391 research outputs found
Spin-Wave and Electromagnon Dispersions in Multiferroic MnWO4 as Observed by Neutron Spectroscopy: Isotropic Heisenberg Exchange versus Anisotropic Dzyaloshinskii-Moriya Interaction
High resolution inelastic neutron scattering reveals that the elementary
magnetic excitations in multiferroic MnWO4 consist of low energy dispersive
electromagnons in addition to the well-known spin-wave excitations. The latter
can well be modeled by a Heisenberg Hamiltonian with magnetic exchange coupling
extending to the 12th nearest neighbor. They exhibit a spin-wave gap of 0.61(1)
meV. Two electromagnon branches appear at lower energies of 0.07(1) meV and
0.45(1) meV at the zone center. They reflect the dynamic magnetoelectric
coupling and persist in both, the collinear magnetic and paraelectric AF1
phase, and the spin spiral ferroelectric AF2 phase. These excitations are
associated with the Dzyaloshinskii-Moriya exchange interaction, which is
significant due to the rather large spin-orbit coupling.Comment: 8 pages, 6 figures, accepted for publication in Physical Review
Revisiting the ground state of CoAlO: comparison to the conventional antiferromagnet MnAlO
The A-site spinel material, CoAl2O4, is a physical realization of the
frustrated diamond-lattice antiferromagnet, a model in which is predicted to
contain unique incommensurate or `spin-spiral liquid' ground states. Our
previous single-crystal neutron scattering study instead classified it as a
`kinetically-inhibited' antiferromagnet, where the long ranged correlations of
a collinear Neel ground state are blocked by the freezing of domain wall motion
below a first-order phase transition at T* = 6.5 K. The current paper expands
on our original results in several important ways. New elastic and inelastic
neutron measurements are presented that show our initial conclusions are
affected by neither the sample measured nor the instrument resolution, while
measurements to temperatures as low as T = 250 mK limit the possible role being
played by low-lying thermal excitations. Polarized diffuse neutron measurements
confirm reports of short-range antiferromagnetic correlations and diffuse
streaks of scattering, but major diffuse features are explained as signatures
of overlapping critical correlations between neighboring Brillouin zones.
Finally, and critically, this paper presents detailed elastic and inelastic
measurements of magnetic correlations in a single-crystal of MnAl2O4, which
acts as an unfrustrated analogue to CoAl2O4. The unfrustrated material is shown
to have a classical continuous phase transition to Neel order at T_N = 39 K,
with collective spinwave excitations and Lorentzian-like critical correlations
which diverge at the transition. Direct comparison between the two compounds
indicates that CoAl2O4 is unique, not in the nature of high-temperature diffuse
correlations, but rather in the nature of the frozen state below T*. The higher
level of cation inversion in the MnAl2O4 sample indicates that this novel
behavior is primarily an effect of greater next-nearest-neighbor exchange.Comment: 13 pages, 8 figures, acccepted for publication in Physical Review
Competing exchange interactions on the verge of a metal-insulator transition in the two-dimensional spiral magnet SrFeO
We report a neutron scattering study of the magnetic order and dynamics of
the bilayer perovskite SrFeO, which exhibits a temperature-driven
metal-insulator transition at 340 K. We show that the Fe moments adopt
incommensurate spiral order below K and provide a
comprehensive description of the corresponding spin wave excitations. The
observed magnetic order and excitation spectra can be well understood in terms
of an effective spin Hamiltonian with interactions ranging up to third
nearest-neighbor pairs. The results indicate that the helical magnetism in
SrFeO results from competition between ferromagnetic
double-exchange and antiferromagnetic superexchange interactions whose
strengths become comparable near the metal-insulator transition. They thus
confirm a decades-old theoretical prediction and provide a firm experimental
basis for models of magnetic correlations in strongly correlated metals.Comment: PRL, in pres
Role of commensurate and incommensurate low-energy excitations in the paramagnetic to hidden-order transition of URuSi
We report low-energy inelastic neutron scattering data of the paramagnetic
(PM) to hidden-order (HO) phase transition at in
URuSi. While confirming previous results for the HO and PM phases, our
data reveal a pronounced wavevector dependence of low-energy excitations across
the phase transition. To analyze the energy scans we employ a damped harmonic
oscillator model containing a fit parameter which is expected to
diverge at a second-order phase transition. Counter to expectations the
excitations at show an abrupt step-like suppression of
below , whereas excitations at , associated
with large-moment antiferromagnetism (LMAF) under pressure, show an enhancement
and a pronounced peak of at . Therefore, at the critical HO
temperature , LMAF fluctuations become nearly critical as well. This is
the behavior expected of a super-vector order parameter with nearly degenerate
components for the HO and LMAF leading to nearly isotropic fluctuations in the
combined order-parameter space.Comment: 6 pages; v3 accepted journal version; minor modifications compared to
v
Theory of Superconducting of doped fullerenes
We develop the nonadiabatic polaron theory of superconductivity of
taking into account the polaron band narrowing and realistic
electron-phonon and Coulomb interactions. We argue that the crossover from the
BCS weak-coupling superconductivity to the strong-coupling polaronic and
bipolaronic superconductivity occurs at the BCS coupling constant independent of the adiabatic ratio, and there is nothing ``beyond'' Migdal's
theorem except small polarons for any realistic electron-phonon interaction. By
the use of the polaronic-type function and the ``exact'' diagonalization in the
truncated Hilbert space of vibrons (``phonons'') we calculate the ground state
energy and the electron spectral density of the molecule. This
allows us to describe the photoemission spectrum of in a wide
energy region and determine the electron-phonon interaction. The strongest
coupling is found with the high-frequency pinch mode and with the
Frenkel exciton. We clarify the crucial role of high-frequency bosonic
excitations in doped fullerenes which reduce the bare bandwidth and the Coulomb
repulsion allowing the intermediate and low-frequency phonons to couple two
small polarons in a Cooper pair. The Eliashberg-type equations are solved for
low-frequency phonons. The value of the superconducting , its pressure
dependence and the isotope effect are found to be in a remarkable agreement
with the available experimental data.Comment: 20 pages, Latex, 4 figures available upon reques
Midinfrared Conductivity in Orientationally Disordered Doped Fullerides
The coupling between the intramolecular vibrational modes and the doped
conduction electrons in is studied by a calculation of the
electronic contributions to the phonon self energies. The calculations are
carried out for an orientationally ordered reference solid with symmetry and for a model with quenched orientational disorder on the
fullerene sites. In both cases, the dispersion and symmetry of the renormalized
modes is governed by the electronic contributions. The current current
correlation functions and frequency dependent conductivity through the
midinfrared are calculated for both models. In the disordered structures, the
renormalized modes derived from even parity intramolecular phonons are resonant
with the dipole excited single particle spectrum, and modulate the predicted
midinfrared conductivity. The spectra for this coupled system are calculated
for several recently proposed microscopic models for the electron phonon
coupling, and a comparison is made with recent experimental data which
demonstrate this effect.Comment: 32 pages + 9 postscript figures (on request), REVTeX 3.
Jahn-Teller polarons and their superconductivity in a molecular conductor
We present a theoretical study of a possibility of superconductivity in a
three dimensional molecular conductor in which the interaction between
electrons in doubly degenerate molecular orbitals and an {\em intra}molecular
vibration mode is large enough to lead to the formation of
Jahn-Teller small polarons. We argue that the effective polaron-polaron
interaction can be attractive for material parameters realizable in molecular
conductors. This interaction is the source of superconductivity in our model.
On analyzing superconducting instability in the weak and strong coupling
regimes of this attractive interaction, we find that superconducting transition
temperatures up to 100 K are achievable in molecular conductors within this
mechanism. We also find, for two particles per molecular site, a novel Mott
insulating state in which a polaron singlet occupies one of the doubly
degenerate orbitals on each site. Relevance of this study in the search for new
molecular superconductors is pointed out.Comment: Submitted to Phys. Rev.
Superconductivity in Ce- and U-based "122" heavy-fermion compounds
This review discusses the heavy-fermion superconductivity in Ce- and U-based
compounds crystallizing in the body-centered tetragonal ThCr2Si2 structure.
Special attention will be paid to the theoretical background of these systems
which are located close to a magnetic instability.Comment: 12 pages, 9 figures. Invited topical review (special issue on "Recent
Developments in Superconductivity") Metadata and references update
Financial diversification before modern portfolio theory: UK financial advice documents in the late nineteenth and the beginning of the twentieth century
The paper offers textual evidence from a series of financial advice documents in the late nineteenth century and the early twentieth century of how UK investors perceived of and managed risk. In the world’s largest financial centre of the time, UK investors were familiar with the concept of correlation and financial advisers’ suggestions were consistent with the recommendations of modern portfolio theory in relation to portfolio selection strategies. From the 1870s, there was an increased awareness of the benefits of financial diversification - primarily putting equal amounts into a number of different securities - with much of the emphasis being on geographical rather than sectoral diversification and some discussion of avoiding highly correlated investments. Investors in the past were not so naïve as mainstream financial discussions suggest today
A Public Option for the Core
This paper is focused not on the Internet architecture – as defined by layering, the narrow waist of IP, and other core design principles – but on the Internet infrastructure, as embodied in the technologies and organizations that provide Internet service. In this paper we discuss both the challenges and the opportunities that make this an auspicious time to revisit how we might best structure the Internet’s infrastructure. Currently, the tasks of transit-between-domains and last-mile-delivery are jointly handled by a set of ISPs who interconnect through BGP. In this paper we propose cleanly separating these two tasks. For transit, we propose the creation of a “public option” for the Internet’s core backbone. This public option core, which complements rather than replaces the backbones used by large-scale ISPs, would (i) run an open market for backbone bandwidth so it could leverage links offered by third-parties, and (ii) structure its terms-of-service to enforce network neutrality so as to encourage competition and reduce the advantage of large incumbents
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