2,370 research outputs found
Entanglement versus mixedness for coupled qubits under a phase damping channel
Quantification of entanglement against mixing is given for a system of
coupled qubits under a phase damping channel. A family of pure initial joint
states is defined, ranging from pure separable states to maximally entangled
state. An ordering of entanglement measures is given for well defined initial
state amount of entanglement.Comment: 9 pages, 2 figures. Replaced with final published versio
Decoherence induced by a phase-damping reservoir
A phase damping reservoir composed by -bosons coupled to a system of
interest through a cross-Kerr interaction is proposed and its effects on
quantum superpo sitions are investigated. By means of analytical calculations
we show that: i-) the reservoir induces a Gaussian decay of quantum coherences,
and ii-) the inher ent incommensurate character of the spectral distribution
yields irreversibility . A state-independent decoherence time and a master
equation are both derived an alytically. These results, which have been
extended for the thermodynamic limit, show that nondissipative decoherence can
be suitably contemplated within the EI D approach. Finally, it is shown that
the same mechanism yielding decoherence ar e also responsible for inducing
dynamical disentanglement.Comment: 8 pages, 3 figure
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Silver-Mediated Fluorination of Functionalized Aryl Stannanes
We report a regiospecific silver-mediated fluorination of aryl stannanes. The presented reaction can afford complex fluoroarenes from readily available phenols in three steps. The operational simplicity and the broad substrate scope of the fluorination should render this reaction a useful tool for the synthesis of milligram to gram quantities of functionalized aryl fluorides. Silver-mediated oxidative transformations of aryl nucleophiles that proceed via bimetallic redox processes are a new avenue to develop carbonâheteroatom bond formations.Chemistry and Chemical Biolog
Mechanism of CâF Reductive Elimination from Palladium(IV) Fluorides
The first systematic mechanism study of CâF reductive elimination from a transition metal complex is described. CâF bond formation from three different Pd(IV) fluoride complexes was mechanistically evaluated. The experimental data suggest that reductive elimination occurs from cationic Pd(IV) fluoride complexes via a dissociative mechanism. The ancillary pyridyl-sulfonamide ligand plays a crucial role for CâF reductive elimination, likely due to a Îș^3 coordination mode, in which an oxygen atom of the sulfonyl group coordinates to Pd. The pyridyl-sulfonamide can support Pd(IV) and has the appropriate geometry and electronic structure to induce reductive elimination
High Resolution Observations of the Massive Protostar in IRAS18566+0408
We report 3 mm continuum, CH3CN(5-4) and 13CS(2-1) line observations with
CARMA, in conjunction with 6 and 1.3 cm continuum VLA data, and 12 and 25
micron broadband data from the Subaru Telescope toward the massive proto-star
IRAS18566+0408. The VLA data resolve the ionized jet into 4 components aligned
in the E-W direction. Radio components A, C, and D have flat cm SEDs indicative
of optically thin emission from ionized gas, and component B has a spectral
index alpha = 1.0, and a decreasing size with frequency proportional to
frequency to the -0.5 power. Emission from the CARMA 3 mm continuum, and from
the 13CS(2-1), and CH3CN(5-4) spectral lines is compact (i.e. < 6700 AU), and
peaks near the position of VLA cm source, component B. Analysis of these lines
indicates hot, and dense molecular gas, typical for HMCs. Our Subaru telescope
observations detect a single compact source, coincident with radio component B,
demonstrating that most of the energy in IRAS18566+0408 originates from a
region of size < 2400 AU. We also present UKIRT near-infrared archival data for
IRAS18566+0408 which show extended K-band emission along the jet direction. We
detect an E-W velocity shift of about 10 km/sec over the HMC in the CH3CN lines
possibly tracing the interface of the ionized jet with the surrounding core
gas. Our data demonstrate the presence of an ionized jet at the base of the
molecular outflow, and support the hypothesis that massive protostars with
O-type luminosity form with a mechanism similar to lower mass stars
Relative Evolutionary Time Scale of Hot Molecular Cores with Respect to Ultra Compact HII Regions
Using the Owens Valley and Nobeyama Radio Observatory interferometers, we
carried out an unbiased search for hot molecular cores and ultracompact UC HII
regions toward the high-mass star forming region G19.61--0.23. In addition, we
performed 1.2 mm imaging with SIMBA, and retrieved 3.5 and 2 cm images from the
VLA archive data base. The newly obtained 3 mm image brings information on a
cluster of high-mass (proto)stars located in the innermost and densest part of
the parsec scale clump detected in the 1.2 mm continuum. We identify a total of
10 high-mass young stellar objects: one hot core (HC) and 9 UC HII regions,
whose physical parameters are obtained from model fits to their continuum
spectra. The ratio between the current and expected final radii of the UC \HII
regions ranges from 0.3 to 0.9, which leaves the possibility that all O-B stars
formed simultaneously. Under the opposite assumption -- namely that star
formation occurred randomly -- we estimate that HC lifetime is less than
1/3 of that of UCHII regions on the basis of the source number ratio
between them.Comment: 13 pages, 2 figs, including a color fi
Global entangling properties of the coupled kicked tops
We study global entangling properties of the system of coupled kicked tops
testing various hypotheses and predictions concerning entanglement in quantum
chaotic systems. In order to analyze the averaged initial entanglement
production rate and the averaged asymptotic entanglement different ensembles of
initial product states are evolved. Two different ensembles with natural
probability distribution are considered: product states of independent
spin-coherent states and product states of arbitrary states. It appears that
the choice of either of these ensembles results in significantly different
averaged entanglement behavior. We investigate also a relation between the
averaged asymptotic entanglement and the mean entanglement of the eigenvectors
of an evolution operator. Lower bound on the averaged asymptotic entanglement
is derived, expressed in terms of the eigenvector entanglement.Comment: 11 pages, 7 figures, RevTe
Structural Design of Back-Plate and its Mechanical Properties in Weld Zones on an Intense Neutron Source for Materials Irradiation
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