1,151 research outputs found

    Resonant charging of Xe clusters in Helium nanodroplets under intense laser fields

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    We theoretically investigate the impact of multiple plasmon resonances on the charging of Xe clusters embedded in He nanodroplets under intense pump-probe laser excitation. Our molecular dynamics simulations on Xe309He10000andcomparisontoresultsforfreeXe309 and comparison to results for free Xe309 give clear evidence for selective resonance heating in the He shell and the Xe cluster, but no corresponding double hump feature in the final Xe charge spectra is found. Though the presence of the He shell substantially increases the maximum charge states, the pump-probe dynamics of the Xe spectra from embedded system is similar to that of the free species. In strong contrast to that, the predicted electron spectra do show well-separated and pronounced features from highly efficient plasmon assisted electron acceleration for both resonances in the embedded clusters. A detailed analysis of the underlying ionization and recombination dynamics is presented and explains the apparent disaccord between the resonance features in the ion and electron spectra.Comment: revised manuscrip

    Ionization heating in rare-gas clusters under intense XUV laser pulses

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    The interaction of intense extreme ultraviolet (XUV) laser pulses (λ=32 nm\lambda=32\rm\,nm, I=1011−14I=10^{11-14}\,W/cm2^2) with small rare-gas clusters (Ar147_{147}) is studied by quasi-classical molecular dynamics simulations. Our analysis supports a very general picture of the charging and heating dynamics in finite samples under short-wavelength radiation that is of relevance for several applications of free-electron lasers. First, up to a certain photon flux, ionization proceeds as a series of direct photoemission events producing a jellium-like cluster potential and a characteristic plateau in the photoelectron spectrum as observed in [Bostedt {\it et al.}, Phys. Rev. Lett. {\bf 100}, 013401 (2008)]. Second, beyond the onset of photoelectron trapping, nanoplasma formation leads to evaporative electron emission with a characteristic thermal tail in the electron spectrum. A detailed analysis of this transition is presented. Third, in contrast to the behavior in the infrared or low vacuum ultraviolet range, the nanoplasma energy capture proceeds via {\it ionization heating}, i.e., inner photoionization of localized electrons, whereas collisional heating of conduction electrons is negligible up to high laser intensities. A direct consequence of the latter is a surprising evolution of the mean energy of emitted electrons as function of laser intensity.Comment: figure problems resolve

    An architecture for rule based system explanation

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    A system architecture is presented which incorporate both graphics and text into explanations provided by rule based expert systems. This architecture facilitates explanation of the knowledge base content, the control strategies employed by the system, and the conclusions made by the system. The suggested approach combines hypermedia and inference engine capabilities. Advantages include: closer integration of user interface, explanation system, and knowledge base; the ability to embed links to deeper knowledge underlying the compiled knowledge used in the knowledge base; and allowing for more direct control of explanation depth and duration by the user. User models are suggested to control the type, amount, and order of information presented

    From/To: Walter Fennel (Chalk\u27s reply filed first)

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    From/To: Walter Fennel (Chalk\u27s reply filed first)

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