming region which displays the largest Halpha equivalent width in the whole system. Comparing our data with the distribution of the molecular gas and cold dust, as well as with radio observations, it becomes evident that the conversion of molecular gas into stars can be triggered over large areas at the very first stages of an interaction. The presence of a very strong continuum at 5 microns in one of the sources indicates that an enshrouded active galactic nucleus may contribute to 40% of its MIR flux. We finally note that the relative variations in the UV to radio spectral properties between the merging galaxies provide evidence that the extinction-corrected star formation rate of similar objects at high z, such as those detected in optical deep surveys, can not be accurately derived from their rest-frame UV properties.Comment: 14 pages, 5 figures, accepted for publication in A&

Transition from Free to Interacting Composite Fermions away from ν\nu=1/3

Spin excitations from a partially populated composite fermion level are studied above and below $\nu=1/3$. In the range $2/7<\nu<2/5$ the experiments uncover significant departures from the non-interacting composite fermion picture that demonstrate the increasing impact of interactions as quasiparticle Landau levels are filled. The observed onset of a transition from free to interacting composite fermions could be linked to condensation into the higher order states suggested by transport experiments and numerical evaluations performed in the same filling factor range.Comment: 4 pages, 5 figures, to appear in PR

Mid-infrared observations of the ultraluminous galaxies IRAS14348-1447, IRAS19254-7245, and IRAS23128-5919

We present a study of the three ultraluminous infrared galaxies IRAS14348-1447, IRAS19254-7245, and IRAS23128-5919, based on mid-infrared (MIR) spectro-imaging (5-18microns) observations performed with ISOCAM. We find that the MIR emission from each system, which consists of a pair of interacting late type galaxies, is principally confined to the nuclear regions with diameters of 1-2kpc and can account for more than 95% of their IRAS 12micron flux. In each interacting system, the galaxy hosting an active galactic nucleus (AGN) dominates the total spectrum and shows stronger dust continuum (12-16microns) relative to the Unidentified Infrared Band (UIB) emission (6-9microns), suggestive of its enhanced radiation field. The MIR dominant galaxy also exhibits elevated 15micron/Halpha and 15micron/K ratios which trace the high extinction due to the large quantities of molecular gas and dust present in its central regions. Using only diagnostics based on our mid-infrared spectra, we can establish that the Seyfert galaxy IRAS19254-7245 exhibits MIR spectral features of an AGN while the MIR spectrum of the Seyfert (or LINER) member of IRAS23128-5919 is characteristic of dust emission principally heated by star forming regions.Comment: Accepted for publication in Astronomy & Astrophysics, 13 pages, 9 figure