4,548 research outputs found

    Toolboxes and handing students a hammer: The effects of cueing and instruction on getting students to think critically

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    Developing critical thinking skills is a common goal of an undergraduate physics curriculum. How do students make sense of evidence and what do they do with it? In this study, we evaluated students' critical thinking behaviors through their written notebooks in an introductory physics laboratory course. We compared student behaviors in the Structured Quantitative Inquiry Labs (SQILabs) curriculum to a control group and evaluated the fragility of these behaviors through procedural cueing. We found that the SQILabs were generally effective at improving the quality of students' reasoning about data and making decisions from data. These improvements in reasoning and sensemaking were thwarted, however, by a procedural cue. We describe these changes in behavior through the lens of epistemological frames and task orientation, invoked by the instructional moves

    Shear Thickening of Dense Suspensions: The Role of Friction

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    Shear thickening of particle suspensions is characterized by a transition between lubricated and frictional contacts between the particles. Using 3D numerical simulations, we study how the inter-particle friction coefficient influences the effective macroscopic friction coefficient and hence the microstructure and rheology of dense shear thickening suspensions. We propose expressions for effective friction coefficient in terms of distance to jamming for varying shear stresses and particle friction coefficient values. We find effective friction coefficient to be rather insensitive to interparticle friction, which is perhaps surprising but agrees with recent theory and experiments

    On the origin of the extremely different solubilities of polyethers in water

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    The solubilities of polyethers are surprisingly counter-intuitive. The best-known example is the difference between polyethylene glycol ([–CH2–CH2–O–]n) which is infinitely soluble, and polyoxymethylene ([–CH2–O–]n) which is completely insoluble in water, exactly the opposite of what one expects from the C/O ratios of these molecules. Similar anomalies exist for oligomeric and cyclic polyethers. To solve this apparent mystery, we use femtosecond vibrational and GHz dielectric spectroscopy with complementary ab initio calculations and molecular dynamics simulations. We find that the dynamics of water molecules solvating polyethers is fundamentally different depending on their C/O composition. The ab initio calculations and simulations show that this is not because of steric effects (as is commonly believed), but because the partial charge on the O atoms depends on the number of C atoms by which they are separated. Our results thus show that inductive effects can have a major impact on aqueous solubilities

    Shear thickening of cornstarch suspensions as a re-entrant jamming transition

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    We study the rheology of cornstarch suspensions, a dense system of non-Brownian particles that exhibits shear thickening, i.e. a viscosity that increases with increasing shear rate. Using MRI velocimetry we show that the suspension has a yield stress. From classical rheology it follows that as a function of the applied stress the suspension is first solid (yield stress), then liquid and then solid again when it shear thickens. The onset shear rate for thickening is found to depend on the measurement geometry: the smaller the gap of the shear cell, the lower the shear rate at which thickening occurs. Shear thickening can then be interpreted as the consequence of the Reynolds dilatancy: the system under flow wants to dilate but instead undergoes a jamming transition because it is confined, as confirmed by measurement of the dilation of the suspension as a function of the shear rate

    Dynamical heterogeneity in aging colloidal glasses of Laponite

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    Glasses behave as solids due to their long relaxation time; however the origin of this slow response remains a puzzle. Growing dynamic length scales due to cooperative motion of particles are believed to be central to the understanding of both the slow dynamics and the emergence of rigidity. Here, we provide experimental evidence of a growing dynamical heterogeneity length scale that increases with increasing waiting time in an aging colloidal glass of Laponite. The signature of heterogeneity in the dynamics follows from dynamic light scattering measurements in which we study both the rotational and translational diffusion of the disk-shaped particles of Laponite in suspension. These measurements are accompanied by simultaneous microrheology and macroscopic rheology experiments. We find that rotational diffusion of particles slows down at a faster rate than their translational motion. Such decoupling of translational and orientational degrees of freedom finds its origin in the dynamic heterogeneity since rotation and translation probe different length scales in the sample. The macroscopic rheology experiments show that the low frequency shear viscosity increases at a much faster rate than both rotational and translational diffusive relaxation times.Comment: 12 pages, 5 figures, Accepted in Soft Matter 201

    Photoinduced Changes of Reflectivity in Single Crystals of YBa2Cu3O6.5 (Ortho II)

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    We report measurements of the photoinduced change in reflectivity of an untwinned single crystal of YBa2Cu3O6.5 in the ortho II structure. The decay rate of the transient change in reflectivity is found to decrease rapidly with decreasing temperature and, below Tc, with decreasing laser intensity. We interpret the decay as a process of thermalization of antinodal quasiparticles, whose rate is determined by an inelastic scattering rate of quasiparticle pairs.Comment: 4 pages, 4 figure

    Aging of rotational diffusion in colloidal gels and glasses

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    We study the rotational diffusion of aging Laponite suspensions for a wide range of concentrations using depolarized dynamic light scattering. The measured orientational correlation functions undergo an ergodic to non-ergodic transition that is characterized by a concentration-dependent ergodicity-breaking time. We find that the relaxation times associated with rotational degree of freedom as a function of waiting time, when scaled with their ergodicity-breaking time, collapse on two distinct master curves. These master curves are similar to those previously found for the translational dynamics; The two different classes of behavior were attributed to colloidal gels and glasses. Therefore, the aging dynamics of rotational degree of freedom provides another signature of the distinct dynamical behavior of colloidal gels and glasses.Comment: 12 pages, 7 figure
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