The global atmospheric electrical circuit and climate

Evidence is emerging for physical links among clouds, global temperatures, the global atmospheric electrical circuit and cosmic ray ionisation. The global circuit extends throughout the atmosphere from the planetary surface to the lower layers of the ionosphere. Cosmic rays are the principal source of atmospheric ions away from the continental boundary layer: the ions formed permit a vertical conduction current to flow in the fair weather part of the global circuit. Through the (inverse) solar modulation of cosmic rays, the resulting columnar ionisation changes may allow the global circuit to convey a solar influence to meteorological phenomena of the lower atmosphere. Electrical effects on non-thunderstorm clouds have been proposed to occur via the ion-assisted formation of ultra-fine aerosol, which can grow to sizes able to act as cloud condensation nuclei, or through the increased ice nucleation capability of charged aerosols. Even small atmospheric electrical modulations on the aerosol size distribution can affect cloud properties and modify the radiative balance of the atmosphere, through changes communicated globally by the atmospheric electrical circuit. Despite a long history of work in related areas of geophysics, the direct and inverse relationships between the global circuit and global climate remain largely quantitatively unexplored. From reviewing atmospheric electrical measurements made over two centuries and possible paleoclimate proxies, global atmospheric electrical circuit variability should be expected on many timescale

Experimental study of aerosol release following liquid leaks of fission products concentrates simulants

International audienceThis article presents an experimental study that encompasses a need for nuclear safety on the consequences of a leakage of fission products (FP) concentrates in a failed vessel during spent fuel reprocessing operations. Particulate airborne release fractions (ARFs), as the result of liquid FP simulants impacting a rigid surface, were assessed for two circular leakage geometries of 1 and 2 mm diameter. The detailed analysis of these ARFs which are between 2.7 × 10−5 and 5.2 × 10−5 for the different experimental configurations revealed their dependence on the surface tension and the viscosity of the solutions, as well as on the impacting jet diameter. The study also makes it possible to develop an empirical correlation that links the ARFs with the dimensionless Ohnesorge and Weber numbers in the considered surface tension and viscosity range

Study of the coalescence/splash threshold of droplet impact on liquid films and its relevance in assessing airborne particle release

International audienceImpingement of droplets on surfaces occurs in many industrial and natural processes. The study of droplet break-up is fundamental in order to determine the potential sources of airborne contamination for scenarios of hazardous liquid falls such as dripping. There are very few data in the literature describing the case of impact of millimetre-size droplets. The purposes of this work were to study experimentally particle emission during the impact of droplets on a liquid film and to assess the use of coalescence/splash relations to predict airborne particle release. The results are described using dimensionless numbers taking into account the inertial, viscosity and surface tension forces. Experiments were carried out for Weber numbers between 62 and 1754 and for Ohnesorge numbers between 2.0×10 -3 and 1.5×10 -2. New results on coalescence/splash thresholds are obtained using highly sensitive aerosol measurement and allow a prediction concerning the presence or absence of airborne particles according to a threshold relation. Moreover, we propose a modification of the Cossali et al.'s [1] relation in order to describe the coalescence/prompt splash threshold. © 2011 Elsevier Inc

Parameter study of microdroplet formation by impact of millimetre-size droplets onto a liquid film

The objective of this work is to carry out an experimental investigation on the influence of different parameters such as liquid properties (viscosity and liquid-gas surface tension), impacting droplet properties (velocity vi and diameter di) and the thickness of liquid film on the emission of airborne particles produced by the impact of millimetre-size droplets onto a liquid film. Our results show that in the variation range studied, the increase of vi and di or the decrease in liquid film thickness produces an increase in the mean number of microdroplets emitted by impact in the size range 2-50 μm. Furthermore, it was also observed that an increase in viscosity involves a steep decrease in the mean number of microdroplets emitted. These microdroplets may be produced by the fingers pinching of the crown formed during impact. In the case of low surface tension liquid, the formation of bubbles involves high production of droplets smaller than 15 μm. The results presented here constitute a database of the micro-droplets produced to validate models of droplet impact outcomes. © 2009 Elsevier Ltd. All rights reserved

Study of airborne particles produced by normal impact of millimetric droplets onto a liquid film

The aim of this work is to carry out an experimental investigation into the generation of airborne microparticles when millimetric droplets of aqueous solutions impact onto a liquid film. Impact experiments using 3.9 mm diameter droplets were carried out for Weber numbers between 159 and 808, with a fixed Ohnesorge number of 2 × 10-3 and film parameters S f (the ratio between the thickness of the liquid film h film and the diameter of the impacting droplet d i) between 0.3 and 1. Observed results show that the deposition/splashing threshold is independent of the parameter S f in agreement with the data in the literature. The aerosol measurement results demonstrate the production of solid particles from the evaporation of secondary microdroplets with diameters less than 30 μm formed when splash occurs. The median diameter of these microdroplets is around 20 μm, corresponding to a value of d 50/d i = 5 × 10-3. Taken together, the results show that the mass and the number of particles emitted increase as the Weber number increases. Moreover, at a Weber number of 808, the results show that the mass and number of particles emitted increases as the parameter S f decreases. In this case, the mean number of microdroplets emitted per impact is equal to 14 for S f = 1 and equal to 76 for S f = 0.3

Performance assessment of probes dedicated to the monitoring of surface particle contamination

International audienceSurface probes, based on airflow particle detachment coupled with optical particle counter, are actually available to measure the particle cleanliness of surfaces in cleanroom. No reliable data exits dealing with the performance assessment of these probes in unstuck and counting particles deposited on surfaces. This work presents a method for determining the efficiency of instruments dedicated to particle surface cleanliness measurements. The method is based on the realisation of standard particle deposits by sedimentation and analysis of whole of the contaminated surface by microscopy combined with a micrometric displacement bench. The method is used to assess a trial surface probe with 30 μm and 80 μm glass beads deposited on transparent (glass) or opaque (aluminium) surfaces at concentrations ranging from 1 particle·cm-2 to 50 particles·cm -2. The results obtained show that the overall efficiency of the instrument tested is less than 5 %. The detailed analysis of results shows that this low value is mainly due to poor efficiency of sampling and detection of particles in the optical counter. When analysed in terms of particle detachment efficiency, the results agree qualitatively with a force balance analysis taking into account the friction by airflow and the distribution of adhesion forces of glass particles to glass substrates or rough aluminium substrates. Such result shows that airflow based surface probes for particle cleanliness measurements should be systematically qualified for representative conditions of operations whereas analytical microscopy measurements could be considered as reference. Copyright © 2012 WILEY-VCH Verlag GmbH andamp; Co. KGaA, Weinheim

Mobilization of tungsten dust by electric forces and its bearing on tritiated particles in the ITER tokamak

International audienceExperimental investigations on the electric field strength required to overcome the adhesion forces of micron size tungsten metallic dust as well as silver and aluminum oxide in powdery form deposited on a conductive surface are presented. The results reveal a strong influence of particulate surface properties on the detachment threshold, especially for tungsten particles which exhibit a thin surface oxide layer that screens their electrical conductivity. Such tungsten particles makes possible that electrostatic self-charging occurs when tritiated because of their dielectric properties even if there are deposited on a conductive grounded surface. © 2017 Elsevier B.V

Theoretical and experimental approach for the determination of the gyration / mobility ratio of soot representative diameters

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Aerosol characterization and particle scrubbing efficiency of underwater operations during laser cutting of steel components for dismantling of nuclear facilities

International audienceThe goal of this article is to provide results on aerosol particles emissions of a laser Nd:YAG cutting technique used for the decommissioning of nuclear facilities. In particular, the study aims at characterizing the aerosol emitted during the cutting of steel specimens of different thicknesses and to study particulate emissions for cuts in air and under water. To do so, we calculate the emitted aerosol mass per unit area of cut. Overall, it was found that the mass of aerosol per unit area of cut by laser cutting decreases when the laser power and cutting speed increase. We also examine the performance of the height of the water column above the cut on the particle collection efficiency. We found that the driving phenomenon for particle collection is the scrubbing of particles by bubbles present in the water column. When cuts are realized under water, the production of aerosol particles mass per unit area of cut is reduced by a factor of 10 and limited below 70 g m–2. © Taiwan Association for Aerosol Research

Increase in thermophoretic velocity of carbon aggregates as a function of particle size

WOS:000342541100008International audienceThe Radial Flow Thermophoretic Analyser developed by Brugiere et al. (2013) is used to measure the thermophoretic velocity of carbon nanoparticle aggregates produced by combustion with a propane/air diffusion flame. This work is carried out within the scope of the evaluation of aerosol deposition by thermophoresis for nuclear power plant fire risk assessment purposes. Thermophoretic velocity measurements are performed on monodisperse particles with electrical mobility diameters ranging from 30 nm to 600 nm and for a temperature gradient equal to 50 750 K/m. The results obtained show an increase in thermophoretic velocity as a function of the mobility diameter, contrary to what is observed for spherical particles in the transition regime. When the thermophoretic velocity is expressed as a function of the number of primary particles making up the aggregates, a good agreement is found with the experimental results of Messerer et al. (2003). Measurements performed with the Radial Flow Thermophoretic Analyser show, for the first time, an increase in the thermophoretic velocity of carbon aggregates as a function of the number of primary particles, in qualitative agreement with the Monte Carlo simulation results of Mackowski (2006). (C) 2014 Elsevier Ltd. All rights reserved