1,303 research outputs found
Static and Dynamic Magnetism in Underdoped Superconductor BaFeCoAs
We report neutron scattering measurements on single crystals of
BaFeCoAs. The magnetic Bragg peak intensity is reduced by
6 % upon cooling through T. The spin dynamics exhibit a gap of 8 meV with
anisotropic three-dimensional (3d) interactions. Below T additional
intensity appears at an energy of 4.5(0.5) meV similar to previous
observations of a spin resonance in other Fe-based superconductors. No further
gapping of the spin excitations is observed below T for energies down to 2
meV. These observations suggest the redistribution of spectral weight from the
magnetic Bragg position to a spin resonance demonstrating the direct
competition between static magnetic order and superconductivity.Comment: 4 pages, 4 figure
Revisiting the ground state of CoAlO: comparison to the conventional antiferromagnet MnAlO
The A-site spinel material, CoAl2O4, is a physical realization of the
frustrated diamond-lattice antiferromagnet, a model in which is predicted to
contain unique incommensurate or `spin-spiral liquid' ground states. Our
previous single-crystal neutron scattering study instead classified it as a
`kinetically-inhibited' antiferromagnet, where the long ranged correlations of
a collinear Neel ground state are blocked by the freezing of domain wall motion
below a first-order phase transition at T* = 6.5 K. The current paper expands
on our original results in several important ways. New elastic and inelastic
neutron measurements are presented that show our initial conclusions are
affected by neither the sample measured nor the instrument resolution, while
measurements to temperatures as low as T = 250 mK limit the possible role being
played by low-lying thermal excitations. Polarized diffuse neutron measurements
confirm reports of short-range antiferromagnetic correlations and diffuse
streaks of scattering, but major diffuse features are explained as signatures
of overlapping critical correlations between neighboring Brillouin zones.
Finally, and critically, this paper presents detailed elastic and inelastic
measurements of magnetic correlations in a single-crystal of MnAl2O4, which
acts as an unfrustrated analogue to CoAl2O4. The unfrustrated material is shown
to have a classical continuous phase transition to Neel order at T_N = 39 K,
with collective spinwave excitations and Lorentzian-like critical correlations
which diverge at the transition. Direct comparison between the two compounds
indicates that CoAl2O4 is unique, not in the nature of high-temperature diffuse
correlations, but rather in the nature of the frozen state below T*. The higher
level of cation inversion in the MnAl2O4 sample indicates that this novel
behavior is primarily an effect of greater next-nearest-neighbor exchange.Comment: 13 pages, 8 figures, acccepted for publication in Physical Review
Kinetically Inhibited Order in a Diamond-Lattice Antiferromagnet
Frustrated magnetic systems exhibit highly degenerate ground states and
strong fluctuations, often leading to new physics. An intriguing example of
current interest is the antiferromagnet on a diamond lattice, realized
physically in A-site spinel materials. This is a prototypical system in three
dimensions where frustration arises from competing interactions rather than
purely geometric constraints, and theory suggests the possibility of unusual
magnetic order at low temperature. Here we present a comprehensive
single-crystal neutron scattering study of CoAl2O4, a highly frustrated A-site
spinel. We observe strong diffuse scattering that peaks at wavevectors
associated with Neel ordering. Below the temperature T*=6.5 K, there is a
dramatic change in the elastic scattering lineshape accompanied by the
emergence of well-defined spin-wave excitations. T* had previously been
associated with the onset of glassy behavior. Our new results suggest instead
that T* signifies a first-order phase transition, but with true long-range
order inhibited by the kinetic freezing of domain walls. This scenario might be
expected to occur widely in frustrated systems containing first-order phase
transitions and is a natural explanation for existing reports of anomalous
glassy behavior in other materials.Comment: 40 pages, 9 figures, Introduction and discussion altered and
expanded. Additional section and figure added to Supplementary Informatio
Structural contributions to the pressure-tuned charge-density-wave to superconductor transition in ZrTe3: Raman scattering studies
Superconductivity evolves as functions of pressure or doping from
charge-ordered phases in a variety of strongly correlated systems, suggesting
that there may be universal characteristics associated with the competition
between superconductivity and charge order in these materials. We present an
inelastic light (Raman) scattering study of the structural changes that precede
the pressure-tuned charge-density-wave (CDW) to superconductor transition in
one such system, ZrTe3. In certain phonon bands, we observe dramatic linewidth
reductions that accompany CDW formation, indicating that these phonons couple
strongly to the electronic degrees of freedom associated with the CDW. The same
phonon bands, which represent internal vibrations of ZrTe3 prismatic chains,
are suppressed at pressures above ~10 kbar, indicating a loss of long-range
order within the chains, specifically amongst intrachain Zr-Te bonds. These
results suggest a distinct structural mechanism for the observed
pressure-induced suppression of CDW formation and provide insights into the
origin of pressure-induced superconductivity in ZrTe3.Comment: 6 pages, 5 figure
Surface collective modes in the topological insulators BiSe and BiSbTeSe
We used low-energy, momentum-resolved inelastic electron scattering to study
surface collective modes of the three-dimensional topological insulators
BiSe and BiSbTeSe. Our goal was to
identify the "spin plasmon" predicted by Raghu and co-workers [S. Raghu, et
al., Phys. Rev. Lett. 104, 116401 (2010)]. Instead, we found that the primary
collective mode is a surface plasmon arising from the bulk, free carrers in
these materials. This excitation dominates the spectral weight in the bosonic
function of the surface, , at THz energy scales, and
is the most likely origin of a quasiparticle dispersion kink observed in
previous photoemission experiments. Our study suggests that the spin plasmon
may mix with this other surface mode, calling for a more nuanced understanding
of optical experiments in which the spin plasmon is reported to play a role.Comment: 5 pages, 4 figure
Observations of polar patches generated by solar wind Alfvén wave coupling to the dayside magnetosphere
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