A 4-Component Dirac Theory of Ionization of Hydrogen Molecular Ion in a Super-Intense Laser Field

In this paper a 4-component Dirac theory of ionization of hydrogen molecular ion in a super-intense laser field is developed. Simple analytic expressions for the spin specific as well as the total ionization currents emitted from the ground state of the ion are derived. The results are given for all polarization and finite propagation vectors of the field. They apply for inner-shell ionization of analogous heavier molecular ions as well. The presence of molecular two-slit interference effect, first found in the non-relativistic case, and the spin-flip ionization current, and an asymmetry of the up- and down-spin currents similar to that predicted in the atomic case, are found also to hold for the present relativistic molecular ionic case. Finally, the possibility of controlling the dominant spin currents by selecting the handedness of a circularly polarized incident laser field is pointed out.Comment: 7 pages, no figure

Autoionization of H2 near threshold

Autoionization of H2 near threshol

Interplay of polarization geometry and rotational dynamics in high harmonic generation from coherently rotating linear molecule

Recent reports on intense-field pump-probe experiments for high harmonic generation from coherently rotating linear molecules, have revealed remarkable characteristic effects of the simultaneous variation of the polarization geometry and the time delay on the high harmonic signals. We analyze the effects and give a unified theoretical account of the experimental observationsComment: 4 pages, 5 figure

Multiphoton excitations in vibrational rotational states of diatomic molecules in intense electromagnetic field

A theory is presented and a calculational procedure is outlined for evaluating transition amplitudes of multiphoton excitations of vibrational-rotational levels in diatomic molecules. This theory can be utilized in studying behavior of molecules in intense electromagnetic fields

Vibro-rotational excitations of H2/+/ by e/+/ impact - A semi-classical approach

Semiclassical approach to vibrorotational excitations of H2/+/ by positron impac

Geometric phases in open tripod systems

We first consider stimulated Raman adibatic passages (STIRAP) in a closed four-level tripod system. In this case, the adiabatic eigenstates of the system acquire real geometric phases. When the system is open and subject to decoherence they acquire complex geometric phases that we determine by a Monte Carlo wave function approach. We calculate the geometric phases and the state evolution in the closed as well as in the open system cases and describe the deviation between these in terms of the phases acquired. When the system is closed, the adiabatic evolution implements a Hadamard gate. The open system implements an imperfect gate and hence has a fidelity below unity. We express this fidelity in terms of the acquired geometric phases.Comment: 10 pages 7 figure

Attosecond probing of instantaneous AC Stark shifts in helium atoms

Based on numerical solutions of the time-dependent Schr\"odinger equation for either one or two active electrons, we propose a method for observing instantaneous level shifts in an oscillating strong infrared (IR) field in time, using a single tunable attosecond pulse to probe excited states of the perturbed atom. The ionization probability in the combined fields depends on both, the frequency of the attosecond pulse and the time delay between both pulses, since the IR field shifts excited energy levels into and out of resonance with the attosecond probe pulse. We show that this method (i) allows the detection of instantaneous atomic energy gaps with sub-laser-cycle time resolution and (ii) can be applied as an ultrafast gate for more complex processes such as non-sequential double-ionization