5,351 research outputs found
Thermally activated exchange narrowing of the Gd3+ ESR fine structure in a single crystal of Ce1-xGdxFe4P12 (x = 0.001) skutterudite
We report electron spin resonance (ESR) measurements in the Gd3+ doped
semiconducting filled skutterudite compound Ce1-xGdxFe4P12 (x = 0.001). As the
temperature T varies from T = 150 K to T = 165 K, the Gd3+ ESR fine and
hyperfine structures coalesce into a broad inhomogeneous single resonance. At T
= 200 K the line narrows and as T increases further, the resonance becomes
homogeneous with a thermal broadening of 1.1(2) Oe/K. These results suggest
that the origin of these features may be associated to a subtle interdependence
of thermally activated mechanisms that combine: i) an increase with T of the
density of activated conduction-carriers across the T-dependent semiconducting
pseudogap; ii) the Gd3+ Korringa relaxation process due to an exchange
interaction, J_{fd}S.s, between the Gd3+ localized magnetic moments and the
thermally activated conduction-carriers and; iii) a relatively weak confining
potential of the rare-earth ions inside the oversized (Fe2P3)4 cage, which
allows the rare-earths to become rattler Einstein oscillators above T = 148 K.
We argue that the rattling of the Gd3+ ions, via a motional narrowing
mechanism, also contributes to the coalescence of the ESR fine and hyperfine
structure.Comment: 7 pages, 9 figures, accepted for publication in Phys Rev
Site specific spin dynamics in BaFe2As2: tuning the ground state by orbital differentiation
The role of orbital differentiation on the emergence of superconductivity in
the Fe-based superconductors remains an open question to the scientific
community. In this investigation, we employ a suitable microscopic spin probe
technique, namely Electron Spin Resonance (ESR), to investigate this issue on
selected chemically substituted BaFeAs single crystals. As the
spin-density wave (SDW) phase is suppressed, we observe a clear increase of the
Fe 3 bands anisotropy along with their localization at the FeAs plane. Such
an increase of the planar orbital content interestingly occurs independently on
the chemical substitution responsible for suppressing the SDW phase. As a
consequence, the magnetic fluctuations combined with the resultant particular
symmetry of the Fe 3 bands are propitious ingredients to the emergence of
superconductivity in this class of materials.Comment: 6 pages, 5 figure
Unconventional Metallic Magnetism in LaCrSb{3}
Neutron-diffraction measurements in LaCrSb{3} show a coexistence of
ferromagnetic and antiferromagnetic sublattices below Tc=126 K, with ordered
moments of 1.65(4) and 0.49(4) Bohr magnetons per formula unit, respectively
(T=10 K), and a spin reorientation transition at ~95 K. No clear peak or step
was observed in the specific heat at Tc. Coexisting localized and itinerant
spins are suggested.Comment: PRL, in pres
Dependence of nuclear magnetic moments on quark masses and limits on temporal variation of fundamental constants from atomic clock experiments
We calculate the dependence of the nuclear magnetic moments on the quark
masses including the spin-spin interaction effects and obtain limits on the
variation of the fine structure constant and
using recent atomic clock experiments examining hyperfine transitions in H, Rb,
Cs, Yb and Hg and the optical transition in H, Hg and Yb
Spectroscopic Evidence for Multiple Order Parameter Components in the Heavy Fermion Superconductor CeCoIn_5
Point-contact spectroscopy was performed on single crystals of the
heavy-fermion superconductor CeCoIn_5 between 150 mK and 2.5 K. A pulsed
measurement technique ensured minimal Joule heating over a wide voltage range.
The spectra show Andreev-reflection characteristics with multiple structures
which depend on junction impedance. Spectral analysis using the generalized
Blonder-Tinkham-Klapwijk formalism for d-wave pairing revealed two coexisting
order parameter components, with amplitudes Delta_1 = 0.95 +/- 0.15 meV and
Delta_2 = 2.4 +/- 0.3 meV, which evolve differently with temperature. Our
observations indicate a highly unconventional pairing mechanism, possibly
involving multiple bands.Comment: 4 pages, 3 figure
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