Spin Anisotropy and Slow Dynamics in Spin Glasses

We report on an extensive study of the influence of spin anisotropy on spin glass aging dynamics. New temperature cycle experiments allow us to compare quantitatively the memory effect in four Heisenberg spin glasses with various degrees of random anisotropy and one Ising spin glass. The sharpness of the memory effect appears to decrease continuously with the spin anisotropy. Besides, the spin glass coherence length is determined by magnetic field change experiments for the first time in the Ising sample. For three representative samples, from Heisenberg to Ising spin glasses, we can consistently account for both sets of experiments (temperature cycle and magnetic field change) using a single expression for the growth of the coherence length with time.Comment: 4 pages and 4 figures - Service de Physique de l'Etat Condense CNRS URA 2464), DSM/DRECAM, CEA Saclay, Franc

Memory interference effects in spin glasses

When a spin glass is cooled down, a memory of the cooling process is imprinted in the spin structure. This memory can be disclosed in a continuous heating measurement of the ac-susceptibility. E.g., if a continuous cooling process is intermittently halted during a certain aging time at one or two intermediate temperatures, the trace of the previous stop(s) is recovered when the sample is continuously re-heated [1]. However, heating the sample above the aging temperature, but keeping it below Tg, erases the memory of the thermal history at lower temperatures. We also show that a memory imprinted at a higher temperature can be erased by waiting a long enough time at a lower temperature. Predictions from two complementary spin glass descriptions, a hierarchical phase space model and a real space droplet picture are contested with these memory phenomena and interference effects. [1] K. Jonason, E. Vincent, J. Hammann, J. P. Bouchaud and P. Nordblad, Phys. Rev. Lett. 31, 3243 (1998).Comment: 7 pages, 1 LaTex file + 5 figures in EPS Revised version of June 17, 1999 (minor changes), to appear in EPJ B around November 9

Low-Temperature Features of Nano-Particle Dynamics

In view of better characterizing possible quantum effects in the dynamics of nanometric particles, we measure the effect on the relaxation of a slight heating cycle. The effect of the field amplitude is studied; its magnitude is chosen in order to induce the relaxation of large particles (~7nm), even at very low temperatures (100mK). Below 1K, the results significantly depart from a simple thermal dynamics scenario.Comment: 1 tex file, 4 PostScript figure

A new experimental procedure for characterizing quantum effects in small magnetic particle systems

A new experimental procedure is discussed, which aims at separating thermal from quantum behavior independently of the energy barrier distribution in small particle systems. Magnetization relaxation data measured between 60 mK and 5 K on a sample of nanoparticles is presented. The comparison between experimental data and numerical calculations shows a clear departure from thermal dynamics for our sample, which was not obvious without using the new procedure presented here.Comment: LaTeX source, 6 pages, 5 PostScript figure

Disentangling Distribution Effects and Nature of the Dynamics in Relaxation Measurements: the RMR Method

URL: http://www-spht.cea.fr/articles/s00/004 (sur invitation). Comment séparer les effets de distribution et la nature de la dynamique dans des mesures de relaxation magnétiques: la méthode RMRWe discuss here the nature of the low temperature magnetic relaxation in samples of magnetic nanoparticles. In addition to usual magnetic viscosity measurement, we have used the Residual Memory Ratio (RMR) method. This procedure enables us to overcome the uncertainties usually associated with the energy barrier distribution, thus giving a more detailed insight on the nature of the observed dynamics. A custom made apparatus coupling dilution refrigeration and SQUID magnetometry allowed measurements of very diluted samples at temperatures ranging between 60mK and 7K. Two types of particles have been studied: $\gamma$-Fe$_2$O$_3$ of moderate anisotropy, and CoFe$_2$O$_4$ of higher anisotropy where quantum effects are more likely to occur. In both cases, the data cannot simply be interpreted in terms of mere thermally activated dynamics of independent particles. The deviation from thermal activation seems to go opposite of what is expected from the possible effect of particle interactions. We therefore believe that it suggests the occurrence of quantum dynamics at very low temperatures

Aging in the Relaxor Ferroelectric PMN/PT

The relaxor ferroelectric (PbMn$_{1/3}$Nb$_{2/3}$O$_3$)$_{1-x}$(PbTiO$_3$)$_{x}$, $x=0.1$, (PMN/PT(90/10)) is found to exhibit several regimes of complicated aging behavior. Just below the susceptibility peak there is a regime exhibiting rejuvenation but little memory. At lower temperature, there is a regime with mainly cumulative aging, expected for simple domain-growth. At still lower temperature, there is a regime with both rejuvenation and memory, reminiscent of spin glasses. PMN/PT (88/12) is also found to exhibit some of these aging regimes. This qualitative aging behavior is reminiscent of that seen in reentrant ferromagnets, which exhibit a crossover from a domain-growth ferromagnetic regime into a reentrant spin glass regime at lower temperatures. These striking parallels suggest a picture of competition in PMN/PT (90/10) between ferroelectric correlations formed in the domain-growth regime with glassy correlations formed in the spin glass regime. PMN/PT (90/10) is also found to exhibit frequency-aging time scaling of the time-dependent part of the out-of-phase susceptibility for temperatures 260 K and below. The stability of aging effects to thermal cycles and field perturbations is also reported.Comment: 8 pages RevTeX4, 11 figures; submitted to Phys. Rev.