3,677 research outputs found

    Madelung potentials and covalency effect in strained La1x_{1-x}Srx_xMnO3_3 thin films studied by core-level photoemission spectroscopy

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    We have investigated the shifts of the core-level photoemission spectra of La0.6_{0.6}Sr0.4_{0.4}MnO3_3 thin films grown on three kinds of substrates, SrTiO3_3, (LaAlO3_3)0.3_{0.3}-(SrAl0.5_{0.5}Ta0.5_{0.5}O3_3)0.7_{0.7}, and LaAlO3_3. The experimental shifts of the La 4d and Sr 3d core levels are almost the same as the calculation, which we attribute to the absence of covalency effects on the Madelung potentials at these atomic sites due to the nearly ionic character of these atoms. On the other hand, the experimental shifts of the O 1s1s and Mn 2p2p core levels are negligibly small, in disagreement with the calculation. We consider that this is due to the strong covalent character of the Mn-O bonds.Comment: 4 pages, 5 figure

    A two dimensional model for ferromagnetic martensites

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    We consider a recently introduced 2-D square-to-rectangle martensite model that explains several unusual features of martensites to study ferromagnetic martensites. The strain order parameter is coupled to the magnetic order parameter through a 4-state clock model. Studies are carried out for several combinations of the ordering of the Curie temperatures of the austenite and martensite phases and, the martensite transformation temperature. We find that the orientation of the magnetic order which generally points along the short axis of the rectangular variant, changes as one crosses the twin or the martensite-austenite interface. The model shows the possibility of a subtle interplay between the growth of strain and magnetic order parameters as the temperature is decreased. In some cases, this leads to qualitatively different magnetization curves from those predicted by earlier mean field models. Further, we find that strain morphology can be substantially altered by the magnetic order. We have also studied the dynamic hysteresis behavior. The corresponding dissipation during the forward and reverse cycles has features similar to the Barkhausen's noise.Comment: 9 pages, 11 figure

    Effect of strong localization of doped holes in angle-resolved photoemission spectra of La1x_{1-x}Srx_xFeO3_3

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    We have performed an angle-resolved photoemission spectroscopy study of La0.6_{0.6}Sr0.4_{0.4}FeO3_3 using {\it in situ} prepared thin films and determined its band structure. The experimental band dispersions could be well explained by an empirical band structure assuming the G-type antiferromagnetic state. However, the Fe 3d bands were found to be shifted downward relative to the Fermi level (EFE_F) by 1\sim 1 eV compared with the calculation and to form a (pseudo)gap of 1\sim 1 eV at EFE_F. We attribute this observation to a strong localization effect of doped holes due to polaron formation.Comment: 5 pages, 5 figure

    Depth profile photoemission study of thermally diffused Mn/GaAs (001) interfaces

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    We have performed a depth profile study of thermally diffused Mn/GaAs (001) interfaces using photoemission spectroscopy combined with Ar+^+-ion sputtering. We found that Mn ion was thermally diffused into the deep region of the GaAs substrate and completely reacted with GaAs. In the deep region, the Mn 2pp core-level and Mn 3dd valence-band spectra of the Mn/GaAs (001) sample heated to 600 ^{\circ}C were similar to those of Ga1x_{1-x}Mnx_xAs, zinc-blende-type MnAs dots, and/or interstitial Mn in tetrahedrally coordinated by As atoms, suggesting that the Mn 3dd states were essentially localized but were hybridized with the electronic states of the host GaAs. Ferromagnetism was observed in the dilute Mn phase.Comment: 5 pages, 4 figure

    Simulations of Spinodal Nucleation in Systems with Elastic Interactions

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    Systems with long-range interactions quenched into a metastable state near the pseudospinodal exhibit nucleation that is qualitatively different than the classical nucleation observed near the coexistence curve. We have observed nucleation droplets in our Langevin simulations of a two-dimensional model of martensitic transformations and have determined that the structure of the nucleating droplet differs from the stable martensite structure. Our results, together with experimental measurements of the phonon dispersion curve, allow us to predict the nature of the droplet. These results have implications for nucleation in many solid-solid transitions and the structure of the final state

    Linear approach to the orbiting spacecraft thermal problem

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    We develop a linear method for solving the nonlinear differential equations of a lumped-parameter thermal model of a spacecraft moving in a closed orbit. Our method, based on perturbation theory, is compared with heuristic linearizations of the same equations. The essential feature of the linear approach is that it provides a decomposition in thermal modes, like the decomposition of mechanical vibrations in normal modes. The stationary periodic solution of the linear equations can be alternately expressed as an explicit integral or as a Fourier series. We apply our method to a minimal thermal model of a satellite with ten isothermal parts (nodes) and we compare the method with direct numerical integration of the nonlinear equations. We briefly study the computational complexity of our method for general thermal models of orbiting spacecraft and conclude that it is certainly useful for reduced models and conceptual design but it can also be more efficient than the direct integration of the equations for large models. The results of the Fourier series computations for the ten-node satellite model show that the periodic solution at the second perturbative order is sufficiently accurate.Comment: 20 pages, 11 figures, accepted in Journal of Thermophysics and Heat Transfe

    Tweed in Martensites: A Potential New Spin Glass

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    We've been studying the ``tweed'' precursors above the martensitic transition in shape--memory alloys. These characteristic cross--hatched modulations occur for hundreds of degrees above the first--order shape--changing transition. Our two--dimensional model for this transition, in the limit of infinite elastic anisotropy, can be mapped onto a spin--glass Hamiltonian in a random field. We suggest that the tweed precursors are a direct analogy of the spin--glass phase. The tweed is intermediate between the high--temperature cubic phase and the low--temperature martensitic phase in the same way as the spin--glass phase can be intermediate between ferromagnet and antiferromagnet.Comment: 18 pages and four figures (included

    Resonant electron transmission through a finite quantum spin chain

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    Electron transport in a finite one dimensional quantum spin chain (with ferromagnetic exchange) is studied within an sds-d exchange Hamiltonian. Spin transfer coefficients strongly depend on the sign of the sds-d exchange constant. For a ferromagnetic coupling, they exhibit a novel resonant pattern, reflecting the salient features of the combined electron-spin system. Spin-flip processes are inelastic and feasible at finite voltage or at finite temperature.Comment: 4 pages including 4 .eps figure
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