1,304 research outputs found
Anomalously slow spin dynamics and short-range correlations in the quantum spin ice systems Yb2Ti2O7 and Yb2Sn2O7
We report a positive muon spin relaxation and rotation (\muSR) study of the
quantum spin ice materials Yb2Ti2O7 and Yb2Sn2O7 focusing on the low field
response. In agreement with earlier reports, data recorded in small
longitudinal fields evidence anomalously slow spin dynamics in the microsecond
range below the temperature T_c at which the specific heat displays an intense
peak, namely T_c = 0.24 K and 0.15 K, respectively, for the two systems. We
found that slow dynamics extends above T_c up to at least 0.7 K for both
compounds. The conventional dynamical Gaussian Kubo-Toyabe model describes the
\muSR spectra recorded above T_c. At lower temperatures a published analytical
extension of the Gaussian Kubo-Toyabe model provides a good description,
consistent with the existence of short-range magnetic correlations. While the
physical response of the two systems is qualitatively the same, Yb2Ti2O7
exhibits a much larger local magnetic susceptibility than Yb2Sn2O7 below T_c.
Considering previously reported ac susceptibility, neutron scattering and \muSR
results, we suggest the existence of anomalously slow spin dynamics to be a
common physical property of pyrochlore magnetic materials. The possibility of
molecular spin substructures to be associated to the slow dynamics and
therefore the short-range correlations is mentioned. The slow spin dynamics
observed under field does not exclude the presence of much faster dynamics
detected in extremely low or zero field.Comment: 11 pages, 10 figure
Highly efficient multilayer organic pure-blue-light emitting diodes with substituted carbazoles compounds in the emitting layer
Bright blue organic light-emitting diodes (OLEDs) based on
1,4,5,8,N-pentamethylcarbazole (PMC) and on dimer of N-ethylcarbazole
(N,N'-diethyl-3,3'-bicarbazyl) (DEC) as emitting layers or as dopants in a
4,4'-bis(2,2'-diphenylvinyl)-1,1'-biphenyl (DPVBi) matrix are described. Pure
blue-light with the C.I.E. coordinates x = 0.153 y = 0.100, electroluminescence
efficiency \eta_{EL} of 0.4 cd/A, external quantum efficiency \eta_{ext.} of
0.6% and luminance L of 236 cd/m2 (at 60 mA/cm2) were obtained with PMC as an
emitter and the 2,9-dimethyl-4,7-diphenyl-1,10-phenantroline (BCP) as a
hole-blocking material in five-layer emitting devices. The highest efficiencies
\eta_{EL.} of 4.7 cd/A, and \eta_{ext} = 3.3% were obtained with a four-layer
structure and a DPVBi DEC-doped active layer (CIE coordinates x = 0.158,
y=0.169, \lambda_{peak} = 456 nm). The \eta_{ext.} value is one the highest
reported at this wavelength for blue OLEDs and is related to an internal
quantum efficiency up to 20%
BaCu3O4: High Temperature Magnetic Order in One-Dimensional S=1/2 Diamond-Chains
The magnetic properties of the alkaline earth oxocuprate BaCu3O4 are
investigated. We show that the characteristic Cu3O4 layers of this material can
be described with diamond chains of antiferromagnetically coupled Cu 1/2 spins
with only a weak coupling between two adjacent chains. These Cu3O4 layers seem
to represent a so far unique system of weakly coupled one-dimensional magnetic
objects where the local AF ordering of the Cu2+ ions leads to an actual net
magnetic moment of an isolated diamond chain. We demonstrate a magnetic
transition at a high N\'eel temperature T_{N}=336 K
The Neonatal Development of Intraepithelial and Lamina Propria Lymphocytes in the Murine Small Intestine
During early neonatal life, important changes occur in the gut. The intestine is challenged by
both milk and a microbial flora. Later on, at weaning, the diet of mice changes from milk to
pelleted food leading to changes in microbial contents. This period seems essential for a complete
development of the mucosal immune system. We investigated the development of both
intraepithelial (IEL) and lamina propria lymphocytes (LPL), from day 5, and every 5 days, up
to day 30 after birth. IEL and LPL were isolated from the small intestine and the phenotype
was assessed by FACS analyses, using antibodies for detection of T-cell markers CD3,
TCRαβ, TCRγδ, CD4, CD8α, CD8β, CD5, CD18, CD54, and CD49d. Our data show a clear
increase in the number of LPL just before weaning, while the number of IEL increased after
day 15. A more mature pattern of membrane antigen expression of both IEL and LPL was observed
at weaning. The adhesion molecules CD18, CD54, and CD49d, essential for cellular
communication of lymphocytes, showed an expression peak at weaning. In conclusion, the
mouse mucosal immune system develops during the first 3 weeks of neonatal life leading to
the formation of a more mature immune system at weaning
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Atmospheric Mars Entry and Landing Investigations & Analysis (AMELIA) by ExoMars 2016 Schiaparelli Entry Descent Module
Incommensurate spin density wave in Co-doped BaFe2As2
57Fe Mossbauer spectroscopy measurements are presented in the underdoped
Ba(Fe{1-x}Cox)2As2 series for x=0.014 (T_c < 1.4K) and x=0.03 and 0.045 (T_c ~
2 and 12K respectively). The spectral shapes in the so-called spin-density wave
(SDW) phase are interpreted in terms of incommensurate modulation of the
magnetic structure, and allow the shape of the modulation to be determined. In
undoped BaFe2As2, the magnetic structure is commensurate, and we find that
incommensurability is present at the lowest doping level (x=0.014). As Co
doping increases, the low temperature modulation progressively loses its
"squaredness" and tends to a sine-wave. The same trend occurs for a given
doping level, as temperature increases. We find that a magnetic hyperfine
component persists far above the SDW transition, its intensity being
progressively tranferred to a paramagnetic component on heating.Comment: 7 pages, 8 figures, published in EP
Local Approach of the Charpy Test at Low Temperature
Charpy V-notch impact testing is widely used in the toughness assessment of large forged components, e.g. the pressure vessel for pressurised water reactors (PWR). At low temperature, A508 Cl.3 nuclear pressure vessel steel fails by cleavage fracture. The results reported here are part of both an experimental program and numerical investigations which aim at the establishment of a non-empirical relationship between the lower shelf Charpy V-notch energy, CVN, and the fracture toughness, KIc, of this material. Here, the applicability of the Beremin cleavage fracture model to the Charpy specimen is demonstrated
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