130 research outputs found
Non Thermal Plasma Sources of Production of Active Species for Biomedical Uses: Analyses, Optimization and Prospect
Simulation of the discharge propagation in a capillary tube in air at atmospheric pressure
International audienceThis paper presents simulations of an air plasma discharge at atmospheric pressure initiated by a needle anode set inside a dielectric capillary tube. We have studied the influence of the tube inner radius and its relative permittivity ε r on the discharge structure and dynamics. As a reference, we have used a relative permittivity ε r = 1 to study only the influence of the cylindrical constraint of the tube on the discharge. For a tube radius of 100 µm and ε r = 1, we have shown that the discharge fills the tube during its propagation and is rather homogeneous behind the discharge front. When the radius of the tube is in the range 300 to 600 µm, the discharge structure is tubular with peak values of electric field and electron density close to the dielectric surface. When the radius of the tube is larger than 700 µm, the tube has no influence on the discharge which propagates axially. For a tube radius of 100 µm, when ε r increases from 1 to 10, the discharge structure becomes tubular. We have noted that the velocity of propagation of the discharge in the tube increases when the front is more homogeneous and then, the discharge velocity increases with the decrease of the tube radius and ε r. Then, we have compared the relative influence of the value of tube radius and ε r on the discharge characteristics. Our simulations indicate that the geometrical constraint of the cylindrical tube has more influence than the value of ε r on the discharge structure and dynamics. Finally, we have studied the influence of photoemission processes on the discharge structure by varying the photoemission coefficient. As expected, we have shown that photoemission, as it increases the number of secondary electrons close to the dielectric surface, promotes the tubular structure of the discharge
High-order fluid model for streamer discharges: II. Numerical solution and investigation of planar fronts
Spatiotemporally resolved imaging of streamer discharges in air generated in a wire-cylinder reactor with (sub)nanosecond voltage pulses
We use (sub)nanosecond high-voltage pulses to generate streamers in atmospheric-pressure air in
a wire-cylinder reactor. We study the effect of reactor length, pulse duration, pulse amplitude,
pulse polarity, and pulse rise time on the streamer development, specifically on the streamer
distribution in the reactor to relate it to plasma-processing results. We use ICCD imaging with a
fully automated setup that can image the streamers in the entire corona-plasma reactor. From the
images, we calculate streamer lengths and velocities. We also develop a circuit simulation model
of the reactor to support the analysis of the streamer development. The results show how the
propagation of the high-voltage pulse through the reactor determines the streamer development.
As the pulse travels through the reactor, it generates streamers and attenuates and disperses. At
the end of the reactor, it reflects and adds to itself. The local voltage on the wire together with the
voltage rise time determine the streamer velocities, and the pulse duration the consequent
maximal streamer length
Prise en compte de l'anisotropie des collisions ion-atome sur le transport des ions par simulation de Monte-Carlo
This paper is devoted to the determination of the differential and integral collision cross sections needed for the calculation of the transport coefficient of ions in weakly ionized gases. In the case of Ar/Ar system and for energy interval varying up to 100 eV, the cross sections are obtained from the interaction potential of polarization for low energies and of Lennard-Jones for higher energies. The calculation method of the collision cross sections based on the classical mechanics has been first validated from comparisons of measured and calculated differential cross sections. Then, these cross sections have been used in a Monte-Carlo code for simulation of the transport of Ar ions in Ar gas at room temperature (300 K). The obtained transport coefficients (ion mobility, drift velocity and diffusion coefficient) are in good agreement with the drift tube measurements given in the literature thus confirming the validity of the method of collision cross section calculation.Cet article est consacré à la détermination des sections efficaces différentielles et intégrales ion-atome nécessaires au calcul des coefficients de transport des ions dans les gaz faiblement ionisés. Dans le cas du système Ar/Ar et pour des intervalles d'énergie allant jusqu'à quelques dizaines d'eV, les sections efficaces sont obtenues à partir des potentiels d'interaction de polarisation pour les faibles énergies et de Lennard-Jones pour les énergies plus élevées. La méthode de calcul des sections efficaces basée sur la mécanique classique a d'abord été validée par comparaison des sections efficaces différentielles mesurées et calculées. Ensuite, ces sections efficaces ont été utilisées dans un code de simulation statistique de Monte-Carlo du transport des ions Ar dans l'Argon à la température ambiante (300 K). Les coefficients de transport (vitesse de dérive, mobilité ionique et coefficient de diffusion) obtenus sont en bon accord avec les mesures de tube de dérive de la littérature confirmant ainsi la validation de la méthode de détermination des sections efficaces
Ion swarm data of N
The ion swarm data such as reduced mobilities, diffusion coefficients and
reaction rates of N4+ in N2, O2 and dry air (80%
N2, 20% O2) have been determined from a Monte Carlo simulation
using calculated and measured elastic and inelastic cross sections. The
elastic cross sections used have been determined from a semi-classical JWKB
approximation based on a rigid core potential model. The inelastic cross
section of N4+ in N2 has been deduced from the measured
experimental rates whereas for N4+ in O2 the measured
inelastic cross sections have been extended to low and high energies by
appropriate approximations. Then the cross sections sets have been validated
from comparison of calculated and measured ion swarm data. From the cross
sections sets obtained in pure N2 and O2, the ion swarm data for
N4+ in dry air are then calculated for a large E/N range
[1–104] Td. Finally, the influence of N4+ ions on the
streamer development was analyzed with a 2D fluid model in the case of dry
air at atmospheric pressure for a point-to-plane electrode configuration
2D simulation of active species and ozone production in a multi-tip DC air corona discharge
The present paper shows for the first time in the literature a complete 2D simulation of the ozone production in a DC positive multi-tip to plane corona discharge reactor crossed by a dry air flow at atmospheric pressure. The simulation is undertaken until 1 ms and involves tens of successive discharge and post-discharge phases. The air flow is stressed by several monofilament corona discharges generated by a maximum of four anodic tips distributed along the reactor. The nonstationary hydrodynamics model for reactive gas mixture is solved using the commercial FLUENT software. During each discharge phase, thermal and vibrational energies as well as densities of radical and metastable excited species are locally injected as source terms in the gas medium surrounding each tip. The chosen chemical model involves 10 neutral species reacting following 24 reactions. The obtained results allow us to follow the cartography of the temperature and the ozone production inside the corona reactor as a function of the number of high voltage anodic tips
Optical and electrical analyses of DC positive corona discharge in N
This paper presents an experimental analysis of the electrical and optical
behaviour of positive point-plane corona discharges. The measurements of the
instantaneous corona current and the current-voltage characteristics are
used with the imagery analyses (CCD and streak camera) to determine the
streamer properties such as the streamer morphology and velocity with the
primary and secondary streamer developments. These analyses are performed
first in synthetic air as a function of operating parameters such the
applied voltage. Then the effect of gas mixtures (several proportions of
N2, O2 with or without CO2) is analysed. When the gas
concentration is varied the discharge morphology, the shape and amplitude of
the corona current are significantly affected due to the variation of the
gas electronegativity following its composition and concentration
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