36 research outputs found
Optimized fabrication of high quality La0.67Sr0.33MnO3 thin films considering all essential characteristics
In this article, an overview of the fabrication and properties of high
quality La0.67Sr0.33MnO3 (LSMO) thin films is given. A high quality LSMO film
combines a smooth surface morphology with a large magnetization and a small
residual resistivity, while avoiding precipitates and surface segregation. In
literature, typically only a few of these issues are adressed. We therefore
present a thorough characterization of our films, which were grown by pulsed
laser deposition. The films were characterized with reflection high energy
electron diffraction, atomic force microscopy, x-ray diffraction, magnetization
and transport measurements, x-ray photoelectron spectroscopy and scanning
transmission electron microscopy. The films have a saturation magnetization of
4.0 {\mu}B/Mn, a Curie temperature of 350 K and a residual resistivity of 60
{\mu}{\Omega}cm. These results indicate that high quality films, combining both
large magnetization and small residual resistivity, were realized. A comparison
between different samples presented in literature shows that focussing on a
single property is insufficient for the optimization of the deposition process.
For high quality films, all properties have to be adressed. For LSMO devices,
the thin film quality is crucial for the device performance. Therefore, this
research is important for the application of LSMO in devices.Comment: Accepted for publication in Journal of Physics D - Applied Physic
Work function changes in the double layered manganite La1.2Sr1.8Mn2O7
We have investigated the behaviour of the work function of La1.2Sr1.8Mn2O7 as
a function of temperature by means of photoemission. We found a decrease of 55
+/- 10 meV in going from 60 K to just above the Curie temperature (125 K) of
the sample. Above T_C the work function appears to be roughly constant. Our
results are exactly opposite to the work function changes calculated from the
double-exchange model by Furukawa, but are consistent with other measurements.
The disagreement with double-exchange can be explained using a general
thermodynamic relation valid for second order transitions and including the
extra processes involved in the manganites besides double-exchange interaction.Comment: 6 pages, 4 figures included in tex
Doping induced metal-insulator transition in two-dimensional Hubbard, , and extended Hubbard, , models
We show numerically that the nature of the doping induced metal-insulator
transition in the two-dimensional Hubbard model is radically altered by the
inclusion of a term, , which depends upon a square of a single-particle
nearest-neighbor hopping. This result is reached by computing the localization
length, , in the insulating state. At finite values of we find
results consistent with where is
the critical chemical potential. In contrast, for the Hubbard model. At finite values of , the presented
numerical results imply that doping the antiferromagnetic Mott insulator leads
to a superconductor.Comment: 19 pages (latex) including 7 figures in encapsulated postscript
format. Submitted for publication in Phys. Rev.
Metallic ferromagnetism without exchange splitting
In the band theory of ferromagnetism there is a relative shift in the
position of majority and minority spin bands due to the self-consistent field
due to opposite spin electrons. In the simplest realization, the Stoner model,
the majority and minority spin bands are rigidly shifted with respect to each
other. Here we consider models at the opposite extreme, where there is no
overall shift of the energy bands. Instead, upon spin polarization one of the
bands broadens relative to the other. Ferromagnetism is driven by the resulting
gain in kinetic energy. A signature of this class of mechanisms is that a
transfer of spectral weight in optical absorption from high to low frequencies
occurs upon spin polarization. We show that such models arise from generalized
tight binding models that include off-diagonal matrix elements of the Coulomb
interaction. For certain parameter ranges it is also found that reentrant
ferromagnetism occurs. We examine properties of these models at zero and finite
temperatures, and discuss their possible relevance to real materials
Superconductivity in the two dimensional Hubbard Model.
Quasiparticle bands of the two-dimensional Hubbard model are calculated using
the Roth two-pole approximation to the one particle Green's function. Excellent
agreement is obtained with recent Monte Carlo calculations, including an
anomalous volume of the Fermi surface near half-filling, which can possibly be
explained in terms of a breakdown of Fermi liquid theory. The calculated bands
are very flat around the (pi,0) points of the Brillouin zone in agreement with
photoemission measurements of cuprate superconductors. With doping there is a
shift in spectral weight from the upper band to the lower band. The Roth method
is extended to deal with superconductivity within a four-pole approximation
allowing electron-hole mixing. It is shown that triplet p-wave pairing never
occurs. Singlet d_{x^2-y^2}-wave pairing is strongly favoured and optimal
doping occurs when the van Hove singularity, corresponding to the flat band
part, lies at the Fermi level. Nearest neighbour antiferromagnetic correlations
play an important role in flattening the bands near the Fermi level and in
favouring superconductivity. However the mechanism for superconductivity is a
local one, in contrast to spin fluctuation exchange models. For reasonable
values of the hopping parameter the transition temperature T_c is in the range
10-100K. The optimum doping delta_c lies between 0.14 and 0.25, depending on
the ratio U/t. The gap equation has a BCS-like form and (2*Delta_{max})/(kT_c)
~ 4.Comment: REVTeX, 35 pages, including 19 PostScript figures numbered 1a to 11.
Uses epsf.sty (included). Everything in uuencoded gz-compressed .tar file,
(self-unpacking, see header). Submitted to Phys. Rev. B (24-2-95
Properties of lightly doped t-J two-leg ladders
We have numerically investigated the doped t-J ladder using exact
diagonalization. We have studied both the limit of strong inter-chain coupling
and isotropic coupling. The ladder scales to the Luther-Emery liquid regime in
the strong inter-chain coupling limit. In this strong coupling limit there is a
simple picture of the excitation spectrum that can be continued to explain the
behavior at isotropic coupling. At J=0 we have indications of a ferromagnetic
ground state. At a large the ladder is phase separated into holes and a
Heisenberg ladder. At intermediate coupling the ground state shows hole pairing
with a modified d-wave symmetry. The excitation spectrum separates into a
limited number of quasiparticles which carry charge and spin and a triplet magnon mode. At half-filling the former vanish but the latter
evolves continuously into the magnon band of the spin liquid. At low doping the
quasiparticles form a dilute Fermi gas with a strong attraction but
simultaneously the Fermi wave vector, as would be measured in photoemission, is
large. The dynamical structure factors are calculated and are found to be very
similar to calculations on 2D clusters
Quantum Monte Carlo Evidence for d-wave Pairing in the 2D Hubbard Model at a van Hove Singularity
We implement a Quantum Monte Carlo calculation for a repulsive Hubbard model
with nearest and next-nearest neighbor hopping interactions on clusters up to
12x12. A parameter region where the Fermi level lies close to the van Hove
singularity at the Saddle Points in the bulk band structure is investigated. A
pairing tendency in the symmetry channel, but no other channel,
is found. Estimates of the effective pairing interaction show that it is close
to the value required for a 40 K superconductor. Finite-size scaling compares
with the attractive Hubbard model.Comment: 11 pages, REVTex, 4 figures, postscrip
Hole Doping Evolution of the Quasiparticle Band in Models of Strongly Correlated Electrons for the High-T_c Cuprates
Quantum Monte Carlo (QMC) and Maximum Entropy (ME) techniques are used to
study the spectral function of the one band Hubbard model
in strong coupling including a next-nearest-neighbor electronic hopping with
amplitude . These values of parameters are chosen to improve the
comparison of the Hubbard model with angle-resolved photoemission (ARPES) data
for . A narrow quasiparticle (q.p.) band is observed in the
QMC analysis at the temperature of the simulation , both at and away
from half-filling. Such a narrow band produces a large accumulation of weight
in the density of states at the top of the valence band. As the electronic
density decreases further away from half-filling, the chemical
potential travels through this energy window with a large number of states, and
by it has crossed it entirely. The region near momentum
and in the spectral function is more sensitive to doping
than momenta along the diagonal from to . The evolution with
hole density of the quasiparticle dispersion contains some of the features
observed in recent ARPES data in the underdoped regime. For sufficiently large
hole densities the ``flat'' bands at cross the Fermi energy, a
prediction that could be tested with ARPES techniques applied to overdoped
cuprates. The population of the q.p. band introduces a {\it hidden} density in
the system which produces interesting consequences when the quasiparticles are
assumed to interact through antiferromagnetic fluctuations and studied with the
BCS gap equation formalism. In particular, a region of extended s-wave is found
to compete with d-wave in the overdoped regime, i.e. when the chemical
potential has almost entirely crossed the q.p.Comment: 14 pages, Revtex, with 13 embedded ps figures, submitted to Phys.
Rev. B., minor modifications in the text and in figures 1b, 2b, 3b, 4b, and
6
Interlayer hopping properties of electrons in layered metals
A formalism is proposed to study the electron tunneling between extended
states, based on the spin-boson Hamiltonian previously used in two-level
systems. It is applied to analyze the out--of--plane tunneling in layered
metals considering different models. By studying the effects of in--plane
interactions on the interlayer tunneling of electrons near the Fermi level, we
establish the relation between departure from Fermi liquid behavior driven by
electron correlations inside the layer and the out of plane coherence. Response
functions, directly comparable with experimental data are obtained
The Hubbard model within the equations of motion approach
The Hubbard model has a special role in Condensed Matter Theory as it is
considered as the simplest Hamiltonian model one can write in order to describe
anomalous physical properties of some class of real materials. Unfortunately,
this model is not exactly solved except for some limits and therefore one
should resort to analytical methods, like the Equations of Motion Approach, or
to numerical techniques in order to attain a description of its relevant
features in the whole range of physical parameters (interaction, filling and
temperature). In this manuscript, the Composite Operator Method, which exploits
the above mentioned analytical technique, is presented and systematically
applied in order to get information about the behavior of all relevant
properties of the model (local, thermodynamic, single- and two- particle ones)
in comparison with many other analytical techniques, the above cited known
limits and numerical simulations. Within this approach, the Hubbard model is
shown to be also capable to describe some anomalous behaviors of the cuprate
superconductors.Comment: 232 pages, more than 300 figures, more than 500 reference