Frustration effects in magnetic molecules

Besides being a fascinating class of new materials, magnetic molecules provide the opportunity to study concepts of condensed matter physics in zero dimensions. This contribution will exemplify the impact of molecular magnetism on concepts of frustrated spin systems. We will discuss spin rings and the unexpected rules that govern their low-energy behavior. Rotational bands, which are experimentally observed in various molecular magnets, provide a useful, simplified framework for characterizing the energy spectrum, but there are also deviations thereof with far-reaching consequences. It will be shown that localized independent magnons on certain frustrated spin systems lead to giant magnetization jumps, a new macroscopic quantum effect. In addition a frustration-induced metamagnetic phase transitions will be discussed, which demonstrates that hysteresis can exist without anisotropy. Finally, it is demonstrated that frustrated magnetic molecules could give rise to an enhanced magnetocaloric effect.Comment: 6 pages, 4 figures; submitted to J. Low. Temp. Phys.; proceedings of the Sixth International Symposium on Crystalline Organic Metals, Superconductors, and Ferromagnets (ISCOM

Density Matrix Functional Calculations for Matter in Strong Magnetic Fields: I. Atomic Properties

We report on a numerical study of the density matrix functional introduced by Lieb, Solovej and Yngvason for the investigation of heavy atoms in high magnetic fields. This functional describes {\em exactly} the quantum mechanical ground state of atoms and ions in the limit when the nuclear charge $Z$ and the electron number $N$ tend to infinity with $N/Z$ fixed, and the magnetic field $B$ tends to infinity in such a way that $B/Z^{4/3}\to\infty$. We have calculated electronic density profiles and ground state energies for values of the parameters that prevail on neutron star surfaces and compared them with results obtained by other methods. For iron at $B=10^{12}$ G the ground state energy differs by less than 2 \% from the Hartree-Fock value. We have also studied the maximal negative ionization of heavy atoms in this model at various field strengths. In contrast to Thomas-Fermi type theories atoms can bind excess negative charge in the density matrix model. For iron at $B=10^{12}$ G the maximal excess charge in this model corresponds to about one electron.Comment: Revtex, 13 pages with 6 eps figures include

Symmetry Properties on Magnetization in the Hubbard Model at Finite Temperatures

By making use of some symmetry properties of the relevant Hamiltonian, two fundamental relations between the ferromagnetic magnetization and a spin correlation function are derived for the $d (=1,2,3)$-dimensional Hubbard model at finite temperatures. These can be viewed as a kind of Ward-Takahashi identities. The properties of the magnetization as a function of the applied field are discussed. The results thus obtained hold true for both repulsive and attractive on-site Coulomb interactions, and for arbitrary electron fillings.Comment: Latex file, no figur

Impact of long-range interactions on the disordered vortex lattice

The interaction between the vortex lines in a type-II superconductor is mediated by currents. In the absence of transverse screening this interaction is long-ranged, stiffening up the vortex lattice as expressed by the dispersive elastic moduli. The effect of disorder is strongly reduced, resulting in a mean-squared displacement correlator = characterized by a mere logarithmic growth with distance. Finite screening cuts the interaction on the scale of the London penetration depth \lambda and limits the above behavior to distances R<\lambda. Using a functional renormalization group (RG) approach, we derive the flow equation for the disorder correlation function and calculate the disorder-averaged mean-squared relative displacement \propto ln^{2\sigma} (R/a_0). The logarithmic growth (2\sigma=1) in the perturbative regime at small distances [A.I. Larkin and Yu.N. Ovchinnikov, J. Low Temp. Phys. 34, 409 (1979)] crosses over to a sub-logarithmic growth with 2\sigma=0.348 at large distances.Comment: 9 pages, no figure

Generalized hole-particle transformations and spin reflection positivity in multi-orbital systems

We propose a scheme combining spin reflection positivity and generalized hole-particle and orbital transformations to characterize the symmetry properties of the ground state for some correlated electron models on bipartite lattices. In particular, we rigorously determine at half-filling and for different regions of the parameter space the spin, orbital and $\eta$ pairing pseudospin of the ground state of generalized two-orbital Hubbard models which include the Hund's rule coupling.Comment: 6 pages, 2 figure

Aspects of radiative K^+_e3 decays

We re-investigate the radiative charged kaon decay K+- --> pi0 e+- nu_e gamma in chiral perturbation theory, merging the chiral expansion with Low's theorem. We thoroughly analyze the precision of the predicted branching ratio relative to the non-radiative decay channel. Structure dependent terms and their impact on differential decay distributions are investigated in detail, and the possibility to see effects of the chiral anomaly in this decay channel is emphasized.Comment: 15 pages, 6 figure

Magnetic and Dynamic Properties of the Hubbard Model in Infinite Dimensions

An essentially exact solution of the infinite dimensional Hubbard model is made possible by using a self-consistent mapping of the Hubbard model in this limit to an effective single impurity Anderson model. Solving the latter with quantum Monte Carlo procedures enables us to obtain exact results for the one and two-particle properties of the infinite dimensional Hubbard model. In particular we find antiferromagnetism and a pseudogap in the single-particle density of states for sufficiently large values of the intrasite Coulomb interaction at half filling. Both the antiferromagnetic phase and the insulating phase above the N\'eel temperature are found to be quickly suppressed on doping. The latter is replaced by a heavy electron metal with a quasiparticle mass strongly dependent on doping as soon as $n<1$. At half filling the antiferromagnetic phase boundary agrees surprisingly well in shape and order of magnitude with results for the three dimensional Hubbard model.Comment: 32 page

Phase diagrams of spin ladders with ferromagnetic legs

The low-temperature properties of the spin S=1/2 ladder with anisotropic ferromagnetic legs are studied using the continuum limit bosonization approach. The weak-coupling ground state phase diagram of the model is obtained for a wide range of coupling constants and several unconventional gapless ''spin-liquid'' phases are shown to exist for ferromagnetic coupling. The behavior of the ladder system in the vicinity of the ferromagnetic instability point is discussed in detail.Comment: 11 pages, 4 figure

Symmetry breaking in the Hubbard model at weak coupling

The phase diagram of the Hubbard model is studied at weak coupling in two and three spatial dimensions. It is shown that the Neel temperature and the order parameter in d=3 are smaller than the Hartree-Fock predictions by a factor of q=0.2599. For d=2 we show that the self-consistent (sc) perturbation series bears no relevance to the behavior of the exact solution of the Hubbard model in the symmetry-broken phase. We also investigate an anisotropic model and show that the coupling between planes is essential for the validity of mean-field-type order parameters

Persistent Currents in Small, Imperfect Hubbard Rings

We have done a study with small, imperfect Hubbard rings with exact diagonalization. The results for few-electron rings show, that the imperfection, whether localized or not, nearly always decrease, but can also \emph{increase} the persistent current, depending on the character of the imperfection and the on-site interaction. The calculations are generally in agreement with more specialized studies. In most cases the electron spin plays an important role.Comment: 6 pages, 4 figure