Experimental Verification of the Chemical Sensitivity of Two-Site Double Core-Hole States Formed by an X-ray FEL

We have performed X-ray two-photon photoelectron spectroscopy (XTPPS) using the Linac Coherent Light Source (LCLS) X-ray free-electron laser (FEL) in order to study double core-hole (DCH) states of CO2, N2O and N2. The experiment verifies the theory behind the chemical sensitivity of two-site (ts) DCH states by comparing a set of small molecules with respect to the energy shift of the tsDCH state and by extracting the relevant parameters from this shift.Comment: 11 pages, 2 figure

Observation of Two-Dimensional Longitudinal-Transverse Correlations in an Electron Beam by Laser-Electron Interactions

During the preparatory work for the optical-replica synthesizer experiment in the free-electron laser FLASH at DESY, we were able to superimpose a short, approximately 200 fs long pulse from a frequency-doubled mode-locked erbium laser with titanium-sapphire amplifier and an approximately 20 ps long electron bunch in an undulator. This induces an energy modulation in a longitudinal slice of the electron bunch. A magnetic chicane downstream of the undulator converts the energy modulation into a density modulation within the slice that causes the emission of coherent optical transition radiation from a silver-coated silicon screen. Varying the relative timing between electron and laser, we use a camera to record two-dimensional images of the slices as a function of the longitudinal position within the electron bunch

The soft X-ray laser project at MAX IV

A Soft X-ray Laser (SXL) beamline utilising FEL technology is being designed for the Short Pulse Facility (SPF) at the MAX IV Laboratory. A conceptual design study has been started following on the scientific case already prepared in collaboration between several Swedish Universities and driven by a strong (Swedish) user demand. The baseline goal of the SXL beamline is to generate intense and short pulses in the range 1-5 nm (0.2-1 keV). The system is building on the MAX IV linac system, already today providing 100 fs 3 GeV and pulses compressed to 100 fs for other applications within the SPF. As a special feature we foresee a variety of pump-probe capabilities